Magnetic kagome materials provide a fascinating playground for exploring the interplay of magnetism, correlation and topology. Many magnetic kagome systems have been reported including the binary FeX (X = Sn, Ge; m:n = 3:1, 3:2, 1:1) family and the rare earth RMnSn (R = rare earth) family, where their kagome flat bands are calculated to be near the Fermi level in the paramagnetic phase. While partially filling a kagome flat band is predicted to give rise to a Stoner-type ferromagnetism, experimental visualization of the magnetic splitting across the ordering temperature has not been reported for any of these systems due to the high ordering temperatures, hence leaving the nature of magnetism in kagome magnets an open question.
View Article and Find Full Text PDFStudies on the heavy-fermion pyrochlore iridate (Pr_{2}Ir_{2}O_{7}) point to the role of time-reversal-symmetry breaking in geometrically frustrated Kondo lattices. Here, we address the effect of Kondo coupling and chiral spin liquids in a J_{1}-J_{2} model on a square lattice and a model on a kagome lattice via a large-N method, based on a fermionic representation of the spin operators, and consider a new mechanism for anomalous Hall effect for the chiral phases. We calculate the anomalous Hall response for the chiral states of both the Kondo destroyed and Kondo screened phases.
View Article and Find Full Text PDFFlat electronic bands are expected to show proportionally enhanced electron correlations, which may generate a plethora of novel quantum phases and unusual low-energy excitations. They are increasingly being pursued in d-electron-based systems with crystalline lattices that feature destructive electronic interference, where they are often topological. Such flat bands, though, are generically located far away from the Fermi energy, which limits their capacity to partake in the low-energy physics.
View Article and Find Full Text PDFNon-volatile phase-change memory devices utilize local heating to toggle between crystalline and amorphous states with distinct electrical properties. Expanding on this kind of switching to two topologically distinct phases requires controlled non-volatile switching between two crystalline phases with distinct symmetries. Here, we report the observation of reversible and non-volatile switching between two stable and closely related crystal structures, with remarkably distinct electronic structures, in the near-room-temperature van der Waals ferromagnet FeGeTe.
View Article and Find Full Text PDFStrange-metal behavior has been observed in materials ranging from high-temperature superconductors to heavy fermion metals. In conventional metals, current is carried by quasiparticles; although it has been suggested that quasiparticles are absent in strange metals, direct experimental evidence is lacking. We measured shot noise to probe the granularity of the current-carrying excitations in nanowires of the heavy fermion strange metal YbRhSi.
View Article and Find Full Text PDFFlat bands amplify correlation effects and are of extensive current interest. They provide a platform to explore both topology in correlated settings and correlation physics enriched by topology. Recent experiments in correlated kagome metals have found evidence for strange-metal behavior.
View Article and Find Full Text PDFStrange metals appear in a wide range of correlated materials. Electronic localization-delocalization and the expected loss of quasiparticles characterize beyond-Landau metallic quantum critical points and the associated strange metals. Typical settings involve local spins.
View Article and Find Full Text PDFKagome materials often host exotic quantum phases, including spin liquids, Chern gap, charge density wave, and superconductivity. Existing scanning microscopy studies of the kagome charge order have been limited to nonkagome surface layers. Here, we tunnel into the kagome lattice of FeGe to uncover features of the charge order.
View Article and Find Full Text PDFIt is becoming increasingly clear that breakthrough in quantum applications necessitates materials innovation. In high demand are conductors with robust topological states that can be manipulated at will. This is what we demonstrate in the present work.
View Article and Find Full Text PDFThe observation of quantum criticality in diverse classes of strongly correlated electron systems has been instrumental in establishing ordering principles, discovering new phases, and identifying the relevant degrees of freedom and interactions. At focus so far have been insulators and metals. Semimetals, which are of great current interest as candidate phases with nontrivial topology, are much less explored in experiments.
View Article and Find Full Text PDFMagnetic fluctuations induced by geometric frustration of local Ir-spins disturb the formation of long-range magnetic order in the family of pyrochlore iridates. As a consequence, PrIrO lies at a tuning-free antiferromagnetic-to-paramagnetic quantum critical point and exhibits an array of complex phenomena including the Kondo effect, biquadratic band structure, and metallic spin liquid. Using spectroscopic imaging with the scanning tunneling microscope, complemented with machine learning, density functional theory and theoretical modeling, we probe the local electronic states in PrIrO and find an electronic phase separation.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
February 2021
Nontrivial topology in condensed-matter systems enriches quantum states of matter to go beyond either the classification into metals and insulators in terms of conventional band theory or that of symmetry-broken phases by Landau's order parameter framework. So far, focus has been on weakly interacting systems, and little is known about the limit of strong electron correlations. Heavy fermion systems are a highly versatile platform to explore this regime.
View Article and Find Full Text PDFSpin-triplet superconductors are of extensive current interest because they can host topological state and Majorana fermions important for quantum computation. The uranium-based heavy-fermion superconductor UTe_{2} has been argued as a spin-triplet superconductor similar to UGe_{2}, URhGe, and UCoGe, where the superconducting phase is near (or coexists with) a ferromagnetic (FM) instability and spin-triplet electron pairing is driven by FM spin fluctuations. Here we use neutron scattering to show that, although UTe_{2} exhibits no static magnetic order down to 0.
View Article and Find Full Text PDFFractionalized excitations develop in many unusual many-body states such as quantum spin liquids, disordered phases that cannot be described using any local order parameter. Because these exotic excitations correspond to emergent degrees of freedom, how to probe them and establish their existence is a long-standing challenge. We present a general procedure to reveal the fractionalized excitations using real-space entanglement entropy in critical spin liquids that are particularly relevant to experiments.
View Article and Find Full Text PDFQuantum critical points often arise in metals perched at the border of an antiferromagnetic order. The recent observation of singular and dynamically scaling charge conductivity in an antiferromagnetic quantum critical heavy fermion metal implicates beyond-Landau quantum criticality. Here we study the charge and spin dynamics of a Kondo destruction quantum critical point (QCP), as realized in an SU(2)-symmetric Bose-Fermi Kondo model.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
September 2019
Complex and correlated quantum systems with promise for new functionality often involve entwined electronic degrees of freedom. In such materials, highly unusual properties emerge and could be the result of electron localization. Here, a cubic heavy fermion metal governed by spins and orbitals is chosen as a model system for this physics.
View Article and Find Full Text PDFMotivated by the recent low-temperature experiments on bulk FeSe, we study the electron correlation effects in a multiorbital model for this compound in the nematic phase using the U(1) slave-spin theory. We find that a finite nematic order helps to stabilize an orbital selective Mott phase. Moreover, we propose that when the d- and s-wave bond nematic orders are combined with the ferro-orbital order, there exists a surprisingly large orbital selectivity between the xz and yz orbitals even though the associated band splitting is relatively small.
View Article and Find Full Text PDFThe nature of the pairing symmetry of the first heavy fermion superconductor CeCuSi has recently become the subject of controversy. While CeCuSi was generally believed to be a d-wave superconductor, recent low-temperature specific heat measurements showed evidence for fully gapped superconductivity, contrary to the nodal behavior inferred from earlier results. Here, we report London penetration depth measurements, which also reveal fully gapped behavior at very low temperatures.
View Article and Find Full Text PDFInsulating states can be topologically nontrivial, a well-established notion that is exemplified by the quantum Hall effect and topological insulators. By contrast, topological metals have not been experimentally evidenced until recently. In systems with strong correlations, they have yet to be identified.
View Article and Find Full Text PDFWe report on temperature-dependent pair distribution function measurements of Sr_{1-x}Na_{x}Fe_{2}As_{2}, an iron-based superconductor system that contains a magnetic phase with reentrant tetragonal symmetry, known as the magnetic C_{4} phase. Quantitative refinements indicate that the instantaneous local structure in the C_{4} phase comprises fluctuating orthorhombic regions with a length scale of ∼2 nm, despite the tetragonal symmetry of the average static structure. Additionally, local orthorhombic fluctuations exist on a similar length scale at temperatures well into the paramagnetic tetragonal phase.
View Article and Find Full Text PDFSci Bull (Beijing)
November 2017
SmB has been a well-known Kondo insulator for decades, but recently attracts extensive new attention as a candidate topological system. Studying SmB under pressure provides an opportunity to acquire the much-needed understanding about the effect of electron correlations on both the metallic surface state and bulk insulating state. Here we do so by studying the evolution of two transport gaps (low temperature gap E and high temperature gap E) associated with the Kondo effect by measuring the electrical resistivity under high pressure and low temperature (0.
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