Probing the Magnetic Ground State of BaYIrO: Impact of Nonmagnetic Dopants and Spin-Orbit Coupling.

Strong spin-orbit coupling (SOC) in iridates has long been predicted to lead to exotic electronic and magnetic ground states. Ba2YIrO6 (BYIO) has attracted particular attention due to the expectation of a Jeff = 0 state for Ir5+ ions under the jj-coupling scheme. However, controversies surround the actual realization of this state, as finite magnetic moments are consistently observed experimentally.