Monomethylmercury (MMHg) is a potent neurotoxin that poses a threat to human health. MMHg cycles in all spheres of the Earth but the sources and fate of atmospheric MMHg are unclear. Here, we develop a global model for atmospheric MMHg, which integrates the presently available data and indicates the limitations of the current study.
View Article and Find Full Text PDFThe redox chemistry of mercury (Hg) in the atmosphere exerts a significant influence on its global cycle. However, our understanding of this important process remains shrouded in uncertainty. In this study, we utilize three-dimensional atmospheric Hg isotope modeling to evaluate the isotopic composition of particle-bound mercury [Hg(P)] in the global atmosphere.
View Article and Find Full Text PDFMercury (Hg), a potent neurotoxin posing risks to human health, is cycled through vegetation uptake, which is susceptible to climate change impacts. However, the extent and pattern of these impacts are largely unknown, obstructing predictions of Hg's fate in terrestrial ecosystems. Here, we evaluate the effects of climate change on vegetation elemental Hg [Hg(0)] uptake using a state-of-the-art global terrestrial Hg model (CLM5-Hg) that incorporates plant physiology.
View Article and Find Full Text PDFSea ice (including overlying snow) is a dynamic interface between the atmosphere and the ocean, influencing the mercury (Hg) cycling in polar oceans. However, a large-scale and process-based model for the Hg cycle in the sea ice environment is lacking, hampering our understanding of regional Hg budget and critical processes. Here, we develop a comprehensive model for the Hg cycle at the ocean-sea ice-atmosphere interface with constraints from observational polar cryospheric data.
View Article and Find Full Text PDFRiverine processes are crucial for the biogeochemical cycle of mercury (Hg). The Yangtze River, the largest river in East Asia, discharges a substantial amount of Hg into the East China Sea. However, the influencing factors of the Hg budget and its recent trends remain unclear.
View Article and Find Full Text PDFBackground: The effects of postoperative adjuvant therapy for high-risk recurrent hepatocellular carcinoma (HCC) in immunotherapy are still under investigation. This study evaluated the preventive effects and safety of postoperative adjuvant therapy, including atezolizumab, and bevacizumab, against the early recurrence of HCC with high-risk factors.
Methods: The complete data of HCC patients who underwent radical hepatectomy with or without postoperative adjuvant therapy after two-year follow-up were analyzed retrospectively.
The vegetation uptake of atmospheric elemental mercury [Hg(0)] and its subsequent littering are critical processes of the terrestrial Hg cycles. There is a large uncertainty in the estimated global fluxes of these processes due to the knowledge gap in the underlying mechanisms and their relationship with environmental factors. Here, we develop a new global model based on the Community Land Model Version 5 (CLM5-Hg) as an independent component of the Community Earth System Model 2 (CESM2).
View Article and Find Full Text PDFMercury is a potent neurotoxin that poses health risks to the global population. Anthropogenic mercury emissions to the atmosphere are projected to decrease in the future due to enhanced policy efforts such as the Minamata Convention, a legally-binding international treaty entered into force in 2017. Here, we report the development of a comprehensive climate-atmosphere-land-ocean-ecosystem and exposure-risk model framework for mercury and its application to project the health effects of future atmospheric emissions.
View Article and Find Full Text PDFAir-sea exchange of gaseous elemental mercury (Hg(0)) is influenced by different meteorological factors and the availability of Hg in seawater. Here, we use the MITgcm ocean model to explore the interannual variability of this flux and the influence of oceanographic and atmospheric dynamics. We apply the GEOS-Chem model to further simulate the potential impact of the evasion variability on the atmospheric Hg levels.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
January 2019
Atmospheric particulate matter (PM) and ammonia pollution from livestock feeding have gradually become the environmental concerns due to the spring up of livestock farms in worldwide. However, researches about the formation of atmospheric particulate matter related to ammonia are still limited. Therefore, a study to survey the total suspended particles (TSP), PM with the diameter less than 10 μm (PM), PM, PM, PM, and ammonia was conducted at four types of hog houses distinguished by its building design as well as manure handling methods in South China.
View Article and Find Full Text PDFPlant leaves play a key role in the accumulation of PAHs, as they are able to capture PAHs from the air. In this paper, the mechanism, including absorption and adsorption, for plants to scavenge PAHs from the air was reviewed. Moreover, the differences of PAHs accumulating capability are mainly compared among three representative plant species, including pine needles, Holm oak leaves, and moss.
View Article and Find Full Text PDFThis study focused on the heavy metal concentrations in the soil and their representative input and output fluxes to paddy fields in four types of contaminated areas in Changzhutan urban agglomerations, Hunan, China. Four types of contaminated areas (mining area, livestock breeding area, suburb area and control area) were chosen for monitoring. Three input pathways and three output pathways were considered so as to figure out the heavy metal balance throughout the topsoil.
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