Spin torque-driven electron paramagnetic resonance of a single spin in a pentacene molecule.

Control over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here, we demonstrate coherent driving of a single spin by a radiofrequency spin-polarized current injected from the tip of a scanning tunneling microscope into an organic molecule.

A mixed-methods evaluation of the impacts of an online Carer wellbeing and connection program.

Objective: To evaluate a facilitated, 90-min session, delivered for four weeks, Online Carer Wellbeing and Connection Program in Victoria, Australia.

Methods: One hundred and three carers took part in the evaluation. Eighty-six completed both pre- and post-program surveys evaluating program impacts on psychological distress, perceived loneliness, and social support.

Electron Paramagnetic Resonance of Alkali Metal Atoms and Dimers on Ultrathin MgO.

Electron paramagnetic resonance (EPR) can provide unique insight into the chemical structure and magnetic properties of dopants in oxide and semiconducting materials that are of interest for applications in electronics, catalysis, and quantum sensing. Here, we demonstrate that EPR in combination with scanning tunneling microscopy (STM) allows for probing the bonding and charge state of alkali metal atoms on an ultrathin magnesium oxide layer on a Ag substrate. We observe a magnetic moment of 1 μ for Li, LiNa, and Na dimers corresponding to spin radicals with a charge state of +1.

Longitudinal and transverse electron paramagnetic resonance in a scanning tunneling microscope.

Electron paramagnetic resonance (EPR) spectroscopy is widely used to characterize paramagnetic complexes. Recently, EPR combined with scanning tunneling microscopy (STM) achieved single-spin sensitivity with sub-angstrom spatial resolution. The excitation mechanism of EPR in STM, however, is broadly debated, raising concerns about widespread application of this technique.

Vacuum Resonance States as Atomic-Scale Probes of Noncollinear Surface Magnetism.

The reflection of electrons at noncollinear magnetic surfaces is investigated by spin-polarized scanning tunneling microscopy and spectroscopy on unoccupied resonance states located in vacuo. Even for energies up to 20 eV above the Fermi level, the resonance states are found to be spin split, exhibiting the same local spin quantization axis as the underlying spin texture. Mapping the spin-dependent electron phase shift upon reflection at the surface on the atomic scale demonstrates the relevance of all magnetic ground state interactions for the scattering of spin-polarized low-energy electrons.