Determination of plasma properties in liquid jets through time-resolved experiments on third harmonic reflection dynamics.

The study of plasma in liquid jets represents a significant area of research encompassing plasma science, dynamics, and properties. This paper presents experimental studies on plasma formation processes in liquid jets of water, ethanol, and isopropyl based on the dynamics of the third harmonic (TH) reflection from the induced plasma. Through time-resolved experiments, and theoretical estimations using the Keldysh theory, plasma properties including density and frequency for all three media are evaluated.

Controlling water giant low-inertia nonlinear refractive index in the THz frequency range via temperature variation.

To create self-controlled radiation photonics systems, it is necessary to have complete information about the nonlinear properties of the materials used. In this Letter, the vibrational mechanism of the giant low-inertia cubic nonlinearity of the refractive index of water in the terahertz (THz) frequency range is experimentally proven. Its dominance, which manifests itself when the temperature of the liquid changes, is demonstrated.

Revealing the nature of optical activity in carbon dots produced from different chiral precursor molecules.

Carbon dots (CDs) are light-emitting nanoparticles that show great promise for applications in biology and medicine due to the ease of fabrication, biocompatibility, and attractive optical properties. Optical chirality, on the other hand, is an intrinsic feature inherent in many objects in nature, and it can play an important role in the formation of artificial complexes based on CDs that are implemented for enantiomer recognition, site-specific bonding, etc. We employed a one-step hydrothermal synthesis to produce chiral CDs from the commonly used precursors citric acid and ethylenediamine together with a set of different chiral precursors, namely, L-isomers of cysteine, glutathione, phenylglycine, and tryptophan.

Hyperspectral data denoising for terahertz pulse time-domain holography.

We investigated data denoising in hyperspectral terahertz pulse time-domain holography. Using the block-matching algorithms adapted for spatio-temporal and spatio-spectral volumetric data we studied and optimized parameters of these algorithms to improve phase image reconstruction quality. We propose a sequential application of the two algorithms oriented on work in temporal and spectral domains.

Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle.

Luminescent molecules attached to resonant colloidal particles are an important tool to study light-matter interaction. A traditional approach to enhance the photoluminescence intensity of the luminescent molecules in such conjugates is to incorporate spacer-coated plasmonic nanoantennas, where the spacer prevents intense non-radiative decay of the luminescent molecules. Here, we explore the capabilities of an alternative platform for photoluminescence enhancement, which is based on low-loss Mie-resonant colloidal silicon particles.

Resonant silicon nanoparticles for enhancement of light absorption and photoluminescence from hybrid perovskite films and metasurfaces.

Recently, hybrid halide perovskites have emerged as one of the most promising types of materials for thin-film photovoltaic and light-emitting devices because of their low-cost and potential for high efficiency. Further boosting their performance without detrimentally increasing the complexity of the architecture is critically important for commercialization. Despite a number of plasmonic nanoparticle based designs having been proposed for solar cell improvement, inherent optical losses of the nanoparticles reduce photoluminescence from perovskites.

Self-adjusted all-dielectric metasurfaces for deep ultraviolet femtosecond pulse generation.

The advantage of metasurfaces and nanostructures with a high nonlinear response is that they do not require phase matching, and the generated pulses are short in the time domain without additional pulse compression. However, the fabrication of large-scale planar structures by lithography-based methods is expensive, time consuming, and requires complicated preliminary simulations to obtain the most optimized geometry. Here, we propose a novel strategy for the self-assembled fabrication of large-scale resonant metasurfaces, where incident femtosecond laser pulses adjust the initial silicon films via specific surface deformation to be as resonant as possible for a given wavelength.

Direct measurement of the parameters of a femtosecond pulse train with a THz repetition rate generated by the interference of two phase-modulated femtosecond pulses.

A femtosecond pulse train with THz repetition rate generated by the interference of two phase-modulated pulses has been recorded experimentally. Pulse repetition rates and their duration have been measured. It has been shown that at the 50-fs time delay between phase-modulated pulses the repetition rate is 3.