Publications by authors named "Ramesh Ramamoorthy"

The discovery of polar vortices and skyrmions in ferroelectric-dielectric superlattices [such as (PbTiO)/(SrTiO)] has ushered in an era of novel dipolar topologies and corresponding emergent phenomena. The key to creating such emergent features has generally been considered to be related to counterpoising strongly polar and non-polar materials thus creating the appropriate boundary conditions. This limits the utility these materials can have, however, by rendering (effectively) half of the structure unresponsive to applied stimuli.

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The exotic polarization configurations of topologically protected dipolar textures have opened new avenues for realizing novel phenomena absent in traditional ferroelectric systems. While multiple recent studies have revealed a diverse array of emergent properties in such polar topologies, the details of their atomic and mesoscale structures remain incomplete. Through atomic- and meso-scale imaging techniques, the emergence of a macroscopic ferroelectric polarization along both principal axes of the vortex lattice while performing phase-field modeling to probe the atomic scale origins of these distinct polarization components is demonstrated.

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Article Synopsis
  • Ultrafast stimuli can create stable states of matter that can't be achieved under normal conditions, highlighting the need to understand the relationship between ultrafast processes and these states.
  • The study uses advanced optical and X-ray techniques to observe how a polar vortex supercrystal forms in a specially designed material when it's excited by light, demonstrating various phases in just a few picoseconds.
  • Over time, fluctuations in the structure of the supercrystal are gradually eliminated, leading to the stable formation of a single vortex supercrystal phase, with theoretical models supporting these observations.
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  • - The 4D Camera is a high-speed sensor designed for electron microscopy, capable of scanning at 87,000 Hz and generating data at approximately 480 Gbit/s, which is processed by specialized computers handling large datasets between 10-700 GB in size.
  • - It features a back illuminated detector that can detect single electron events at voltages ranging from 30 to 300 kV, enabling efficient electron counting that compresses data size significantly (by 10-300 times).
  • - The camera allows for rapid analysis through open-source processing algorithms, facilitating complex scanning diffraction experiments typically done in scanning transmission electron microscopy.
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Spin waves in magnetic materials are promising information carriers for future computing technologies due to their ultra-low energy dissipation and long coherence length. Antiferromagnets are strong candidate materials due, in part, to their stability to external fields and larger group velocities. Multiferroic antiferromagnets, such as BiFeO (BFO), have an additional degree of freedom stemming from magnetoelectric coupling, allowing for control of the magnetic structure, and thus spin waves, with the electric field.

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Antiferromagnets have attracted significant attention in the field of magnonics, as promising candidates for ultralow-energy carriers for information transfer for future computing. The role of crystalline orientation distribution on magnon transport has received very little attention. In multiferroics such as BiFeO the coupling between antiferromagnetic and polar order imposes yet another boundary condition on spin transport.

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A 45-year-old woman on treatment for HIV infection with highly active antiretroviral therapy for the past 10 years presented to us with a history of Raynaud's phenomenon and hyperpigmentation of the skin for 2 years. She was diagnosed to have pulmonary arterial hypertension 8 months ago. On examination, she had salt-and-pepper pigmentation and sclerodactyly.

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  • Adaptive networks can adjust to changes in their environment, which is crucial for advancing technologies like nanodevices and neuromorphic computing.
  • Researchers visually tracked how nanodomain networks in superlattices respond to rapid light pulses, uncovering new metastable states and measuring these changes with precision.
  • The study reveals that light can significantly reshape domain boundaries in these networks, hinting at future applications in light-controlled nanocircuits similar to how synapses adapt in the brain.
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Stabilization of topological spin textures in layered magnets has the potential to drive the development of advanced low-dimensional spintronics devices. However, achieving reliable and flexible manipulation of the topological spin textures beyond skyrmion in a two-dimensional magnet system remains challenging. Here, we demonstrate the introduction of magnetic iron atoms between the van der Waals gap of a layered magnet, FeGaTe, to modify local anisotropic magnetic interactions.

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A magnon is a collective excitation of the spin structure in a magnetic insulator and can transmit spin angular momentum with negligible dissipation. This quantum of a spin wave has always been manipulated through magnetic dipoles (that is, by breaking time-reversal symmetry). Here we report the experimental observation of chiral spin transport in multiferroic BiFeO and its control by reversing the ferroelectric polarization (that is, by breaking spatial inversion symmetry).

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Bismuth ferrite (BiFeO) is a multiferroic material that exhibits both ferroelectricity and canted antiferromagnetism at room temperature, making it a unique candidate in the development of electric-field controllable magnetic devices. The magnetic moments in BiFeO are arranged into a spin cycloid, resulting in unique magnetic properties which are tied to the ferroelectric order. Previous understanding of this coupling has relied on average, mesoscale measurements.

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Overlap syndromes are diseases that meet the criteria of two or more rheumatic diseases. In this case report, a woman in her 20s presented with a constellation of symptoms, including skin thickening, Raynaud's phenomenon, hypertension, absent pulse in both lower limbs with bilateral renal artery bruit. The antinuclear antibody profile revealed Scl-70 positivity.

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As CMOS technologies face challenges in dimensional and voltage scaling, the demand for novel logic devices has never been greater, with spin-based devices offering scaling potential, at the cost of significantly high switching energies. Alternatively, magnetoelectric materials are predicted to enable low-power magnetization control, a solution with limited device-level results. Here, we demonstrate voltage-based magnetization switching and reading in nanodevices at room temperature, enabled by exchange coupling between multiferroic BiFeO and ferromagnetic CoFe, for writing, and spin-to-charge current conversion between CoFe and Pt, for reading.

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The recent discovery of polar topological structures has opened the door for exciting physics and emergent properties. There is, however, little methodology to engineer stability and ordering in these systems, properties of interest for engineering emergent functionalities. Notably, when the surface area is extended to arbitrary thicknesses, the topological polar texture becomes unstable.

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Retinal haemorrhage stands as an early indicator of diabetic retinopathy, necessitating accurate detection for timely diagnosis. Addressing this need, this study proposes an enhanced machine-based diagnostic test for diabetic retinopathy through an updated UNet framework, adept at scrutinizing fundus images for signs of retinal haemorrhages. The customized UNet underwent GPU training using the IDRiD database, validated against the publicly available DIARETDB1 and IDRiD datasets.

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Bismuth ferrite has garnered considerable attention as a promising candidate for magnetoelectric spin-orbit coupled logic-in-memory. As model systems, epitaxial BiFeO thin films have typically been deposited at relatively high temperatures (650-800 °C), higher than allowed for direct integration with silicon-CMOS platforms. Here, we circumvent this problem by growing lanthanum-substituted BiFeO at 450 °C (which is reasonably compatible with silicon-CMOS integration) on epitaxial BaPbBiO electrodes.

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2D layered materials with broken inversion symmetry are being extensively pursued as  spin source layers to realize high-efficiency magnetic switching. Such low-symmetry layered systems are, however, scarce. In addition, most layered magnets with perpendicular magnetic anisotropy show a low Curie temperature.

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Article Synopsis
  • Chirality, or handedness, is an important factor in discovering new electronic properties in materials for quantum information science, often found in natural biomolecules and magnetic materials.
  • Researchers engineered chirality in a specific ferroelectric/dielectric system using advanced techniques like four-dimensional scanning transmission electron microscopy (4D-STEM) to analyze three-dimensional domain walls and their interactions.
  • The unique characteristics of these domain walls, influenced by local polarization and symmetry-breaking, lead to the formation of triple points, which could enhance electrostatic and magnetic properties relevant for quantum sensing technologies.
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Four-dimensional scanning transmission electron microscopy (4D-STEM) has recently gained widespread attention for its ability to image atomic electric fields with sub-Ångstrom spatial resolution. These electric field maps represent the integrated effect of the nucleus, core electrons and valence electrons, and separating their contributions is non-trivial. In this paper, we utilized simultaneously acquired 4D-STEM center of mass (CoM) images and annular dark field (ADF) images to determine the projected electron charge density in monolayer MoS.

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Nontrivial polarization textures have been demonstrated in ferroelectric/dielectric superlattices, where the electrostatic, elastic, and different gradient energies compete in a delicate balance. When PbTiO/SrTiO superlattices are grown on DyScO, the coexistence of ferroelectric domains and vortex structure is observed for = 12-20 unit cells. Here, we report an approach to achieve single-phase vortex structures in superlattices by controlling the epitaxial strain using SrAlGaTaO substrates.

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Complex-oxide superlattices provide a pathway to numerous emergent phenomena because of the juxtaposition of disparate properties and the strong interfacial interactions in these unit-cell-precise structures. This is particularly true in superlattices of ferroelectric and dielectric materials, wherein new forms of ferroelectricity, exotic dipolar textures, and distinctive domain structures can be produced. Here, relaxor-like behavior, typically associated with the chemical inhomogeneity and complexity of solid solutions, is observed in (BaTiO ) /(SrTiO ) (n = 4-20 unit cells) superlattices.

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Control and understanding of ensembles of skyrmions is important for realization of future technologies. In particular, the order-disorder transition associated with the 2D lattice of magnetic skyrmions can have significant implications for transport and other dynamic functionalities. To date, skyrmion ensembles have been primarily studied in bulk crystals, or as isolated skyrmions in thin film devices.

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Nanobeam electron diffraction can probe local structural properties of complex crystalline materials including phase, orientation, tilt, strain, and polarization. Ideally, each diffraction pattern from a projected area of a few unit cells would produce a clear Bragg diffraction pattern, where the reciprocal lattice vectors can be measured from the spacing of the diffracted spots, and the spot intensities are equal to the square of the structure factor amplitudes. However, many samples are too thick for this simple interpretation of their diffraction patterns, as multiple scattering of the electron beam can produce a highly nonlinear relationship between the spot intensities and the underlying structure.

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Topologically protected polar textures have provided a rich playground for the exploration of novel, emergent phenomena. Recent discoveries indicate that ferroelectric vortices and skyrmions not only host properties markedly different from traditional ferroelectrics, but also that these properties can be harnessed for unique memory devices. Using a combination of capacitor-based capacitance measurements and computational models, it is demonstrated that polar vortices in dielectric-ferroelectric-dielectric trilayers exhibit classical ferroelectric bi-stability together with the existence of low-field metastable polarization states.

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