Earth is constantly bombarded with extraterrestrial dust containing invaluable information about extraterrestrial processes, such as structure formation by stellar explosions or nucleosynthesis, which could be traced back by long-lived radionuclides. Here, we report the very first detection of a recent ^{60}Fe influx onto Earth by analyzing 500 kg of snow from Antarctica by accelerator mass spectrometry. By the measurement of the cosmogenically produced radionuclide ^{53}Mn, an atomic ratio of ^{60}Fe/^{53}Mn=0.
View Article and Find Full Text PDFIn the frame of studies on the safe disposal of nuclear waste, there is a great interest for understanding the migration behavior of Tc. Tc originating from nuclear energy production and global fallout shows environmental levels down to 10 atoms/g of soil (∼2 fg/g). Extremely low concentrations are also expected in groundwater after diffusion of Tc through the bentonite constituting the technical barrier for nuclear waste disposal.
View Article and Find Full Text PDFThe Mn flux onto Earth is a quantity relevant for different extraterrestrial and astrophysical questions. It is a proxy for related fluxes, such as supernova-produced material or interplanetary dust particles. In this work, we performed a first attempt to assess the Mn flux by measuring the Mn/Be isotopic ratio in a 1400 L sample of molten Antarctic snow by AMS (Accelerator Mass Spectrometry).
View Article and Find Full Text PDFThe concentration of plutonium (Pu) and the isotopic ratios of Pu to Pu and Pu to Pu were determined by accelerator mass spectrometry (AMS) in Pacific Ocean water samples (20 L each) collected in late 2012. The isotopic Pu ratios are important indicators of different contamination sources and were used to identify a possible release of Pu into the ocean by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. In particular, Pu is a well-suited indicator for a recent entry of Pu because Pu from fallout of nuclear weapon testings has already significantly decayed.
View Article and Find Full Text PDFMassive stars ([Formula: see text]), which terminate their evolution as core-collapse supernovae, are theoretically predicted to eject [Formula: see text] of the radioisotope (60)Fe (half-life 2.61 Ma). If such an event occurs sufficiently close to our solar system, traces of the supernova debris could be deposited on Earth.
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