Microbial electrosynthesis is a promising technology that recovers energy from wastewater while converting CO into CH. Constructing a biocathode with both strong H-mediated and direct electron transfer capacities is crucial for efficient startup and long-term stable CH production. This study found that introducing carboxyl groups onto the cathode effectively enhanced both electron transfer pathways, improving the reduction rate and coulombic efficiency of CH production and increasing the CH yield by 2-3 times.
View Article and Find Full Text PDFFor the simultaneous energetic utilization of corn stalk and azo-dye contaminated wastewater, an ECMO-like integrated reactor was come up to achieve the biogas production and azo-dye degradation during anaerobic digestion (AD). Methyl orange (MO) was selected as the model compound for azo-dye. The ECMO-like reactor included AD main reactor with a spray device and solid-liquid separation components, integrated with an aeration reactor for biogas slurry.
View Article and Find Full Text PDFMicrobial electrolysis cells (MECs) are increasingly recognized as a promising technology for converting CO to CH, offering the dual benefits of energy recovery from organic wastewater and CO emission reduction. A critical aspect of this technology is the enhancement of the electron-accepting capacity of the methanogenic biocathode to improve CH production efficiency. This study demonstrates that adjusting the cathode resistivity is an effective way to control the electric field intensity, thereby enhancing the electron accepting capacity and CH production.
View Article and Find Full Text PDFBioaugmentation technology for improving the performance of thermophilic anaerobic digestion (TAD) of food waste (FW) treatment is gaining more attention. In this study, four thermophilic strains (Ureibacillus suwonensis E11, Clostridium thermopalmarium HK1, Bacillus thermoamylovorans Y25 and Caldibacillus thermoamylovorans QK5) were inoculated in the TAD of FW system, and the biochemical methane potential (BMP) batch study was conducted to assess the potential of different bioaugmented strains to enhance methane production. The results showed that the cumulative methane production in groups inoculated with E11, HK1, Y25 and QK5 improved by 2.
View Article and Find Full Text PDFNitrogen removal is often limited in municipal wastewater treatment due to the lack of sufficient carbon source. Utilizing volatile fatty acids (VFAs) from waste activated sludge (WAS) fermentation broth as a carbon source is an ideal alternative to reduce the cost for wastewater treatment plants (WWTPs) and improve denitrification efficiency simultaneously. In this study, an anaerobic system was applied for simultaneous denitrification and WAS fermentation and the addition of magnetic microparticles (MMP) were confirmed to enhance both denitrification and WAS fermentation.
View Article and Find Full Text PDFIn this work, a new type, highly sensitive, and reusable nanoplastics (NPs) microwave detection method is proposed, which can be used to rapidly analyze NPs with different surface charges and sizes. The effective dielectric constant of NPs varies according to the different concentrations, particle sizes, and surface charges of NPs in aqueous solution. The feasibility of the microwave method for differential-charged NPs detection is verified using a complementary split ring resonator sensor manufactured on a cost-effective printed circuit board, which shows a high sensitivity only for positively charged NPs (PS-NH) detection.
View Article and Find Full Text PDFStudies on the adverse effects of nanoplastics (NPs, particle diameter <1000 nm) including physical damage, oxidative stress, impaired cell signaling, altered metabolism, developmental defects, and possible genetic damage have intensified in recent years. However, the analytical detection of NPs is still a bottleneck. To overcome this bottleneck and obtain a reliable and quantitative distribution analysis in complex freshwater ecosystems, an easily applicable NP tracer to simulate their fate and behavior is needed.
View Article and Find Full Text PDFThe accumulation of a large amount of organic solid waste and the lack of sufficient protein supply worldwide are two major challenges caused by rapid population growth. Anaerobic digestion is the main force of organic waste treatment, and the high-value utilization of its products (biogas and digestate) has been widely concerned. These products can be used as nutrients and energy sources for microorganisms such as microalgae, yeast, methane-oxidizing bacteria(MOB), and hydrogen-oxidizing bacteria(HOB) to produce single cell protein(SCP), which contributes to the achievement of sustainable development goals.
View Article and Find Full Text PDFAgriculture wastes have been proved to be the potential adsorbents to remove azo dye from textile wastewater, but the post-treatment of azo dye loaded agriculture waste is generally ignored. A three-step strategy including sequential adsorption-biomethanation-composting was developed to realize the co-processing of azo dye and corn straw (CS). Results showed that CS represented a potential adsorbent to remove methyl orange (MO) from textile wastewater, with the maximum MO adsorption capacity of 10.
View Article and Find Full Text PDFThe environmental issues caused by nanoplastics (NPs) are increasingly noticeable. Environmental behavior study of the NPs could provide vital information for their environmental impact assessment. However, associations between NPs' inherent properties and their sedimentation behaviors were seldom investigated.
View Article and Find Full Text PDFHumic acids (HAs) are important byproducts of anaerobic digestion (AD), which have complex structures and dynamic electrochemical activities. However, the effects of HAs on AD process were usually misestimated due to the neglect of the in situ generated HAs and the interaction between HAs and metal ions. This study explored the effects of HAs on AD performance using corn straw as typical "clean" substrate (rare in metals content) via commercial HAs (C-HAs) addition and in-situ-generated HAs (In-HAs) removal.
View Article and Find Full Text PDFMicro-aeration can facilitate anaerobic digestion (AD) by regulating microbial communities and promoting the growth of facultative taxa, thereby increasing methane yield and stabilizing the AD process. Additionally, micro-aeration contributes to hydrogen sulfide stripping by oxidization to produce molecular sulfur or sulfuric acid. Although micro-aeration can positively affect AD, it must be strictly regulated to maintain an overall anaerobic environment that permits anaerobic microorganisms to thrive.
View Article and Find Full Text PDFCyanobacteria salvage is widely used to deal with massive cyanobacterial blooms. Improper disposal of salvaged cyanobacteria would cause secondary pollution. Black soldier fly (Hermetia illucens) larvae (BSFL) can bio-convert organic wastes into larval biomass, which is rich in protein and lipid.
View Article and Find Full Text PDFThe aim of this work was to study the effects of the magnetic microparticles (MMP) on nitrogen removal under low C/N conditions. A 30-day anaerobic/oxic progress illustrated that nitrification and denitrification were promoted in the presence of MMP. MMP could facilitate the production of extracellular polymeric substances (EPS) and act as pH buffering in aerobic conditions.
View Article and Find Full Text PDFBioresour Technol
September 2022
Humic acids (HAs) are abundant on earth, yet their effects on anaerobic digestion (AD) of cellulosic substrate are not fully uncovered. The effects of HAs on AD of corn straw and the mechanisms behind were analyzed in this study. Results showed that the effects of HAs on methane yield were closely related to the total solids (TS) content.
View Article and Find Full Text PDFThe treatment of food waste digestate with high salinity is a big challenge. This paper evaluated the possibility of using black soldier fly larvae for food waste digestate disposal and insect protein production. Results showed that both digestates from hydrogen and methane fermentations were rich in protein and lipid contents, which benefited the BSFL cultivation.
View Article and Find Full Text PDFThe resistant structure and high carbon/nitrogen ratio (C/N) of cellulosic substrate are the barriers during their anaerobic digestion (AD). Solid-state urea pretreatment was developed in this study to pretreat corn straw and adjust C/N ratio simultaneously for the downstream AD of corn straw. Results showed solid-state urea pretreatment was efficient in lignin removal and achieved the highest lignin reduction of 7.
View Article and Find Full Text PDFEnviron Sci Process Impacts
December 2021
Nanoplastics (NPs) have drawn increasing attention in recent years due to their potential threats to aquatic ecosystems. Microalgae are primary producers, which play important roles in the normal functioning of ecosystems. According to the source of production and laboratory experiments, both NPs and microalgae are likely to be widely found in various water environments, so they have a great chance of interacting with each other.
View Article and Find Full Text PDFBiogas produced by anaerobic digestion is an important renewable energy carrier. Nevertheless, the high CO content in biogas limits its utilization to mainly heat and electricity generation. Upgrading biogas into biomethane broadens its potential as a vehicle fuel or substitute for natural gas.
View Article and Find Full Text PDFHigh-solid anaerobic digestion (AD) faces the problems of easy acidification and low methane production efficiency. In this study, activated carbon (AC)-enhanced direct interspecies electron transfer (DIET) was investigated to overcome such problems. Results showed the conversion of volatile fatty acids (VFAs) into methane rate was increased with AC addition, which led improved methane production efficiency.
View Article and Find Full Text PDFGrain stillage from the liquor industry was pretreated by using microwave-assisted hydrothermal pretreatment, fungal pretreatments, and their combination to enable efficient enzymatic hydrolysis for sugar production. The microwave-assisted hydrothermal (MH) pretreatment was optimized by using a response surface methodology, and the respective maximum reducing sugar yield and saccharification efficiency of 17.59 g/100 g and 33.
View Article and Find Full Text PDFIn order to enable rapid disposal and proper preservation of discarded vegetable for waste valorization, ensiling was employed to preserve cauliflower leaves for 30 days at different temperatures (20 ~ 45 °C) with and without the addition of Lactobacillus plantarum L8. The L. plantarum inoculant reduced dry matter (DM) loss and enhanced the preservation of protein and soluble carbohydrate while decreasing pH and ammonia nitrogen content.
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