Enhanced Performance of a Self-Powered Au/WSe/TaNiS/Au Heterojunction by the Interfacial Pyro-phototronic Effect.

The growing need for wearable electronics and self-powered electronic devices has driven the successful development of self-powered two-dimensional (2D) photodetectors using the photovoltaic effect of Schottky and p-n junctions. However, there is an urgent need to develop multifunctional photodetectors capable of harvesting energy from different sources to overcome their limitations in efficiency and cost. While the pyro-phototronic effect has been shown to effectively influence optoelectronic processes in heterojunctions, the number of reported two-dimensional heterojunctions exhibiting interfacial pyroelectricity is still limited, and the responsivity and detectivity based on such heterojunctions tend to be low.