Publications by authors named "Thomas A Clair"

Unlabelled: The ambient ion monitor-ion chromatography (AIM-IC) system, which provides hourly measurements of the main chemical components of PM2.5 (particulate matter with an aerodynamic diameter<2.5 μm) and its precursor gases, was evaluated and deployed from May to July 2011 and April to December 2013 in the Athabasca Oil Sands Region (AOSR) of northeastern Alberta, Canada.

View Article and Find Full Text PDF

The physical factors controlling total mercury (HgT) and methylmercury (MeHg) concentrations in lakes and streams of northeastern USA were assessed in a regional data set containing 693 HgT and 385 corresponding MeHg concentrations in surface waters. Multiple regression models using watershed characteristics and climatic variables explained 38% or less of the variance in HgT and MeHg. Land cover percentages and soil permeability generally provided modest predictive power.

View Article and Find Full Text PDF

We assembled 831 data points for total mercury (Hg(t)) and 277 overlapping points for methyl mercury (CH3Hg+) in surface waters from Massachussetts, USA to the Island of Newfoundland, Canada from State, Provincial, and Federal government databases. These geographically indexed values were used to determine: (a) if large-scale spatial distribution patterns existed and (b) whether there were significant relationships between the two main forms of aquatic Hg as well as with total organic carbon (TOC), a well know complexer of metals. We analyzed the catchments where samples were collected using a Geographical Information System (GIS) approach, calculating catchment sizes, mean slope, and mean wetness index.

View Article and Find Full Text PDF

We report on an inventory and analysis of sediment mercury (Hg) concentrations from 579 sites across northeastern North America. Sediment Hg concentrations ranged from the limit of detection ca. 0.

View Article and Find Full Text PDF

A large number of datasets representing mercury (Hg) levels in northeastern North America were assembled in a standardized format between 2000 and 2003. Based on support from the Northeastern States Research Cooperative, scientists annually gathered and developed an operational template to collaboratively analyze and interpret these data for a series of peer-reviewed publications. The diverse group covered Hg policy connections, Hg in air, sediment and surface water, Hg in biota, and Hg collection, assessment and monitoring tools.

View Article and Find Full Text PDF

Reductions in North American sulfur dioxide (SO2) emissions promoted expectations that aquatic ecosystems in southeastern Canada would soon recover from acidification. Only lakes located near smelters that have dramatically reduced emissions approach this expectation. Lakes in the Atlantic provinces, Quebec and Ontario affected only by long-range sources show a general decline in sulfate (SO4(2-)) concentrations, but with a relatively smaller compensating increase in pH or alkalinity.

View Article and Find Full Text PDF