In this paper, we demonstrate a novel optical characterization method for ultrathin semitransparent and absorbing materials through multispectral intensity and phase imaging. The method is based on a lateral-shearing interferometric microscopy (LIM) technique, where phase-shifting allows extraction of both the intensity and the phase of transmitted optical fields. To demonstrate the performance in characterizing semitransparent thin films, we fabricated and measured cupric oxide (CuO) seeded gold ultrathin metal films (UTMFs) with mass-equivalent thicknesses from 2 to 27 nm on fused silica substrates.
View Article and Find Full Text PDFTraditional multilayer antireflection (AR) surfaces are of significant importance for numerous applications, such as laser optics, camera lenses, and eyeglasses. Recently, technological advances in the fabrication of biomimetic AR surfaces capable of delivering broadband omnidirectional high transparency combined with self-cleaning properties have opened an alternative route toward realization of multifunctional surfaces which would be beneficial for touchscreen displays or solar harvesting devices. However, achieving the desired surface properties often requires sophisticated lithography fabrication methods consisting of multiple steps.
View Article and Find Full Text PDFCompressing light into nanocavities substantially enhances light-matter interactions, which has been a major driver for nanostructured materials research. However, extreme confinement generally comes at the cost of absorption and low resonator quality factors. Here we suggest an alternative optical multimodal confinement mechanism, unlocking the potential of hyperbolic phonon polaritons in isotopically pure hexagonal boron nitride.
View Article and Find Full Text PDFAdvances in optical imaging always look for an increase in sensitivity and resolution among other practicability aspects. Within the same scope, in this work we report a versatile interference contrast imaging technique, with high phase sensitivity and a large field-of-view of several mm. Sensitivity is increased through the use of a self-imaging non-resonant cavity, which causes photons to probe the sample in multiple rounds before being detected, where the configuration can be transmissive or reflective.
View Article and Find Full Text PDFWe present a new compact and robust polarization state transmitter designed to execute the BB84 quantum key distribution protocol. Our transmitter prepares polarization states using a single commercial-off-the-shelf phase modulator. Our scheme does not require global biasing to compensate thermal and mechanical drifts, as both of the system's two time-demultiplexed polarization modes share a single optical path.
View Article and Find Full Text PDFPhotonic crystals and metamaterials are two overarching paradigms for manipulating light. By combining these approaches, hypercrystals can be created, which are hyperbolic dispersion metamaterials that undergo periodic modulation and mix photonic-crystal-like aspects with hyperbolic dispersion physics. Despite several attempts, there has been limited experimental realization of hypercrystals due to technical and design constraints.
View Article and Find Full Text PDFUltrathin metal films (UTMFs) are used in a wide range of applications, from transparent electrodes to infrared mirrors and metasurfaces. Due to their small thickness (5 nm), the electrical and optical properties of UTMFs can be changed by external stimuli, for example, by applying an electric field through an ion gel. It is also known that oxidized thin films and nanostructures of Au can be reduced by irradiating with short-wavelength light.
View Article and Find Full Text PDFQuantum resources can provide supersensitive performance in optical imaging. Detecting entangled photon pairs from spontaneous parametric down conversion (SPDC) with single-photon avalanche diode (SPAD) image sensor arrays (ISAs) enables practical wide-field quantum-enhanced imaging. However, matching the SPDC wavelength to the peak detection efficiency range of complementary metal-oxide-semiconductor (CMOS) compatible mass-producible SPAD-ISAs has remained technologically elusive, resulting in low imaging speeds to date.
View Article and Find Full Text PDFWe report a directly modulated distributed feedback laser operating in gain-switching mode for preparing the coherent states required for the Gaussian-modulated coherent-state (GMCS) continuous-variable quantum key distribution (CV-QKD) protocol. The proposed single-component quantum transmitter design eliminates the need for external modulators, decreasing the complexity of GMCS CV-QKD systems. The experimental results demonstrate a potential asymptotic secret key rate value of 2.
View Article and Find Full Text PDFACS Appl Nano Mater
December 2022
The increasing global use of cooling systems and the need of reducing greenhouse effect are pushing the emergence of more efficient cooling methods. In particular, passive radiative cooling technology extracts heat from objects by tailoring their optical emissivity using surface micro- and nanostructuring. Being capable of increasing thermal emissivity is especially relevant for widespread glass structures and devices, e.
View Article and Find Full Text PDFPhotosynthesis is a fundamental process that converts photons into chemical energy, driven by large protein complexes at the thylakoid membranes of plants, cyanobacteria, and algae. In plants, water-soluble plastocyanin (Pc) is responsible for shuttling electrons between cytochrome complex and the photosystem I (PSI) complex in the photosynthetic electron transport chain (PETC). For an efficient turnover, a transient complex must form between PSI and Pc in the PETC, which implies a balance between specificity and binding strength.
View Article and Find Full Text PDFCurrent diagnostics of severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) infection heavily rely on reverse transcription-polymerase chain reaction (RT-PCR) or on rapid antigen detection tests. The former suffers from long time-to-result and high cost while the latter from poor sensitivity. Therefore, it is crucial to develop rapid, sensitive, robust, and inexpensive methods for SARS-CoV-2 testing.
View Article and Find Full Text PDFQuantum techniques can be used to enhance the signal-to-noise ratio in optical imaging. Leveraging the latest advances in single-photon avalanche diode array cameras and multiphoton detection techniques, here, we introduce a supersensitive phase imager, which uses space-polarization hyperentanglement to operate over a large field of view without the need of scanning operation. We show quantum-enhanced imaging of birefringent and nonbirefringent phase samples over large areas, with sensitivity improvements over equivalent classical measurements carried out with equal number of photons.
View Article and Find Full Text PDFRecently, the European Commission supported by many European countries has announced large investments towards the commercialization of quantum technology (QT) to address and mitigate some of the biggest challenges facing today's digital era - e.g. secure communication and computing power.
View Article and Find Full Text PDFACS Appl Mater Interfaces
October 2021
Ultrathin metal films (UTMFs) are widely used in optoelectronic applications, from transparent conductors to photovoltaic cells, low emissivity windows, and plasmonic metasurfaces. During the initial deposition phase, many metals tend to form islands on the receiving substrate rather than a physically connected (percolated) network, which eventually evolves into continuous films as the thickness increases. For example, in the case of Ag and Au on dielectric surfaces, percolation begins when the thickness of the metal film is at least about 5 nm.
View Article and Find Full Text PDFWe present a versatile transmitter capable of performing both discrete variable and continuous variable quantum key distribution protocols (DV-QKD and CV-QKD, respectively). Using this transmitter, we implement a time-bin encoded BB84 DV-QKD protocol over a physical quantum channel of 47 km and a GG02 CV-QKD protocol with true local oscillator over a 10.5 km channel, achieving secret key rates of 4.
View Article and Find Full Text PDFSpider mites constitute an assemblage of well-known pests in agriculture, but are less known for their ability to spin silk of nanoscale diameters and high Young's moduli. Here, we characterize silk of the gorse spider mite Tetranychus lintearius, which produces copious amounts of silk with nano-dimensions. We determined biophysical characteristics of the silk fibres and manufactured nanoparticles and biofilm derived from native silk.
View Article and Find Full Text PDFWe report a plug-and-play continuous variable quantum key distribution system (CV-QKD) with Gaussian modulated quadratures and a true local oscillator. The proposed configuration avoids the need for frequency locking two narrow line-width lasers. To minimize Rayleigh back-scattering, we utilize two independent fiber strands for the distribution of the laser and the transmission of the quantum signals.
View Article and Find Full Text PDFUltrathin materials often require high temperatures for growth and processing, which cannot be withstood by the substrate underneath. For example, polymers are widely used as a supporting layer but unfortunately have low strain-point temperatures. This is the case of polyethylene terephthalate (PET) which has glass transition and melting temperatures of 76 and 250 °C, respectively.
View Article and Find Full Text PDFWith the alarming rise of antimicrobial resistance, studies on bacteria-surface interactions are both relevant and timely. Scanning electron microscopy and colony forming unit counting are commonly used techniques but require sophisticated sample preparation and long incubation time. Here, we present a direct method based on molecular dynamics simulation of nanostructured surfaces providing in silico predictions, complemented with time-lapse fluorescence imaging to study live interactions of bacteria at the membrane-substrate level.
View Article and Find Full Text PDFLight scattering is a fundamental property that can be exploited to create essential devices such as particle analysers. The most common particle size analyser relies on measuring the angle-dependent diffracted light from a sample illuminated by a laser beam. Compared to other non-light-based counterparts, such a laser diffraction scheme offers precision, but it does so at the expense of size, complexity and cost.
View Article and Find Full Text PDFHighly transparent optical surfaces with antireflection (AR) properties have the potential to increase the performance of a wide range of applications, such as windows for photovoltaic cells, photodetectors, and display screens among others. Biomimetic structures inspired by the moth-eye have attracted much attention as they can offer superior AR properties, which can generate broadband, omnidirectional optical transmission, and water-repellent self-cleaning behavior. However, many biomimetic surfaces suffer from time-consuming and complex processing, for example, electron beam and nanoimprint lithography, and/or sub-optimal mechanical reliability.
View Article and Find Full Text PDF[This corrects the article on p. 2101 in vol. 10, PMID: 31061773.
View Article and Find Full Text PDFSepsis is a condition characterized by a severe stage of blood-infection often leading to tissue damage, organ failure and finally death. Fast diagnosis and identification of the sepsis stage (sepsis, severe sepsis or septic shock) is critical for the patient's evolution and could help in defining the most adequate treatment in order to reduce its mortality. The combined detection of several biomarkers in a timely, specific and simultaneous way could ensure a more accurate diagnosis.
View Article and Find Full Text PDFMonitoring the early onset of bacterial film formation is critical in many clinical, environmental, and food quality control applications. We built a small inexpensive optical surface cytometer, in contrast with bulk spectroscopic methods, around a light-emitting diode (LED) and a complementary metal-oxide-semiconductor (CMOS) image sensor. It is designed to offer a large field-of-view of 200 mm and a large depth-of-field of 2-3 mm to overcome the limitations of routine methods like spectrophotometry and fluorescence microscopy.
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