This article describes the development and application of hydrogen (H) chirped-probe-pulse femtosecond coherent anti-Stokes Raman scattering (CPP fs CARS) in high-temperature and high-pressure conditions. H fs CARS thermometry was performed in Hencken burner flames up to 2300 K, as well as in a heated gas-cell at temperatures up to 1000 K. It was observed that the H fs CARS spectra are highly sensitive to the pump and Stokes chirp.
View Article and Find Full Text PDFAn electro-optical shutter (EOS), comprising a Pockels cell located between crossed-axis polarizers, is integrated into a nanosecond coherent anti-Stokes Raman scattering (CARS) system. The use of the EOS enables thermometry measurements in high-luminosity flames through significant reduction of the background resulting from broadband flame emission. A temporal gating ≤100 ns along with an extinction ratio >10,000:1 are achieved using the EOS.
View Article and Find Full Text PDFThis paper discusses a novel model combustion experiment that was built for studying the structure and dynamics of a reacting jet in an unsteady crossflow. A natural-gas-fired dump combustor is used to generate and sustain an acoustically oscillating vitiated flow that serves as the crossflow for transverse jet injection. Unlike most other techniques that are limited in operating pressure or acoustic amplitude, this method of generating an unsteady flow field is demonstrated at a pressure of 10 atm with peak-to-peak oscillation amplitudes approaching 20% of the mean pressure.
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