Semimetal electrodes for 2D semiconductors have been extensively studied; however, research on p-type semimetals has been limited due to the scarcity of materials that satisfy both high work functions and low resistances. In response, we investigated the behavior of NiSe as an electrode. Utilizing a novel co-evaporation method that suppresses oxidation and contamination, we synthesized NiSe demonstrating a high work function of 5.
View Article and Find Full Text PDFThe relentless miniaturization inherent in complementary metal-oxide semiconductor technology has created challenges at the interface of two-dimensional (2D) materials and metal electrodes. These challenges, predominantly stemming from metal-induced gap states (MIGS) and Schottky barrier heights (SBHs), critically impede device performance. This work introduces an innovative implementation of damage-free SbTe topological van der Waals (T-vdW) contacts, representing an ultimate contact electrode for 2D materials.
View Article and Find Full Text PDFCrystallographic characteristics, including grain boundaries and crystallographic orientation of each grain, are crucial in defining the properties of two-dimensional materials (2DMs). To date, local microstructure analysis of 2DMs, which requires destructive and complex processes, is primarily used to identify unknown 2DM specimens, hindering the subsequent use of characterized samples. Here, a nondestructive large-area 2D crystallographic analytical method through sticky-note-like van der Waals (vdW) assembling-disassembling is presented.
View Article and Find Full Text PDFSemi-infinite single-atom-thick graphene is an ideal reinforcing material that can simultaneously improve the mechanical, electrical, and thermal properties of matrix. Here, we present a float-stacking strategy to accurately align the monolayer graphene reinforcement in polymer matrix. We float graphene-poly(methylmethacrylate) (PMMA) membrane (GPM) at the water-air interface, and wind-up layer-by-layer by roller.
View Article and Find Full Text PDFTailoring the electrical properties of one-dimensional (1D) van der Waals (vdW) materials is desirable for their applications toward electronic devices by exploiting their unique characteristics. However, 1D vdW materials have not been extensively investigated for modulation of their electrical properties. Here we control doping levels and types of 1D vdW NbPdSe over a wide energy range by immersion in AuCl or β-nicotinamide adenine dinucleotide (NADH) solutions, respectively.
View Article and Find Full Text PDFSelf-powered detectors based on triboelectric nanogenerators (TENG) have been considered because of their capability to convert ambient mechanical energy to electrical out-put signal, instead of conventional usage of electrochemical batteries as power sources. In this regard, the self-powered photodetectors have been designed through totally two lay out called passive and active circuit. in former model, impedance matching between the TENG and the resistance of the circuit's elements is crucial, which is not investigated systematically till now.
View Article and Find Full Text PDFHigh-performance photodetectors play crucial roles as an essential tool in many fields of science and technology, such as photonics, imaging, spectroscopy, and data communications. Demands for desired efficiency and low-cost new photodetectors through facile manufacturing methods have become a long-standing challenge. We used a simple successive ionic layer adsorption and reaction (SILAR) method to synthesize CdS, CdSe, and PbS nanoparticles directly grown on WSe crystalline flakes.
View Article and Find Full Text PDFEnhancing the photoresponse of single-layered semiconductor materials is a challenge for high-performance photodetectors due to atomically thickness and limited quantum efficiency of these devices. Band engineering in heterostructure of transition metal chalcogenides (TMDs) can sort out part of this challenge. Here, we address this issue by utilizing the plasmonics phenomenon to enrich the optoelectronics property of the WSe/MoSheterojunction and further enhancement of photoresponse.
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