We report on a comprehensive experimental investigation into the spatial-spectral complexity of the laser beam during Kerr-induced beam self-cleaning in graded-index multimode fibers. We demonstrate the self-cleaning of beams using both transform-limited and chirped femtosecond pulses. By utilizing the spectrally resolved imaging technique, we examine variations in beam homogeneity during the beam cleanup process and reveal correlations observed among spatial beam profiles at different wavelengths for the various cleaned pulses.
View Article and Find Full Text PDFWe demonstrate experimentally high-speed ptychographic imaging of non-repetitive complex-valued events. Three time-resolved complex-valued frames are reconstructed from data recorded in a single camera snapshot. The temporal resolution of the microscope is determined by delays between illuminating pulses.
View Article and Find Full Text PDFTwo-photon excited fluorescence microscopy is a widely-employed imaging technique that enables the noninvasive study of biological specimens in three dimensions with sub-micrometer resolution. Here, we report an assessment of a gain-managed nonlinear (GMN) fiber amplifier for multiphoton microscopy. This recently-developed source delivers 58-nJ and 33-fs pulses at 31-MHz repetition rate.
View Article and Find Full Text PDFMamyshev oscillators produce high-performance pulses, but technical and practical issues render them unsuitable for widespread use. Here we present a Mamyshev oscillator with several key design features that enable self-starting operation and unprecedented performance and simplicity from an all-fiber laser. The laser generates 110 nJ pulses that compress to 40 fs and 80 nJ with a grating pair.
View Article and Find Full Text PDFWe demonstrate an optical parametric chirped-pulse amplifier (OPCPA) that uses birefringence phase matching in a step-index single-mode optical fiber. The OPCPA is pumped with chirped pulses that can be compressed to sub-30-fs duration. The signal (idler) pulses are generated at 905 nm (1270 nm), have 26 nJ (20 nJ) pulse energy, and are compressible to 70 fs duration.
View Article and Find Full Text PDFWe report a study of soliton self-frequency shifting in a hydrogen-filled hollow-core fiber. The combination of hydrogen and short 40-fs input pulses underlies clean and efficient generation of Raman solitons between 1080 and 1600 nm. With 240-nJ input pulses, the Raman soliton energy ranges from 110 to 20 nJ over that wavelength range, and the pulse duration is approximately 45 fs.
View Article and Find Full Text PDFWe present a spatiotemporally mode-locked Mamyshev oscillator. A wide variety of multimode mode-locked states, with varying degrees of spatiotemporal coupling, are observed. We find that some control of the modal content of the output beam is possible through the cavity design.
View Article and Find Full Text PDFMamyshev oscillators can generate high-power femtosecond pulses, but starting a mode-locked state has remained a major challenge due to the suppression of continuous-wave lasing. Here, we study the starting dynamics of a linear Mamyshev oscillator designed to generate high-power femtosecond pulses while avoiding component damage. Reliable starting to stable mode-locking is achieved with a combination of modulation of the pump power and shifting of a filter passband.
View Article and Find Full Text PDFTwo-photon fluorescence microscopy is a nonlinear imaging modality frequently used in deep-tissue imaging applications. A tunable-wavelength multicolor short-pulse source is usually required to excite fluorophores with a wide range of excitation wavelengths. This need is most typically met by solid-state lasers, which are bulky, expensive, and complicated systems.
View Article and Find Full Text PDFActa Crystallogr D Struct Biol
May 2021
Serial synchrotron crystallography (SSX) is enabling the efficient use of small crystals for structure-function studies of biomolecules and for drug discovery. An integrated SSX system has been developed comprising ultralow background-scatter sample holders suitable for room and cryogenic temperature crystallographic data collection, a sample-loading station and a humid `gloveless' glovebox. The sample holders incorporate thin-film supports with a variety of designs optimized for different crystal-loading challenges.
View Article and Find Full Text PDFWe demonstrate numerically and experimentally a gain-managed nonlinear amplifier with a large mode area fiber. The amplifier delivers 1.2 µJ and sub-40 fs pulses with the spectrum spanning from ∼1000 to ∼1180.
View Article and Find Full Text PDFUltrafast lasers are becoming increasingly widespread in science and industry alike. Fiber-based ultrafast laser sources are especially attractive because of their compactness, alignment-free setups, and potentially low cost. However, confining short pulses within a fiber core leads to high intensities, which drives a host of nonlinear effects.
View Article and Find Full Text PDFWe propose a simple all-in-line single-shot scheme for diagnostics of ultrashort laser pulses, consisting of a multi-mode fiber, a nonlinear crystal and a camera. The system records a 2D spatial intensity pattern, from which the pulse shape (amplitude and phase) are recovered, through a fast Deep Learning algorithm. We explore this scheme in simulations and demonstrate the recovery of ultrashort pulses, robustness to noise in measurements and to inaccuracies in the parameters of the system components.
View Article and Find Full Text PDFWe propose and demonstrate, numerically and experimentally, use of sparsity as prior information for extending the capabilities and performance of techniques and devices for laser pulse diagnostics. We apply the concept of sparsity in three different applications. First, we improve a photodiode-oscilloscope system's resolution for measuring the intensity structure of laser pulses.
View Article and Find Full Text PDFWe investigated the possibility of reaching nanojoule-level pulse energies in a femtosecond erbium-doped fiber Mamyshev oscillator. In experiments, lasers generate stable pulse trains with energy up to 31.3 nJ, which is comparable to the highest achieved by prior ultrafast erbium fiber lasers.
View Article and Find Full Text PDFWe demonstrate experimentally multiplexed single-shot ptychography. Specifically, we present a polarization-resolved single-shot ptychographic microscope, where the orthogonally polarized amplitudes and phases of a polarization-sensitive object are reconstructed from ptychographic data recorded in a single camera exposure. Moreover, the amplitudes, phases, and polarization states of the probe beams are also recovered.
View Article and Find Full Text PDFWe demonstrate a fiber oscillator that achieves 3 MW peak power, is easily started, and is environmentally stable. The Mamyshev oscillator delivers 190-nJ pulses that can be compressed externally to 35 fs duration. Accurate numerical modeling of the gain medium provides insight into the behavior and performance of the device.
View Article and Find Full Text PDFUltrafast fiber lasers have the potential to make applications of ultrashort pulses widespread - techniques not only for scientists, but also for doctors, manufacturing engineers, and more. Today, this potential is only realized in refractive surgery and some femtosecond micromachining. The existing market for ultrafast lasers remains dominated by solid-state lasers, primarily Ti:sapphire, due to their superior performance.
View Article and Find Full Text PDFWe propose and demonstrate numerically a simple method for ultrahigh-speed imaging of complex (amplitude and phase) samples. Our method exploits redundancy in single-shot ptychography (SSP) for reconstruction of multiple frames from a single camera snapshot. We term the method Time-resolved Imaging by Multiplexed Ptychography (TIMP).
View Article and Find Full Text PDFPhase-retrieval problems of one-dimensional (1D) signals are known to suffer from ambiguity that hampers their recovery from measurements of their Fourier magnitude, even when their support (a region that confines the signal) is known. Here we demonstrate sparsity-based coherent diffraction imaging of 1D objects using extreme-ultraviolet radiation produced from high harmonic generation. Using sparsity as prior information removes the ambiguity in many cases and enhances the resolution beyond the physical limit of the microscope.
View Article and Find Full Text PDFWe propose and numerically demonstrate a method for obtaining high-harmonic radiation with desirable elliptical polarization. Atoms are shined by a combination of a strong linearly-polarized laser field and an additional weak field, which is elliptically polarized in a plane perpendicular to the polarization direction of the strong field. The strong driver ionizes and recollides electrons with their parent ion, while the weak field perturbatively drives the electrons away from "head-on" collision.
View Article and Find Full Text PDFWe demonstrate self-phase modulation (SPM) spectral broadening in two-dimensional solitons in homogeneous media using two different schemes. In the active mode, a train of pulses are collectively trapped and form a spatial soliton through a photorefractive, slowly responding, and electronically controlled self-focusing nonlinearity, and each pulse experiences spectral broadening by the fast SPM nonlinearity. In the passive mode, the pulse-train beam is guided in a waveguide that is optically induced by a continuous-wave thermal spatial soliton.
View Article and Find Full Text PDFCoherent Diffractive Imaging (CDI) is an algorithmic imaging technique where intricate features are reconstructed from measurements of the freely diffracting intensity pattern. An important goal of such lensless imaging methods is to study the structure of molecules that cannot be crystallized. Ideally, one would want to perform CDI at the highest achievable spatial resolution and in a single-shot measurement such that it could be applied to imaging of ultrafast events.
View Article and Find Full Text PDFWe show that a sawtooth phase-modulation is the optimal profile for grating assisted phase matching (GAPM). Perfect (sharp) sawtooth modulation fully corrects the phase-mismatch, exhibiting conversion equal to conventional phase matching, while smoothened, approximate sawtooth structures are more efficient than sinusoidal or square GAPM modulations that were previously studied. As an example, we demonstrate numerically optically-induced sawtooth GAPM for high harmonic generation.
View Article and Find Full Text PDFWe show how bright, tabletop, fully coherent hard X-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By driving the high-order harmonic generation process using longer-wavelength midinfrared light, we show that, in theory, fully phase-matched frequency upconversion can extend into the hard X-ray region of the spectrum. We verify our scaling predictions experimentally by demonstrating phase matching in the soft X-ray region of the spectrum around 330 eV, using ultrafast driving laser pulses at 1.
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