Although microstructure optimization is an effective strategy to improve and regulate electromagnetic wave (EMW) absorption properties, preparing microwave absorbents with enhanced EMW absorbing performance and tuned absorption band by a simple method remains challenging. Herein, ZnInS/reduced graphene oxide (rGO) composites with flower-like and cloud-like morphologies were fabricated by a convenient hydrothermal method. The ZnInS/rGO composites with different morphologies realize efficient EMW absorption and tunable absorption bands, covering a wide frequency range.
View Article and Find Full Text PDFAll-weather personal thermal regulation has far been challenged by variable environments especially the regulatory failure caused by highly-dense solar radiation, low environmental radiation and the fluctuated epidermal moisture in different seasons. Herein, from the design of interface selectivity, dual-asymmetrically optical and wetting selective polylactic acid-based (PLA) Janus-type nanofabric is proposed to achieve on-demand radiative cooling and heating as well as sweat transportation. Hollow TiO particles are introduced in PLA nanofabric causing high interface scattering (∼99%) and infrared emission (∼91.
View Article and Find Full Text PDFIn the practical application of microwave absorbing materials, traditional powder materials need to be mixed with the matrix to fabricate composite coatings. However, the complex preparation process of composite coatings and the uneven dispersion of powders in the matrix limit their application. To solve these problems, two-dimensional (2D) F-WS/CP composite films were prepared by using carbon paper (CP) as a dispersion matrix and loading flower-like WS on its surface through a simple hydrothermal method.
View Article and Find Full Text PDFAlthough intensive efforts have been devoted to fabricating TiCT MXene composites for microwave absorption, it remains a great challenge to achieve excellent MA performance at low loading and thin thickness. Herein, a three-dimensional (3D) lightweight hierarchically structured MnO/TiCT/RGO composite aerogel with abundant heterointerfaces was fabricated via a hydrothermal and chemical reduction self-assembly method. The RGO aerogel embedded with laminated MnO/TiCT provides a lot of heterogeneous interfaces, 3D porous interconnected conductive networks, and reasonable combination of various loss materials for rich interfacial polarization, conductivity loss, multiple reflections and scattering, and good impedance matching.
View Article and Find Full Text PDFCarbon fiber aerogel (CFA) derived from cotton wool as a potential microwave absorbing material has received intensive attention owing to the low density, high conductivity, large surface area, and low cost, but its applications are limited by the relatively high complex permittivity. To solve this problem, TiO@C (derived from TiCT) is introduced into CFA to prepare lightweight TiO@C/CFA composites based on electromagnetic (EM) parameter optimization and enhanced EM wave attenuation performance. The microwave absorption capacity of TiO@C/CFA-2 composite is obviously better than that of CFA.
View Article and Find Full Text PDFHydrogel-based wearable sensors have experienced an explosive development, whereas functional integration to mimic the multisignal responsiveness of skin especially for pressure and temperature remained a challenge. Herein, a functional ionic hydrogel-base flexible sensor was successfully prepared by integrating the thermal-sensitive N-isopropylacrylamide (NIPAAm) into another conductive double-network hydrogel based on polyvinyl alcohol-graphene oxide (PVA-GO) and polyacrylic acid-Fe (PAA-Fe). Because of the multisynergistic network design, the triple-network hydrogel was endowed with excellent conductivity (∼170 Ω/mm), mechanical tolerance (1.
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