Structural and vibrational properties of lanthanide Lindqvist polyoxometalate complexes.

Molecular spin qubits have demonstrated immense potential in quantum information science research due to the addressability of electron spins using microwave frequencies, and the scalability and tunability of molecular systems. Exemplary in this regard is the holmium polyoxometalate, [NaHo(WO)]·35HO (HoW), which features an accessible atomic clock transition at 9.4 GHz; however, the coherence time of this molecule is limited by spin-phonon coupling driven decoherence processes.