The satellite-based tropospheric column ratio of HCHO to NO (FNR) is widely used to diagnose ozone formation sensitivity; however, its representation of surface conditions remains controversial. In this study, an approach to construct the 3D spatial distribution of the FNR in the lower troposphere was proposed. Based on satellite and multiaxes-differential Optical Absorption Spectroscopy (MAX-DOAS) data, the horizontal and vertical distributions of the FNR have been respectively obtained.
View Article and Find Full Text PDFAs an important precursor of secondary inorganic aerosols (SIAs), ammonia (NH) plays a key role in fine particulate matter (PM) formation. In order to investigate its impacts on haze formation in the North China Plain (NCP) during winter, NH concentrations were observed at a high-temporal resolution of 1 min by using the SP-DOAS in Tai'an from December 2021 to February 2022. During the observation period, the average NH concentration was 11.
View Article and Find Full Text PDFTropospheric reactive bromine is important for atmospheric chemistry, regional air pollution, and global climate. Previous studies have reported measurements of atmospheric reactive bromine species in different environments, and proposed their main sources, e.g.
View Article and Find Full Text PDFCuI films present promising optoelectronic properties for transparent conductors. However, the high hole concentration in CuI films hinders the controllable modulation of hole mobility, limiting their application in low-dimensional thin-film transistors. In this study, CuI films were prepared through a Cu film iodination method at room temperature, and a systematic investigation was conducted on the modulation of hole concentration and mobility with varying film thickness.
View Article and Find Full Text PDFJ Environ Sci (China)
February 2024
Increased attentions to vehicle emission of NH have been paid since it is generally regarded as an important source in urban areas. Here, we developed a movable instrument based on Differential Optical Absorption Spectroscopy (DOAS) principle for detecting on-road NH, which can avoid the losses in the sampling process attributed to the non-sampling methods. For this mobile DOAS, the temporal resolution, detection limit and relative error for NH were 1 min, 2.
View Article and Find Full Text PDFJ Environ Sci (China)
January 2023
Nitrous acid (HONO) is considered as one of the main sources of the hydroxyl radical (OH), the most relevant oxidant in the atmosphere. Multi-AXis-Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements were conducted to obtain the vertical profiles of aerosol and HONO from November 1, 2020 to January 31, 2021 at a suburb site of Shanghai, China. HONO was mainly distributed near the surface, but high values HONO occasionally occurred around 0.
View Article and Find Full Text PDFResponses to the COVID-19 pandemic led to major reductions on air pollutant emissions in modern history. To date, there has been no comprehensive assessment for the impact of lockdowns on the vertical distributions of nitrogen dioxide (NO) and formaldehyde (HCHO). Based on profiles from 0 to 2 km retrieved by Multi-AXis-Differential Optical Absorption Spectroscopy observation and a large volume of real-time data at a suburb site in Shanghai, China, four types of machine learning models were developed and compared, including multiple linear regression, support vector machine, bagged trees (BT), and artificial neural network.
View Article and Find Full Text PDFBackground: The spatiotemporal variation of observed trace gases (NO, SO, O) and particulate matter (PM, PM) were investigated over cities of Yangtze River Delta (YRD) region including Nanjing, Hefei, Shanghai and Hangzhou. Furthermore, the characteristics of different pollution episodes, i.e.
View Article and Find Full Text PDFAim: The aim of this study was to understand the effects of revegetation on the diversity of bacteria and fungi in soil by sowing a single species and exploring the underlying mechanism.
Location: Beijing, China.
Taxon: Plants and Microbes.