In a recent field campaign focused on air quality study, aerosol optical properties, particle number concentration, and PM components were monitored in Changzhou, Jiangsu Province, from May 27 to June 27, 2019. An array of instruments were deployed that included scanning mobility particle size spectrometer (SMPS), aethalometer (AE33), cavity attenuation phase shift single albedo monitor (CAPS-ALB), monitor for aerosols and gases in ambient air (MARGA) and RT-4 organic carbon/elemental carbon (OC/EC) carbon analyzer to study the ① changes in chemical composition and optical parameters of the new particles generated during the campaign period. ② comparison of the aerosol extinction coefficient recorded by these instruments and measured value in the reconstruction of IMPROVE (interagency monitoring of protected visual environment) and the calculated coefficient using MIE theory model were carried out.
View Article and Find Full Text PDFDiagnostic indicators for the validation of PM compositional data were calculated, based on the monitoring results of approximately 2100 ambient samples collected in the Yangzi River Delta from 2014 to 2017. According to the results of a correlation analysis, we propose that the audit indexes of the monitoring data of PM components in ambient air should include:equivalent ratios of anion-cation charge balance(), the consistency between sum of all measured components(∑species) and weighed PM, the consistency between mass reconstructed PM(PM) and weighed PM, the chemical consistency between elemental S and water-soluble SO, elemental K and water-soluble K, and the chemical consistency of theoretical and tested NH. The double-sided 95% reference ranges of anion-cation equivalent balance (), ∑species/PM, PM/PM, S/SO, and K/K ratios were determined in terms of and as follows:(0.
View Article and Find Full Text PDFThe study of the sources, compositions, and formation mechanisms of pollutants at the background site is crucial for the understanding of episodic events in the Yangtze River Delta (YRD). Secondary species are major components of PM particles. In this work, the compositions and concentrations of organic matter and secondary organic aerosol (SOA) at a background site of the YRD region were determined.
View Article and Find Full Text PDFParticulate organic matter (POM) has attracted increasing attention recently due to its great contribution to fine particles (PM) and complex components and sources. In the present study, 78 particulate organic compounds in PM were quantified at three sites in Shanghai during summer; these sites were located in urban (Xuhui), suburban (Qingpu), and coastal (Lin'gang) areas of the city. Accordingly, the chemical composition and spatial distribution were investigated and sources were explored based on the indicators and diagnostic ratios combined with backward trajectory.
View Article and Find Full Text PDFCooking is one of important emission sources of fine particles (PM). This study using the catering enterprises of Shanghai as an example, presents a method to estimate the PM emission inventory from cooking according to the number of stoves, cooking time, and number of customers. Based on in situ measurements, the concentrations of PM emissions ranged from 0.
View Article and Find Full Text PDFBased on site investigation of non-road vehicles in Shanghai and Hangzhou located in east China, non-road vehicle emission inventory in 2014 was established in these cities as well as its emission inventory technology. Characteristics of non-road vehicle were also analyzed, including classification, type of fuel, power and emission standard. The results showed that diesel consumed by non-road vehicles was 6.
View Article and Find Full Text PDFThe status of treatment equipment, the emission characteristics, and the ozone formation potential (OFP) of volatile organic compounds (VOCs) for 11 typical enterprises, which were categorized into the 8 major VOC emission industries identified by the emission inventory of a typical city in the Yangtze River Delta, are discussed in this paper. There was a large difference in the removal efficiency of non-methane hydrocarbon (NMHC) between different treatment techniques, and even an increase in concentration occurred after some of the treatments. The current treatment equipment for VOCs needs further optimization.
View Article and Find Full Text PDFVolatile Organic Compounds (VOCs) source profiles of on-road vehicles were widely studied as their critical roles in VOCs source apportionment and abatement measures in megacities. Studies of VOCs source profiles from on-road motor vehicles from 2001 to 2016 were summarized in this study, with a focus on the comparisons among different studies and the potential impact of different factors. Generally, non-methane hydrocarbons dominated the source profile of on-road vehicle emissions.
View Article and Find Full Text PDFIntensive haze shrouded central and eastern parts of China in Dec. 2013. In this study, the mass concentrations of gaseous and particulate pollutants, and also the chemical compositions of fine particulate matters were obtained based on in-situ measurement in Shanghai urban area.
View Article and Find Full Text PDFWith the fast development of urbanization, industrialization and mobilization, the air pollutant emissions with photochemical reactivity become more obvious, causing a severe photochemical pollution with the characteristics of high ozone concentration. However, the ozone source identification is very complicated due to the high non linearity between ozone and its precursors. Thus, ways to reduce ozone is still not clear.
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