Homochiral antiferromagnetic merons, antimerons and bimerons realized in synthetic antiferromagnets.

The ever-growing demand for device miniaturization and energy efficiency in data storage and computing technology has prompted a shift towards antiferromagnetic topological spin textures as information carriers. This shift is primarily owing to their negligible stray fields, leading to higher possible device density and potentially ultrafast dynamics. We realize in this work such chiral in-plane topological antiferromagnetic spin textures namely merons, antimerons, and bimerons in synthetic antiferromagnets by concurrently engineering the effective perpendicular magnetic anisotropy, the interlayer exchange coupling, and the magnetic compensation ratio.

Robust Free Energy Perturbation Protocols for Creating Molecules in Solution.

Accurate methods to estimate free energies play an important role for studying diverse condensed-phase problems in chemistry and biochemistry. The most common methods used in conjunction with molecular dynamics (MD) and Monte Carlo statistical mechanics (MC) simulations are free energy perturbation (FEP) and thermodynamic integration (TI). For common applications featuring the conversion of one molecule to another, simulations are run in stages or multiple "λ-windows" to promote convergence of the results.

Emergent Gauge Fields from Curvature in Single Layers of Transition-Metal Dichalcogenides.

We analyze the electron dynamics in corrugated layers of transition-metal dichalcogenides. Due to the strong spin-orbit coupling, the intrinsic (Gaussian) curvature leads to an emergent gauge field associated with the Berry connection of the spinor wave function. We discuss the gauge field created by topological defects of the lattice, namely, tetragonal and octogonal disclinations and edge dislocations.

Realization of the Haldane-Kane-Mele Model in a System of Localized Spins.

We study a spin Hamiltonian for spin-orbit-coupled ferromagnets on the honeycomb lattice. At sufficiently low temperatures supporting the ordered phase, the effective Hamiltonian for magnons, the quanta of spin-wave excitations, is shown to be equivalent to the Haldane model for electrons, which indicates the nontrivial topology of the band and the existence of the associated edge state. At high temperatures comparable to the ferromagnetic-exchange strength, we take the Schwinger-boson representation of spins, in which the mean-field spinon band forms a bosonic counterpart of the Kane-Mele model.

Narrowing the Zero-Field Tunneling Resonance by Decreasing the Crystal Symmetry of Mn12 Acetate.

We report the discovery of a less symmetric crystalline phase of Mn12 acetate, a triclinic phase, resulting from recrystallizing the original tetragonal phase reported by Lis in acetonitrile and toluene. This new phase exhibits the same structure of Mn12 acetate clusters and the same positions of tunneling resonances on the magnetic field as the conventional tetragonal phase. However, the width of the zero-field resonance is at least 1 order of magnitude smaller-can be as low as 50 Oe-indicating very small inhomogeneous broadening due to dipolar and nuclear fields.