The oriented conversion of CO into target high-value chemicals is an effective way to reduce carbon emissions, but still presents a challenge. In this communication, we report the oriented conversion of CO into value-added aromatics, especially para-xylene, in a single pass by combining core-shell structured Zn-doped H-ZSM-5 (Zn-ZSM-5@SiO ) and a Cr O component. Through precise regulation of the acidity of Zn-ZSM-5@SiO , high para-xylene selectivity (38.
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