Publications by authors named "Vandembroucq D"

We study plastic strain during individual avalanches in overdamped particle-scale molecular dynamics (MD) and mesoscale elastoplastic models (EPM) for amorphous solids sheared in the athermal quasistatic limit. We show that the spatial correlations in plastic activity exhibit a short length scale that grows as t^{3/4} in MD and ballistically in EPM, which is generated by mechanical excitation of nearby sites not necessarily close to their stability thresholds, and a longer lengthscale that grows diffusively for both models and is associated with remote marginally stable sites. These similarities in spatial correlations explain why simple EPMs accurately capture the size distribution of avalanches observed in MD, though the temporal profiles and dynamical critical exponents are quite different.

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While optical fibers display excellent performances in the infrared, visible and ultraviolet ranges remain poorly addressed by them. Obtaining better fibers for the short-wavelength range has been restricted, in all fiber optics, by scattering processes. In hollow-core fibers, the scattering loss arises from the core roughness and represents the limiting factor for loss reduction regardless of the cladding confinement power.

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While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this dramatic slowdown is key for understanding the glass transition. Here, we show by atomistic simulations that the heterogeneous dynamics of glass-forming liquids strongly correlate with the local residual plastic strengths along soft directions computed in the initial inherent structures.

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We develop a mesoscopic model to study the plastic behavior of an amorphous material under cyclic loading. The model is depinning-like and driven by a disordered thresholds dynamics that is coupled by long-range elastic interactions. We propose a simple protocol of "glass preparation" that allows us to mimic thermalization at high temperatures as well as aging at vanishing temperature.

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We present results on an automaton model of an amorphous solid under cyclic shear. After a transient, the steady state falls into one of three cases in order of increasing strain amplitude: (i) pure elastic behavior with no plastic activity, (ii) limit cycles where the state recurs after an integer period of strain cycles, and (iii) irreversible plasticity with longtime diffusion. The number of cycles N required for the system to reach a periodic orbit diverges as the amplitude approaches the yielding transition between regimes (ii) and (iii) from below, while the effective diffusivity D of the plastic strain field vanishes on approach from above.

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We study the structural origin of the Bauschinger effect by accessing numerically the local plastic thresholds in the steady state flow of a two-dimensional model glass under athermal quasistatic deformation. More specifically, we compute the local residual strength, Δτ^{c}, for arbitrary loading orientations and find that plastic deformation generically induces material polarization, i.e.

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We measure the local yield stress, at the scale of small atomic regions, in a deeply quenched two-dimensional glass model undergoing shear banding in response to athermal quasistatic deformation. We find that the occurrence of essentially a single plastic event suffices to bring the local yield stress distribution to a well-defined value for all strain orientations, thus essentially erasing the memory of the initial structure. It follows that in a well-relaxed sample, plastic events cause the abrupt (nucleation-like) emergence of a local softness contrast and thus precipitate the formation of a band, which, in its early stages, is measurably softer than the steady-state flow.

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We provide new insights into the molecular origin of the asymmetry between uniaxial tensile and compressive deformation of glassy and semicrystalline polymers using molecular dynamics simulations. The difference between the two responses strongly depends on the chain length and is the largest at intermediate chain lengths. Irrespective of chain length, the intra- and interchain organization of polymers under extension and compression are remarkably distinct.

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We present results on a mesoscale model for amorphous matter in athermal, quasistatic (a-AQS), steady-state shear flow. In particular, we perform a careful analysis of the scaling with the lateral system size L of (i) statistics of individual relaxation events in terms of stress relaxation S, and individual event mean-squared displacement M, and the subsequent load increments Δγ, required to initiate the next event; (ii) static properties of the system encoded by x=σ_{y}-σ, the distance of local stress values from threshold; and (iii) long-time correlations and the emergence of diffusive behavior. For the event statistics, we find that the distribution of S is similar to, but distinct from, the distribution of M.

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We present results on tagged particle diffusion in a mesoscale lattice model for sheared amorphous material in athermal quasistatic conditions. We find a short time diffusive regime and a long time diffusive regime whose diffusion coefficients depend on system size in dramatically different ways. At short time, we find that the diffusion coefficient, D, scales roughly linearly with system length, D∼L^{1.

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We study the quasistatic penetration of a flexible beam into a two-dimensional dense granular medium lying on a horizontal plate. Rather than a buckling-like behavior we observe a transition between a regime of crack-like penetration in which the fiber only shows small fluctuations around a stable straight geometry and a bending regime in which the fiber fully bends and advances through series of loading and unloading steps. We show that the shape reconfiguration of the fiber is controlled by a single nondimensional parameter L/L_{c}, which is the ratio of the length of the flexible beam L to L_{c}, a bending elastogranular length scale that depends on the rigidity of the fiber and on the departure from the jamming packing fraction of the granular medium.

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Metrological atomic force microscopy measurements are performed on the silica glass interfaces of photonic band-gap fibers and hollow capillaries. The freezing of attenuated out-of-equilibrium capillary waves during the drawing process is shown to result in a reduced surface roughness. The roughness attenuation with respect to the expected thermodynamical limit is determined to vary with the drawing stress following a power law.

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We present optical and atomic force microscopy measurements of the roughness of the core wall surface within a hollow core photonic bandgap fiber (HC-PBGF) over the [3×10  μm-30  μm] spatial frequency range. A recently developed immersion optical profilometry technique with picometer-scale sensitivity was used to measure the roughness of air-glass surfaces inside the fiber at unprecedentedly low spatial frequencies, which are known to have the highest impact on HC-PBGF scattering loss and, thus, determine their loss limit. Optical access to the inner surface of the core was obtained by the selective filling of the cladding holes with index matching liquid using techniques borrowed from micro-fluidics.

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The crucial role of hydrodynamic pinch-off instabilities is evidenced in the coarsening stage of viscous liquids. The phase separation of a barium borosilicate glass melt is studied by in situ synchrotron tomography at high temperature. The high viscosity contrast between the less viscous phase and the more viscous phase induces a topological symmetry breaking: capillary breakups occur preferentially in the less viscous phase.

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In model amorphous solids produced via differing quench protocols, a strong correlation is established between local yield stress measured by direct local probing of shear stress thresholds and the plastic rearrangements observed during remote loading in shear. This purely local measure shows a higher predictive power for identifying sites of plastic activity when compared with more conventional structural properties. Most importantly, the sites of low local yield stress, thus defined, are shown to be persistent, remaining predictive of deformation events even after fifty or more such plastic rearrangements.

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A mesoscopic model of amorphous plasticity is discussed in the context of depinning models. After embedding in a d+1-dimensional space, where the accumulated plastic strain lives along the additional dimension, the gradual plastic deformation of amorphous media can be regarded as the motion of an elastic manifold in a disordered landscape. While the associated depinning transition leads to scaling properties, the quadrupolar Eshelby interactions at play in amorphous plasticity induce specific additional features like shear-banding and weak ergodicity breakdown.

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We discuss the plastic behavior of an amorphous matrix reinforced by hard particles. A mesoscopic depinning-like model accounting for Eshelby elastic interactions is implemented. Only the effect of a plastic disorder is considered.

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A differential profilometry technique is adapted to the problem of measuring the roughness of hollow glass fibres by use of immersion objectives and index-matching liquid. The technique can achieve picometer level sensitivity. Cross validation with AFM measurements is obtained through use of vitreous silica step calibration samples.

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X-ray microtomography was used to follow the coarsening of the structure of a ternary silicate glass experiencing phase separation in the liquid state. The volumes, surfaces, mean, and Gaussian curvatures of the domains of minority phase were measured after reconstruction of the 3D images and segmentation. A linear growth law of the characteristic length scale ℓ∼t was observed.

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The larger structures are, the lower their mechanical strength. Already discussed by Leonardo da Vinci and Edmé Mariotte several centuries ago, size effects on strength remain of crucial importance in modern engineering for the elaboration of safety regulations in structural design or the extrapolation of laboratory results to geophysical field scales. Under tensile loading, statistical size effects are traditionally modeled with a weakest-link approach.

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The propagation of an adhesive crack through an anisotropic heterogeneous interface is considered. Tuning the local toughness distribution function and spatial correlation is numerically shown to induce a transition between weak to strong pinning conditions. While the macroscopic effective toughness is given by the mean local toughness in the case of weak pinning, a systematic toughness enhancement is observed for strong pinning (the critical point of the depinning transition).

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We discuss avalanche and finite-size fluctuations in a mesoscopic model to describe the shear plasticity of amorphous materials. Plastic deformation is assumed to occur through series of local reorganizations. Yield stress criteria are random while each plastic slip event induces a quadrupolar long-range elastic stress redistribution.

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Amorphous silica density at ambient pressure is known to depend on thermal history (through the quenching rate) but also, at room temperature, on the maximum pressure applied in the past. Here we show that beyond density, a mechanical loading can endow the structure with an orientational order. Molecular dynamics simulations show evidence that amorphous silica develops a permanent anisotropic structure after extended shear plastic flow.

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We perform fracture experiments on nanoscale phase-separated glasses and measure crack surface roughness by atomic force microscopy. The ability of tuning the phase domain size by thermal treatment allows us to test thoroughly the predictions of crack front depinning models about the scaling properties of crack surface roughness. It appears that, in the range of validity of these depinning models developed for the fracture of brittle materials, our experimental results show a quantitative agreement with theoretical predictions: Beyond the characteristic size of disorder, the roughness of crack surfaces obeys the logarithmic scaling early predicted by Ramanathan, Ertaş, and Fisher [Phys.

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