Optical vortex induced spatio-temporally modulated superconductivity in a high-T cuprate.

We report an experimental approach to produce spatially localized photoinduced superconducting state in a cuprate superconductor using optical vortices with ultrafast pulses. The measurements were carried out using coaxially aligned three-pulse time-resolved spectroscopy, in which an intense vortex pulse was used for coherent quenching of superconductivity and the resulting spatially modulated metastable states were analyzed by the pump-probe spectroscopy. The transient response after quenching shows a spatially localized superconducting state that remains unquenched at the dark core of the vortex beam for a few picoseconds.

Ultrafast beam pattern modulation by superposition of chirped optical vortex pulses.

As an extension of pulse shaping techniques using the space-time coupling of ultrashort pulses or chirped pulses, we demonstrated the ultrafast beam pattern modulation by the superposition of chirped optical vortex pulses with orthogonal spatial modes. The stable and robust modulations with a modulation frequency of sub-THz were carried out by using the precise phase control technique of the constituent pulses in both the spatial and time/frequency domains. The performed modulations were ultrafast ring-shaped optical lattice modulation with 2, 4 and 6 petals, and beam pattern modulations in the radial direction.

Comprehensive quantitative analysis of vector beam states based on vector field reconstruction.

We demonstrate a comprehensive quantitative analysis of vector beam states (VBSs) by using a vector field reconstruction (VFR) technique integrating interferometry and imaging polarimetry, where the analysis is given by a cylindrically polarized Laguerre-Gaussian (LG) mode expansion of VBSs. From test examples of cylindrically polarized LG mode beams, we obtain the complex amplitude distributions of VBSs and perform their quantitative evaluations both in radial and azimuthal directions. The results show that we generated (l, p) = (1, 0) LG radially polarized state with a high purity of 98%.

Generation of arbitrary axisymmetrically polarized pulses by using the combination of 4-f spatial light modulator and common-path optical system.

We proposed and constructed a system to realize broadband generation of arbitrary axisymmetrically polarized (AP) pulses with spatial complex amplitude modulation. This system employs the combination of a spatial light modulator in the 4-f configuration (4-f SLM), and a space variant wave plate as a common path interferometer. The 4-f SLM and the common path interferometer offer compensation for spatial dispersion with respect to wavelength and stability to perturbation, respectively.

Focus issue introduction: synergy of structured light and structured materials.

Structured light beams, such as optical vortices, vector beams, and non-diffracting beams, have been recently studied in a variety of fields, such as optical manipulations, optical telecommunications, nonlinear interactions, quantum physics, and 'super resolution' microscopy.. Their unique physical properties, such as annular intensity profile, helical wavefront and orbital angular momentum, give rise to a plethora of new, fundamental light-matter interactions and device applications.

Picosecond optical vortex pulse illumination forms a monocrystalline silicon needle.

The formation of a monocrystalline silicon needle by picosecond optical vortex pulse illumination was demonstrated for the first time in this study. The dynamics of this silicon needle formation was further revealed by employing an ultrahigh-speed camera. The melted silicon was collected through picosecond pulse deposition to the dark core of the optical vortex, forming the silicon needle on a submicrosecond time scale.

Full Quantitative Analysis of Arbitrary Cylindrically Polarized Pulses by Using Extended Stokes Parameters.

Cylindrically polarized (CP) modes are laser beam modes which have rotational symmetry of the polarization distribution around the beam axis. Considerable attention has been paid to CP modes for their various applications. In this paper, by using the extended Stokes parameters and the degree of polarization defined for the spatial distribution (DOP-SD), we fully-quantitatively characterize the spectrally-resolved polarization states of arbitrary CP (axisymmetrically polarized and higher-order cylindrically polarized) broadband pulses generated by coherent beam combining.

Nonlinear coupling between axisymmetrically-polarized ultrashort optical pulses in a uniaxial crystal.

Nonlinear propagation of focused axisymmetrically-polarized ultrashort optical pulses along the optic axis in a uniaxial crystal is investigated experimentally and theoretically. The energy transfer between an azimuthally-polarized pulse and a radially-polarized pulse is observed. To analyze the nonlinear propagation, a general paraxial equation with a third-order nonlinearity for axisymmetrically-polarized pulses in a uniaxial crystal is derived and the extended Stokes parameters (ESPs) based on cylindrical coordinates are newly-introduced.

Stable and flexible ring-shaped optical-lattice generation by use of axially symmetric polarization elements.

To overcome a trade-off issue between stability and flexibility in the generation of ring-shaped optical lattices, we proposed and demonstrated a novel generation method by using axially symmetric polarization elements. While two optical vortices were coaxially generated, electrically controlled phase difference between them by an electro-optic modulator enabled a precise rotation of the lattice. Our method has the capability to fulfill the high stability and rapid rotation.

Transfer of light helicity to nanostructures.

We discovered that chiral nanoneedles fabricated by vortex laser ablation can be used to visualize the helicity of an optical vortex. The orbital angular momentum of light determines the chirality of the nanoneedles, since it is transferred from the optical vortex to the metal. Only the spin angular momentum of the optical vortex can reinforce the helical structure of the created chiral nanoneedles.

Ultrashort optical-vortex pulse generation in few-cycle regime.

We generated a 2.3-cycle, 5.9-fs, 56-μJ ultrashort optical-vortex pulse (ranging from ~650 to ~950 nm) in few-cycle regime, by optical parametric amplification.

Using optical vortex to control the chirality of twisted metal nanostructures.

We discovered for the first time that light can twist metal to control the chirality of metal nanostructures (hereafter, chiral metal nanoneedles). The helicity of optical vortices is transferred to the constituent elements of the irradiated material (mostly melted material), resulting in the formation of chiral metal nanoneedles. The chirality of these nanoneedles could be controlled by just changing the sign of the helicity of the optical vortex.

Metal microneedle fabrication using twisted light with spin.

Microneedle fabrication on a metal surface based on laser ablation using twisted light with spin was demonstrated, for the first time. The resulting needle showed a height of at least 10 microm above the target surface and a tip diameter of less than 0.3 microm.

Optical-vortex laser ablation.

Laser ablation of Ta plates using nanosecond optical vortex pulses was carried out, for the first time. It was suggested that owing to orbital angular momentum of optical vortex, clearer and smoother processed surfaces were obtained with less ablation threshold fluence, in comparison with the ablation by a nonvortex annular beam modified from a spatially Gaussian beam.

Global evaluation of closed-loop electron dynamics in quasi-one-dimensional conductors using polarization vortices.

We evaluate the quasi-one-dimensional (1D) electron dynamics in a NbSe3 ring crystal using polarization vortex pulses with various azimuthal distributions. The single particle relaxation component reveals a large anisotropy on the crystal, indicating that the electrons in the ring maintain their 1D character. The results also suggest that the polarization vortex evaluates the global polarization property of the closed-loop electron that plays an important role in the quantum correlation phenomena such as the Aharonov-Bohm effect.

Supercontinuum optical vortex pulse generation without spatial or topological-charge dispersion.

A new achromatic method to generate the optical vortex was proposed and supercontinuum optical vortex generation ranging approximately 500 to approximately 800 nm was experimentally demonstrated without spatial nor topological-charge dispersions. In addition, polarization evolution in our system using Jones vectors and matrices was discussed and the condition of the polarizer to transfer polarizations was elucidated. This method is useful for the application to time-resolved nonlinear spectroscopy utilizing ultrabroadband optical vortex pulses in topological materials such as ring-shaped crystals or annular materials.

Direct production of high-power radially polarized output from a side-pumped Nd:YVO4 bounce amplifier using a photonic crystal mirror.

We produced a high power radially-polarized output directly from a diode-pumped Nd:YVO(4) bounce amplifier, using an autocloned photonic crystal mirror as an output coupler, with a simple cavity configuration. The radially-polarized output power of approximately 6 W was achieved, and a corresponding slope efficiency was estimated to be approximately 17 %. The output was characterized to be an ideal radially-polarized beam from its polarization distribution profiles.

Direct observation of Gouy phase shift in a propagating optical vortex.

Direct observation of Gouy phase shift on an optical vortex was presented through investigating the intensity profiles of a modified LG_p;m beam with an asymmetric defect, around at the focal point. It was quantitatively found that the rotation profile of a modified LG_p;m beam manifests the Gouy phase effect where the rotation direction depends on only the sign of topological charge m. This profile measurement method by introducing an asymmetric defect is a simple and useful technique for obtaining the information of the Gouy phase shift, without need of a conventional interference method.

Optical pulse compression to 3.4 fs in the monocycle region by feedback phase compensation.

We compensated for chirp of optical pulses with an over-one-octave bandwidth (495-1090 nm; center wavelength of 655.4 nm) produced by self-phase modulation in a single argon-filled hollow fiber and generated 3.4-fs, 1.