Novel materials of (E)-N'-(4-chlorobenzylidene)-4-hydroxybenzohydrazide (CBHB) and (E)-N'-(4-(diethylamino) benzylidene)-4-hydroxybenzohydrazide (DEABHB) were synthesized by condensation reaction process and solvent evaporation method was employed to grow CBHB and DEABHB single crystals at room temperature. Lattice parameters of CBHB and DEABHB compounds were recorded using single crystal X-ray diffraction method. The presence of functional groups of the synthesized CBHB and DEABHB compounds were confirmed by Fourier transform infrared and Fourier transform Raman spectral analyses.
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