Publications by authors named "Sergei Preis"

Although prokaryotic microbes in coking wastewater (CWW) treatment have been comprehensively studied, the ecological functions of viruses remain unclear. A full-scale CWW biological treatment AOHO combination was studied for the virus-bacterium interactions involved in element cycles by metaviromics, metagenomics and physicochemical characteristics. Results showed the unique viromic profile with Cirlivirales and Petitvirales as the dominant viruses infecting functional bacteria hosts.

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Article Synopsis
  • The study highlighted how bacterial composition and functions in a treatment system for coking wastewater (CWW) change with the seasons, using advanced sequencing techniques.
  • Core bacterial genera such as Thiobacillus and Pseudomonas were identified, with their relative presence fluctuating across different seasons while effectively removing major contaminants.
  • The findings indicated that dissolved oxygen levels significantly influence microbial community structure, supporting the idea of functional redundancy which allows stable wastewater treatment performance despite seasonal changes.
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Biological treatment is commonly used in coking wastewater (CWW) treatment. Prokaryotic microbial communities in CWW treatment have been comprehensively studied. However, viruses, as the critical microorganisms affecting microbial processes and thus engineering parameters, still remain poorly understood in CWW treatment context.

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In this study, physicochemical pre- and post-treatment of highly polluting coking wastewater (CWW) for the removal of refractory compounds and recovery of high-energy substances/components was investigated. An economic optimization model targeting the development of a cost-effective and sustainable treatment technology was proposed. At the post-treatment stage, powdered activated carbon (PAC) was used to separate the refractory and toxic pollutants from the bio-treated CWW, with the adsorption capacity ranging from 50 to 120 mg chemical oxygen demand (COD) g PAC.

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Taking into account difficulties in exhaustive simultaneous decarbonation and denitrogenation in biological treatment of coking wastewater (CWW), a novel full-scale CWW biological treatment sequentially combining anaerobic, aerobic, hydrolytic, and aerobic reactors (A/O1/H/O2) was designed performing excellent removal of carbon-containing pollutants in the bioreactors A and O1, while the nitrogen-containing compounds in the bioreactors H and O2. To provide an effective tool for the CWW treatment monitoring and control, the succession of microbial community in this unique toxic CWW habitat should be established and characterized in detail. The results of 16S rRNA genes revealed Acidobacteria dominating in the unique CWW habitat.

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Systematically analyzing the problem of heavy metals in the municipal sludge, a meta-analysis of nine metals was undertaken to distinguish the sources and sinks of those with the impact of their accumulation on the environment. Municipal sludge was rich in N, P and K nutrients, was found to contain heavy metals comprising the descending order Zn > Mn > Cu > Cr > Pb > Ni > As > Cd > Hg. The forms, in which heavy metals accumulated in geographical regions, were characterized.

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The application of advanced biological treatment technology results in improved coking wastewater (CW) effluent quality at lower material and energy input practiced by wastewater treatment plants. In wastewater treatment, the diversity of biological processes combinations affects the variety of microorganisms and biochemical reactions resulting in effluent quality. Four full-scale CW processes, anaerobic-anoxic-oxic (A/A/O), anoxic-oxic-hydrolytic-oxic (A/O/H/O), anoxic-oxic-oxic (A/O/O), and oxic-hydrolytic-oxic (O/H/O) were compared for their consumption of chemicals and energy, emissions of greenhouse gases, and excess sludge production.

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The design of biological treatment process for the coking wastewater (CW) is complicated since wastewater treatment demand is gradually increasing lacking the systematic strategy in efficiency evaluation and advisable selection. Therefore, this study develops a holistic approach by means of the analytic hierarchy process (AHP) that uses numerical representation to rank the preferences of each participating alternatives for evaluation of the advanced biological technologies in CW treatment. Based on survey results, six types reactor combinations were selected as the alternatives, which were further classified as two group according to COD load.

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A high-efficiency graphene oxide-terminated hyperbranched amino polymer-carboxymethyl cellulose ternary nanocomposite (GO-HBP-NH-CMC) was fabricated for adsorbing heavy metals from aqueous solutions. The adsorbent was characterized by SEM, FT-IR, Raman, and XPS analyses showing its porous architecture, rough surface, abundant N- and O-containing functional groups providing enhanced binding ability towards Pb and Cu. Experimental adsorption data fitted well to the pseudo-second-order kinetics and Langmuir isotherm models, indicating the adsorption of GO-HBP-NH-CMC towards Pb and Cu being a chemical and monolayer process.

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Article Synopsis
  • * Researchers studied how activated sludge can degrade BaP using phenol as a co-substrate, finding significant changes in the microbial community, particularly with different bacteria thriving under anaerobic or aerobic conditions.
  • * By employing bioinformatics tools, they predicted that certain dominant bacterial genera have the potential to break down PAHs/BaP, suggesting future experiments should investigate these bacteria under varying oxygen levels.
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Sludge collected from industrial wastewater treatment possesses a threatening effect on environment, and changing it into functional material provides an alternative for its disposal. Biochar synthesized by pyrolysis of sludge obtained from coking wastewater treatment was evaluated for the catalytic ozonation of phenol in aqueous solution. The present work focused on testing the catalytic performance of biochar, deducing the kinetics of phenol removal in various reaction conditions, and finally elucidating the mechanism of biochar-enhanced phenol removal.

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The need in simultaneous removal of heavy metals and organic compounds dictates the development of synthetic adsorbents with tailor-made properties. A nitrogen (N) and sulfur (S) co-doped graphene-based aerogel (GBA) modified with 2,5-dithiobisurea was synthesized hydrothermally for simultaneous adsorption of Cd and organic dyes-safranin-O (SO), crystal violet (CV), and methylene blue (MB). 2,5-Dithiobisurea was used as nitrogen and sulfur sources to introduce N and S-containing functional group onto graphene oxide.

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The simultaneous presence of heavy metals and organic acids in nature and wastewaters and their competition for adsorption sites determine the migration, transformation and fate of pollutants in the environment. A Cd-ion-imprinted polymer (Cd-IIP) with a thiol-functional group was hydrothermally synthesized by a surface imprinting technique combined with ultrasonic heating for selective adsorption of Cd from wastewaters. The adsorbent was characterized by SEM, EDS, XPS, BET and FT-IR measurements.

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Coking wastewater (CW) contains toxic and macromolecular substances that inhibit biological treatment. The refractory compounds remaining in biologically treated coking wastewater (BTCW) provide chemical oxygen demand (COD) and color levels that make it unacceptable for reuse or disposal. Gas-phase pulsed corona discharge (PCD) utilizing mostly hydroxyl radicals and ozone as oxidants was applied to both raw coking wastewater (RCW) and BTCW wastewater as a supplemental treatment.

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Polycyclic aromatic hydrocarbons (PAHs) are accumulated in the sludge collected from the coking wastewater treatment. Phenol with its efficient degradation observed in biological treatment promotes the solubility of PAHs in aqueous phase. The interaction mechanism of phenol and PAHs in aqueous and sludge phases was systematically studied in two full-scale engineering projects composed of anaerobic-oxic-oxic (A-O-O) and anaerobic-oxic-hydrolytic-oxic (A-O-H-O) sequences.

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Various products are observed in biological oxidation and reduction of molecules containing elements of variable valence. The variability is caused by the diversity of microorganisms and their metabolic enzymes, which may develop into novel processes in wastewater treatment. The study aimed to develop a novel denitrification process forming nitrite and ammonium in wastewaters containing thiocyanate.

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The highly energetic electrons in non-thermal plasma generated by gas phase pulsed corona discharge (PCD) produce hydroxyl (OH) radicals via collision reactions with water molecules. Previous work has established that OH radicals are formed at the plasma-liquid interface, making it an important location for the oxidation of aqueous pollutants. Here, by contacting water as aerosol with PCD plasma, it is shown that OH radicals are produced on the gas side of the interface, and not in the liquid phase.

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The anti-epileptic drug carbamazepine (CBZ) receives growing attention due to slow biodegradation and inherent accumulation in the aquatic environment. The application of a gas-phase pulsed corona discharge (PCD) was investigated to remove CBZ from synthetic solutions and spiked wastewater effluent from a municipal wastewater treatment facility. The treated water was showered between high voltage (HV) wires and grounded plate electrodes, to which ultra-short HV pulses were applied.

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Photocatalytic water splitting for hydrogen and oxygen production requires sacrificial electron donors, for example, organic compounds. Titanium dioxide catalysts doped with platinum, cobalt, tungsten, copper and iron were experimentally tested for the production of hydrogen, oxygen and low molecular weight hydrocarbons from aqueous solutions of humic substances (HS). Platinum-doped catalyst showed the best results in hydrogen generation, also producing methane, ethene and ethane, whereas the best oxygen production was exhibited by P25, followed by copper--and cobalt-containing photocatalysts.

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Lignin is the mass waste product of pulp and paper industry mostly incinerated for energy recovery. Lignin is, however, a substantial source of raw material for derivatives currently produced in costly wet oxidation processes. The pulsed corona discharge (PCD) for the first time was applied to lignin oxidation aiming a cost-effective environmentally friendly lignin removal and transformation to aldehydes.

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Oxidation of aromatic compounds of phenolic (paracetamol, beta-oestradiol and salicylic acid) and carboxylic (indomethacin and ibuprofen) structure used in pharmaceutics was studied. Aqueous solutions were treated with pulsed corona discharge (PCD) as a means for advanced oxidation. Pulse repetition frequency, delivered energy dose and oxidation media were the main parameters studied for their influence on the process energy efficiency.

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Photocatalytic oxidation (PCO) of acrylonitrile (AN) on titanium dioxide in the gaseous phase was studied. AN readily undergoes photocatalytic degradation in a gas-solid system by using TiO(2) Degussa P25. The AN PCO volatile products, visible in the infrared spectra, included nitrogen dioxide, nitrous oxide, carbon dioxide, water, hydrogen cyanide and carbon monoxide.

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