Publications by authors named "Risto Makkonen"

A total of 16 global chemistry transport models and general circulation models have participated in this study; 14 models have been evaluated with regard to their ability to reproduce the near-surface observed number concentration of aerosol particles and cloud condensation nuclei (CCN), as well as derived cloud droplet number concentration (CDNC). Model results for the period 2011-2015 are compared with aerosol measurements (aerosol particle number, CCN and aerosol particle composition in the submicron fraction) from nine surface stations located in Europe and Japan. The evaluation focuses on the ability of models to simulate the average across time state in diverse environments and on the seasonal and short-term variability in the aerosol properties.

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A significant wetting trend since the early 1980s in Tibetan Plateau (TP) is most conspicuous in central and eastern Asia as shown in the instrumental data and the long-term moisture sensitive tree rings. We found that anomalies in the large-scale oceanic and atmospheric circulations do not play a significant role on the wetting trend in TP. Meanwhile, the weak correlation between local temperature and precipitation suggests that the temperature-induced enhancement of the local water cycle cannot fully explain the wetting trend either.

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Article Synopsis
  • Oxidation of monoterpenes and isoprene significantly impacts global secondary organic aerosol levels and the creation of atmospheric nanoparticles and cloud condensation nuclei (CCN).
  • Laboratory experiments reveal that extremely low volatility organic compounds (ELVOC) are produced rapidly after oxidation, with different efficiencies based on the molecular structure of the compounds.
  • Global modeling indicates that while monoterpene oxidation enhances particle formation and CCN concentrations, isoprene's oxidation has a mixed effect, suppressing new particle creation but aiding in the growth of smaller particles into CCN.
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