The life cycle assessment methodology is a comprehensive environmental impact evaluation approach rooted in the "cradle-to-grave" concept. This study takes a municipal solid waste incineration power plant in central China as an example to comprehensively explore the potential ecological and environmental impacts of municipal solid waste incineration power generation through life cycle assessment methods. Burning one ton of waste can recover 7342 joules of thermal energy.
View Article and Find Full Text PDFBased on the life cycle assessment methodology, this study systematically analyzes the energy utilization of environmental waste through photocatalytic treatment and simultaneous hydrogen production. Using 10,000 tons of organic wastewater as the functional unit, the study evaluates the material consumption, energy utilization, and environmental impact potential of the photocatalytic waste synchronous hydrogen production system (specifically, the synchronous hydrogen production process of 4-NP wastewater with CDs/CdS/CNU). The findings indicate that potential environmental impacts from the photochemical treatment of environmental waste and synchronous hydrogen production primarily manifest in freshwater ecological toxicity, marine ecological toxicity, terrestrial ecological toxicity, and non-carcinogenic toxicity to humans.
View Article and Find Full Text PDFPorous carbon materials are highly desirable for removing benzene due to their low energy for capture and regeneration. Research has demonstrated that narrow microporous volume is crucial for effective adsorption of benzene at ultra-low concentration. Unfortunately, achieving directional increase in the narrow microporous volume in porous carbon remains a challenge.
View Article and Find Full Text PDFPrevious reports have shown that it is difficult to improve the methanol adsorption performance of nitrogen and oxygen groups due to their low polarity. Here, we first prepared porous carbon with a high specific surface area and large pore volume using benzimidazole as a carbon precursor and KOH as an activating agent. Then, we improved the surface polarity of the porous carbon by doping with Lithium (Li) to enhance the methanol adsorption performance.
View Article and Find Full Text PDFThe influence of different pore size and oxygen groups for porous carbons on acetone adsorption at different pressure was studied by using experimental data and theoretical calculation, and the results were applied to prepare carbon-based adsorbents with superior adsorption capacity. First, we successfully prepared five types of porous carbons with different gradient pore structure but similar oxygen contents (4.9 ± 0.
View Article and Find Full Text PDFLead-zinc tailings are complex heavy metal solid wastes produced in the mining process. In this study, two kinds of organic-inorganic mixed improvers mushroom residue + calcium carbonate (M + C) and peat soil + calcium carbonate (N + C) were selected. Then, the effect of two improvers and a woody plant, Nerium oleander L.
View Article and Find Full Text PDFInt J Environ Res Public Health
November 2022
Phytoremediation could be an alternative strategy for lead (Pb) contamination. has been reported as a newly potential plant for sustainable phytoremediation of Pb-contaminated soil. Physiological indexes, enrichment accumulation characteristics, Pb subcellular distribution and microstructure of were carefully studied at different levels of Pb stress (0-1200 mg/L).
View Article and Find Full Text PDFInt J Environ Res Public Health
October 2022
Traditional wastewater treatment technologies have become increasingly inefficient to meet the needs of low-consumption and sustainable wastewater treatment. Researchers are committed to seeking new wastewater treatment technologies, to reduce the pressure on the environment caused by resource shortages. Recently, a microalgal-bacterial granular sludge (MBGS) technology has attracted widespread attention due to its high efficiency wastewater treatment capacity, low energy consumption, low CO emissions, potentially high added values, and resource recovery capabilities.
View Article and Find Full Text PDFInt J Environ Res Public Health
October 2022
Nowadays, with the rapid development of industry and agriculture, heavy metal pollution is becoming more and more serious, mainly deriving from natural and man-made sources [...
View Article and Find Full Text PDFInt J Environ Res Public Health
September 2022
Advanced oxidation technology represented by hydroxyl radicals has great potential to remove residual antibiotics. In this study, we systematically compared the metronidazole (MTZ) degradation behavior and mechanism in the UV and UV/HO systems at pH 3.00 condition.
View Article and Find Full Text PDFPhytoremediation is an ecological technique for tailing area restoration; adding substrate modifiers can reduce the stress of heavy metals on plants and enhance the restoration efficiency. The woody plant was used as a test plant and potted in 100% tailings (S), 90% tailings+5% mushroom residue (SMC)+5% CaCO (MS), and natural red soil (RS). The effects of physiological responses and tolerance enrichment effects on Pb and Zn tolerance in under different treatments were investigated to compare the growth morphology, microscopic morphological changes, and microbial diversity changes in each substrate of seedlings.
View Article and Find Full Text PDFInt J Environ Res Public Health
September 2022
The high salt-alkalinity of bauxite residue (BR) hinders plant growth and revegetation of bauxite residue disposal areas (BRDA), which cause serious potential environmental and ecological risks. Bioneutralization is a promising method for improving the properties of BR and plant colonization. In the present study, a strong saline-alkali tolerant bacteria (ZH-1) was isolated from aged BR and identified as sp.
View Article and Find Full Text PDFInt J Environ Res Public Health
September 2022
With the rapid development of industrialization, human beings have caused many negative effects on the environment that have endangered the survival and development of human beings, such as the greenhouse effect, water pollution, energy depletion, etc [...
View Article and Find Full Text PDFAt present, the application of phytoremediation technology in the ecological remediation of heavy metal tailings is receiving more and more attention. In this study, the physiological and biochemical response and tolerance mechanism of woody plant Nerium indicum to Pb and Zn under different proportions of inorganic modifier calcium carbonate (C1: 5%, C2: 10%, C3: 15%) and organic modifier mushroom residue (M1: 10%, M2: 20%, M3: 30%) was compared. The results showed that the pH value has a trend of C group > M group > CK group and organic matter has a trend of M group > CK group > C group.
View Article and Find Full Text PDFIn this study, we investigated the removal efficiency of a broad-spectrum antimicrobial agent trimethoprim (TMP) in a UV-activated persulfate system (UV/PS). The pseudo-first-order reaction kinetic model based on the steady-state hypothesis was used to explain TMP degradation behavior in UV-activated persulfate system. Due to the low quantum yield and molar absorptivity of TMP at 254 nm, the direct photolysis of TMP was slower.
View Article and Find Full Text PDFLayer-structured graphene oxide excellent carrier for modifications; however, its poor recoverability and stability preclude its application in wastewater treatment fields. Herein, three-dimensional magnetic fungal hyphal/graphene oxide nanofibers (MFHGs) were assembled by a reductive self-assembly (RSA) strategy for the efficient capture of Co(II) and Ni(II) from high-salinity aqueous solution. The RSA strategy is inexpensive, eco-friendly and easy to scale up.
View Article and Find Full Text PDFWater pollution has caused the ecosystem to be in a state of imbalance for a long time. It has become a major global ecological and environmental problem today. Solving the potential hidden dangers of pollutants and avoiding unauthorized access to resources has become the necessary condition and important task to ensure the sustainable development of human society.
View Article and Find Full Text PDFA simple and practical method for the synthesis of thio-substituted esters through copper(i)-catalyzed intermolecular 1,2-estersulfenylation of styrenes with peroxyesters and disulfides was developed. In this transformation, two new C-S bond and C-O bond were constructed simultaneously under a copper catalyst system, and the transformation exhibits a broad substrate scope and good functional group compatibility. In addition, this method can also be applied to arylthiols.
View Article and Find Full Text PDFPhytoremediation is an effective strategy for the remediation of lead-zinc slag, while the response of plant on lead and zinc was less concerned. In this study, mushroom residue was adding in lead-zinc slag to enhance the phytoremediation potential of P. fortunei, the effects of three treatments (lead-zinc slag, red soil, lead-zinc slag + 10% (m/m) mushroom residue) on the growth, physiology and microstructure of P.
View Article and Find Full Text PDFAn annulation cascades of N-allyl- N-((2-bromoaryl)ethynyl)amides with terminal alkynes or 1,3-dicarbonyls involving C-H functionalization for producing 2,3-functionalized indoles has been first developed by means of Cu catalysis. The method is enabled by the formation of the ketenimine intermediates to deliver 2,3-disubstituted indoles through a sequence of aza-Claisen rearrangement, C-H functionalization, Ullmann C-N coupling, and cyclization.
View Article and Find Full Text PDFA new copper-catalyzed oxidative three-component intermolecular 1,2-alkylarylation of styrenes with ethers and indoles is disclosed. This method utilizes TBPB as an oxidant to efficiently construct C(sp)-C(sp) and C(sp)-C(sp) bonds in one step through probable radical and electrophilic alkylation processes, respectively, and a variety of functional groups are well tolerated.
View Article and Find Full Text PDFThe advanced oxidation technologies based on OH can effectively degrade the pharmaceutical and personal care products under operating conditions of normal temperature and pressure. In this study, direct photolysis of ibuprofen (IBU) is slow due to the relatively low molar extinction coefficient and quantum yield. Compared to direct photolysis, the degradation kinetics of IBU was significantly enhanced in the UV/HO system, mainly by OH radical mediated oxidation.
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