Improved characterization of ambient PM mass concentration and chemical speciation is a topic of interest in air quality and climate sciences. Over the past decades, considerable efforts have been made to improve ground-level PM using remotely sensed data. Here we present two new approaches for estimating atmospheric PM and chemical composition based on the High Spectral Resolution Lidar (HSRL)-retrieved aerosol extinction values and types and Creating Aerosol Types from Chemistry (CATCH)-derived aerosol chemical composition.
View Article and Find Full Text PDFTo improve our understanding of the complex role of aerosols in the climate system and on air quality, measurements are needed of optical and microphysical aerosol. From many studies, it has become evident that a satellite-based multiangle, multiwavelength polarimeter will be essential to provide such measurements. Here, high accuracy (∼0.
View Article and Find Full Text PDFWe evaluate the retrieval performance of the automated, unsupervised inversion algorithm, Tikhonov Advanced Regularization Algorithm (TiARA), which is used for the autonomous retrieval of microphysical parameters of anthropogenic and natural pollution particles. TiARA (version 1.0) has been developed in the past 10 years and builds on the legacy of a data-operator-controlled inversion algorithm used since 1998 for the analysis of data from multiwavelength Raman lidar.
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