Oxygen-vacancy (Ov) engineering is an effective strategy to manipulate the electronic configuration of catalysts for electrochemical nitrogen reduction reaction (eNRR). The influence of the stable facet on the electronic configuration of Ov is widely studied, however, the effect of the reactive facet on the local electron density of Ov is unveiled. In this work, an eNRR electrode R(111)-TiO/HGO is provided with a high proportion exposed reactive facet (111) of rutile-TiO (denoted as R(111)-TiO) nanocrystals with Ov anchored in hierarchically porous graphite oxide (HGO) nanofilms.
View Article and Find Full Text PDFA fluorescent immunochromatographic test (FM-ICT) was developed for rapid detection of anti-Orientia tsutsugamushi antibodies in serum samples. The FM-ICT was constructed based on the dual-antigen sandwich method. Truncated 56 kDa outer membrane protein of O.
View Article and Find Full Text PDFElectrocatalytic ethylene (CH) evolution from CO reduction is an intriguing route to mitigate both the energy and environmental crises; however, to acquire industrially relevant high productivity and selectivity at low energy cost remains to be challenging. Membrane assembly electrode has shown great prospect and tailoring its architecture for maximizing CH yield at minimum voltage with long-term stability becomes critical. Here a freestanding Cu membrane cathode is designed and constructed by electrochemically depositing mesoporous Cu film on Cu foam to simultaneously manage CO, electron, water, and product transport, which shows an extraordinary CH Faradaic efficiency of 85.
View Article and Find Full Text PDFChem Commun (Camb)
February 2024
The electrocatalytic nitrogen reduction reaction (eNRR) under ambient conditions is deemed a promising alternative for NH synthesis. In this paper, an FeP-FeO nanocomposite electrocatalyst was prepared by phosphating annealing using FeO as a precursor, and the resulting FeP-FeO exhibited excellent N-to-NH-producing activity over a wide potential window. The highest faradaic efficiency of FeP-FeO is 11.
View Article and Find Full Text PDFExtracting muscle synergies from surface electromyographic signals (sEMGs) during exercises has been widely applied to evaluate motor control strategies. This study explores the relationship between upper-limb muscle synergies and the performance of joystick manipulation tasks. Seventy-seven subjects, divided into three classes according to their maneuvering experience, were recruited to perform the left and right reciprocation of the joystick.
View Article and Find Full Text PDFIEEE Trans Ultrason Ferroelectr Freq Control
February 2022
Droplet injection methods are widely used in the applications of microelectronic manufacturing, biological engineering, and 3-D printing. This work presents a new jet dispenser driven by a single piezoelectric stack that enables the capability of drop-on-demand patterning under a high working frequency (500 Hz). Due to the special designs of the jet dispenser, a broad range of liquids, whose viscosities span more than four orders of magnitude (21-665 320 cps), can be jetted.
View Article and Find Full Text PDFElectrocatalytic synthesis of multicarbon (C) products from CO reduction suffers from poor selectivity and low energy efficiency. Herein, a facile oxidation-reduction cycling method is adopted to reconstruct the Cu electrode surface with the help of halide anions. The surface composed of entangled Cu nanowires with hierarchical pores is synthesized in the presence of I, exhibiting a C faradaic efficiency (FE) of 80% at -1.
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