Development of a Novel Passive Monitoring Technique to Showcase the 3D Distribution of Tritiated Water (HTO) Vapor in Indoor Air of a Nuclear Facility.

Tritiated water (HTO), a ubiquitous byproduct of the nuclear industry, is a radioactive contaminant of major concern for environmental authorities. Although understanding spatiotemporal heterogeneity of airborne HTO vapor holds great importance for radiological safety as well as diagnosing a reactor's status, comprehensive HTO distribution dynamics inside nuclear facilities has not been studied routinely yet due to a lack of appropriate monitoring techniques. For current systems, it is difficult to simultaneously achieve high representativeness, sensitivity, and spatial resolution.

Disproportionately High Contributions of 60 Year Old Weapons-Cs Explain the Persistence of Radioactive Contamination in Bavarian Wild Boars.

Radionuclides released from nuclear accidents or explosions pose long-term threats to ecosystem health. A prominent example is wild boar contamination in central Europe, which is notorious for its persistently high Cs levels. However, without reliable source identification, the origin of this decades old problem has been uncertain.

Uptake of Radionuclides by Bryophytes in the Chornobyl Exclusion Zone.

The "Chernobyl nuclear disaster" released huge amounts of radionuclides, which are still detectable in plants and sediments today. Bryophytes (mosses) are primitive land plants lacking roots and protective cuticles and therefore readily accumulate multiple contaminants, including metals and radionuclides. This study quantifies Cs and Am in moss samples from the cooling pond of the power plant, the surrounding woodland and the city of Prypiat.

Development and calibration of a modifiable passive sampler for monitoring atmospheric tritiated water vapor in different environments.

Anthropogenic release of tritium from nuclear facilities is expected to increase significantly in the coming decades, which may cause radiation exposure to humans through the contamination of water and food chains. It is necessary and urgent to acquire detailed information about tritium in various environments for studying its behavior and assessing the potential radiation risk. In the atmosphere, although the passive sampling technique provides a low-cost and convenient way to characterize the dynamics of tritiated water vapor (HTO), a single, simple sampler configuration makes it difficult to collect sufficient and representative samples within the expected period from different environments.

What's better for our health? Conducting protective actions during a nuclear emergency or accepting a certain radiation dose?

The threat caused by ionising radiation has resulted in the establishment of strict radiation protection guidelines. This is especially true for severe nuclear power plant (NPP) accident scenarios, which may involve the release of significant amounts of ionising radiation. However, we believe that the fine balance between the benefit of a certain protective action (e.

Europe-Wide Atmospheric Radionuclide Dispersion by Unprecedented Wildfires in the Chernobyl Exclusion Zone, April 2020.

From early April 2020, wildfires raged in the highly contaminated areas around the Chernobyl nuclear power plant (CNPP), Ukraine. For about 4 weeks, the fires spread around and into the Chernobyl exclusion zone (CEZ) and came within a few kilometers of both the CNPP and radioactive waste storage facilities. Wildfires occurred on several occasions throughout the month of April.

Determination of Characteristic vs Anomalous Cs/Cs Isotopic Ratios in Radioactively Contaminated Environmental Samples.

A contamination with the ubiquitous radioactive fission product Cs cannot be assigned to its source. We used environmental samples with varying contamination levels from various parts of the world to establish their characteristic Cs/Cs isotope ratios and thereby allow their distinction. The samples included biological materials from Chernobyl and Fukushima, historic ashed human lung tissue from the 1960s from Austria, and trinitite from the Trinity Test Site, USA.

Survival of the basidiomycete Schizophyllum commune in soil under hostile environmental conditions in the Chernobyl Exclusion Zone.

Radioactive contamination resulting from major nuclear accidents presents harsh environmental conditions. Inside the Chernobyl exclusion zone, even more than 30 years after the accident, the resulting contamination levels still does not allow land-use or human dwellings. To study the potential of basidiomycete fungi to survive the conditions, a field trial was set up 5 km south-south-west of the destroyed reactor unit.

Radioactive Games? Radiation Hazard Assessment of the Tokyo Olympic Summer Games.

We conducted a comprehensive radiation hazard assessment of the Tokyo Olympic Games (Tokyo 2020, postponed to 2021). Our combined experimental and literature study focused on both external and internal exposure to ionizing radiation for athletes and visitors of the Games. The effective dose for a visit of 2 weeks ranges from 57 to 310 μSv (including flight dose).

Identification of a chemical fingerprint linking the undeclared 2017 release of Ru to advanced nuclear fuel reprocessing.

The undeclared release and subsequent detection of ruthenium-106 (Ru) across Europe from late September to early October of 2017 prompted an international effort to ascertain the circumstances of the event. While dispersion modeling, corroborated by ground deposition measurements, has narrowed possible locations of origin, there has been a lack of direct empirical evidence to address the nature of the release. This is due to the absence of radiological and chemical signatures in the sample matrices, considering that such signatures encode the history and circumstances of the radioactive contaminant.

Non-natural ruthenium isotope ratios of the undeclared 2017 atmospheric release consistent with civilian nuclear activities.

Understanding the circumstances of the undeclared 2017 nuclear release of ruthenium that led to widespread detections of the radioisotope Ru in the Eurasian region, and whether it derives from a civilian or military source, is of major importance for society and future improvements in nuclear safety. Until now, the released nuclear material has merely been studied by analyzing short-lived radioisotopes. Here, we report precise measurements of the stable isotopic composition of ruthenium captured in air filters before, during, and after the nuclear release, and find that the ruthenium collected during the period of the 2017 nuclear release has a non-natural isotopic composition.

Separation of Ultratraces of Radiosilver from Radiocesium for Environmental Nuclear Forensics.

The presence of environmental radiosilver and the investigation of the Ag/Ag isotopic ratio in the aftermath of a nuclear power plant accident provide valuable information on the condition of the control rods of pressurized water reactors. However, the detection of minute amounts of the γ-emitting radiosilver isotopes is often thwarted by the presence of concomitant and dominating γ emitters, primarily Cs, which results in increased detection limits in the γ spectra. We developed a rapid and robust separation protocol for trace silver extraction in the presence of overwhelming activities of Cs via the autodepostion of silver on a copper plate.

Halide ion influence on the formation of nickel nanoparticles and their conversion into hollow nickel phosphide and sulphide nanocrystals.

A dependence of the formation of tri-n-octylphosphine-capped Ni nanocrystals on the presence of halide ions during their synthesis is shown. For the application-oriented synthesis of Ni particles, this information can be crucial. Furthermore, Ni nanoparticles can be converted to nickel phosphide or sulphide by heating them up in the presence of a phosphorus or sulphur source, resulting in either solid or hollow nanocrystals, formed via the nanoscale Kirkendall effect, depending on the synthesis route.

Airborne concentrations and chemical considerations of radioactive ruthenium from an undeclared major nuclear release in 2017.

In October 2017, most European countries reported unique atmospheric detections of aerosol-bound radioruthenium (Ru). The range of concentrations varied from some tenths of µBq·m to more than 150 mBq·m The widespread detection at such considerable (yet innocuous) levels suggested a considerable release. To compare activity reports of airborne Ru with different sampling periods, concentrations were reconstructed based on the most probable plume presence duration at each location.

Radionuclides in surface waters around the damaged Fukushima Daiichi NPP one month after the accident: Evidence of significant tritium release into the environment.

Following the Fukushima nuclear accident (2011), radionuclides mostly of volatile elements (e.g., I, Cs, Te) have been investigated frequently for their presence in the atmosphere, pedosphere, biosphere, and the Pacific Ocean.

Chemical and radioanalytical investigations of Ru-containing air filters from Vienna in fall 2017: searching for stable element anomalies.

Related to the recent nuclear release of radioactive ruthenium isotopes in fall 2017, we analyzed air filters from Vienna for irregularities in the (stable) elemental composition of particulate matter from this period. Methods were SEM/EDXS and INAA. For comparison, a reference filter from 2007 and blank filters were used.

Radiostrontium transport in plants and phytoremediation.

Radiostrontium is a common product of nuclear fission and was emitted into the environment in the course of nuclear weapon tests as well as from nuclear reactor accidents. The release of Sr and Sr into the environment can pose health threats due to their characteristics such as high specific activities and easy access in human body due to its chemical analogy to calcium. Radiostrontium enters the human food chain by the consumption of plants grown on sites comprising fission-derived radionuclides.

Potential Source Apportionment and Meteorological Conditions Involved in Airborne I Detections in January/February 2017 in Europe.

Traces of particulate radioactive iodine (I) were detected in the European atmosphere in January/February 2017. Concentrations of this nuclear fission product were very low, ranging 0.1 to 10 μBq m except at one location in western Russia where they reached up to several mBq m.

Characteristics of radiocesium contaminations in mushrooms after the Fukushima nuclear accident: evaluation of the food monitoring data from March 2011 to March 2016.

The monitoring inspection of food after the Fukushima nuclear accident (2011) was essential for ensuring food safety in Japan and reducing the adverse health effects due to incorporation of inacceptable amounts of radionuclides, in particular radiocesium (Cs and Cs). In this study, the mushroom fraction of the governmental data set of the first 5 years after the accident has been analyzed for contamination levels in mushrooms, in particular time trends and radioecological characteristics as well as associated health risks. The analyses show that mycorrhiza mushrooms are much more sensitive for radionuclide uptake than saprobiontic mushrooms (the latter of which include the very popular shiitake mushrooms (Lentinula edodes)).

Japanese Food Data Challenge the Claimed Link between Fukushima's Releases and Recently Observed Thyroid Cancer Increase in Japan.

Internal, high-dose exposure with radioiodine is known to increase the risk for thyroid cancer in children and adolescents. Ingestion of contaminated food is generally regarded a dominant route of internal exposure. We analyzed the huge data set of the post-Fukushima food monitoring campaign and deployed a conservative model for the estimation of the doses to the general public in a worst-case scenario.

Fat tissue is not a reservoir for radiocesium in wild boars.

Meat of wild boars is not only known for high Cs activity concentrations but also for the remarkable constancy of these levels. Even decades after the Chernobyl accident, the Cs levels in wild boar meat in Central Europe have not declined but even partly increased. In the present study, we investigated an unusual hypothesis for this very unusual phenomenon: may the boars' fat tissue act as a reservoir for radiocesium? We investigated fat and muscle tissues of four wild boars in Western Germany and found that the Cs concentrations in fat were in the range of 10-30% of the respective activities in muscle tissue.

Mushrooms: from nutrition to mycoremediation.

Mushrooms are well known as important food items. The uses of mushrooms in the cuisine are manifolds and are being utilized for thousands of years in both Oriental and Occidental cultures. Medicinal properties of mushrooms show an immense potential as drugs for the treatment of various diseases as they are rich in a great variety of phytochemicals.

Picomolar Traces of Americium(III) Introduce Drastic Changes in the Structural Chemistry of Terbium(III): A Break in the "Gadolinium Break".

The crystallization of terbium 5,5'-azobis[1H-tetrazol-1-ide] (ZT) in the presence of trace amounts (ca. 50 Bq, ca. 1.

Monitoring and radioecological characteristics of radiocesium in Japanese beef after the Fukushima nuclear accident.

After the Fukushima nuclear accident, beef proved to be a problematic food item with several exceedances entering the market. The reason was contaminated rice straw that was fed to cattle. Japanese authorities responded quickly to the exceedances and made beef one of the most-monitored food items after the Fukushima accident with more than a million samples within 5 years.