Strain superlattices (SL) in 2D materials like graphene provide an ideal test bed for generating flat bands and exploring the effects of strong correlations. Here we report STM/STS measurements on an engineered SL generated by placing graphene on a periodic array of silica nanospheres. A pseudomagnetic field as high as 55 T is observed along with the formation of pseudo-Landau levels (pLLs), not only at the expected integer values but also at fractional values.
View Article and Find Full Text PDFFermi liquids respond differently to perturbations depending on whether their frequency is higher (collisionless regime) or lower (hydrodynamic regime) than the interparticle collision rate. This results in a different phase velocity between the collisionless zero sound and the hydrodynamic first sound. We performed terahertz photocurrent nanoscopy measurements on graphene devices, with a metallic gate close to the graphene layer, to probe the dispersion of propagating acoustic plasmons, the counterpart of sound modes in electronic Fermi liquids.
View Article and Find Full Text PDFTo realize the applicative potential of 2D twistronic devices, scalable synthesis and assembly techniques need to meet stringent requirements in terms of interface cleanness and twist-angle homogeneity. Here, we show that small-angle twisted bilayer graphene assembled from separated CVD-grown graphene single-crystals can ensure high-quality transport properties, determined by a device-scale-uniform moiré potential. Via low-temperature dual-gated magnetotransport, we demonstrate the hallmarks of a 2.
View Article and Find Full Text PDFThe ability to tune the optical response of a material via electrostatic gating is crucial for optoelectronic applications, such as electro-optic modulators, saturable absorbers, optical limiters, photodetectors, and transparent electrodes. The band structure of single layer graphene (SLG), with zero-gap, linearly dispersive conduction and valence bands, enables an easy control of the Fermi energy, , and of the threshold for interband optical absorption. Here, we report the tunability of the SLG nonequilibrium optical response in the near-infrared (1000-1700 nm/0.
View Article and Find Full Text PDFThe exactly solvable Sachdev-Ye-Kitaev (SYK) model has recently received considerable attention in both condensed matter and high energy physics because it describes quantum matter without quasiparticles, while being at the same time the holographic dual of a quantum black hole. In this Letter, we examine SYK-based charging protocols of quantum batteries with N quantum cells. Extensive numerical calculations based on exact diagonalization for N up to 16 strongly suggest that the optimal charging power of our SYK quantum batteries displays a superextensive scaling with N that stems from genuine quantum mechanical effects.
View Article and Find Full Text PDFJ Phys Chem Lett
September 2020
We demonstrate that the plasmonic properties of realistic graphene and graphene-based materials can effectively and accurately be modeled by a novel, fully atomistic, yet classical, approach, named ωFQ. Such a model is able to reproduce all plasmonic features of these materials and their dependence on shape, dimension, and fundamental physical parameters (Fermi energy, relaxation time, and two-dimensional electron density). Remarkably, ωFQ is able to accurately reproduce experimental data for realistic structures of hundreds of nanometers (∼370k atoms), which cannot be afforded by any method.
View Article and Find Full Text PDFAn amendment to this paper has been published and can be accessed via a link at the top of the paper.
View Article and Find Full Text PDFAn amendment to this paper has been published and can be accessed via a link at the top of the paper.
View Article and Find Full Text PDFElectron-electron interactions play a critical role in many condensed matter phenomena, and it is tempting to find a way to control them by changing the interactions' strength. One possible approach is to place a studied system in proximity of a metal, which induces additional screening and hence suppresses electron interactions. Here, using devices with atomically-thin gate dielectrics and atomically-flat metallic gates, we measure the electron-electron scattering length in graphene and report qualitative deviations from the standard behavior.
View Article and Find Full Text PDFMetamaterials have recently established a new paradigm for enhanced light absorption in state-of-the-art photodetectors. Here, we demonstrate broadband, highly efficient, polarization-insensitive, and gate-tunable photodetection at room temperature in a novel metadevice based on gold/graphene Sierpinski carpet plasmonic fractals. We observed an unprecedented internal quantum efficiency up to 100% from the near-infrared to the visible range with an upper bound of optical detectivity of 10 Jones and a gain up to 10, which is a fingerprint of multiple hot carriers photogenerated in graphene.
View Article and Find Full Text PDFMagnons in ferromagnets behave as a viscous fluid over a length scale, the momentum-relaxation length, below which momentum-conserving scattering processes dominate. We show theoretically that in this hydrodynamic regime viscous effects lead to a sign change in the magnon chemical potential, which can be detected as a sign change in the nonlocal resistance measured in spin transport experiments. This sign change is observable when the injector-detector distance becomes comparable to the momentum-relaxation length.
View Article and Find Full Text PDFDespite topological protection and the absence of magnetic impurities, two-dimensional topological insulators display quantized conductance only in surprisingly short channels, which can be as short as 100 nm for atomically thin materials. We show that the combined action of short-range nonmagnetic impurities located near the edges and on site electron-electron interactions effectively creates noncollinear magnetic scatterers, and, hence, results in strong backscattering. The mechanism causes deviations from quantization even at zero temperature and for a modest strength of electron-electron interactions.
View Article and Find Full Text PDFAn electrical conductor subjected to a magnetic field exhibits the Hall effect in the presence of current flow. Here, we report a qualitative deviation from the standard behavior in electron systems with high viscosity. We found that the viscous electron fluid in graphene responds to nonquantizing magnetic fields by producing an electric field opposite to that generated by the ordinary Hall effect.
View Article and Find Full Text PDFWe investigate a quantum battery made of N two-level systems, which is charged by an optical mode via an energy-conserving interaction. We quantify the fraction of energy stored in the battery that can be extracted in order to perform thermodynamic work. We first demonstrate that this quantity is highly reduced by the presence of correlations between the charger and the battery or between the subsystems composing the battery.
View Article and Find Full Text PDFBased on extensive numerical simulations, accounting for electrostatic interactions and dissipative electron-phonon scattering, we propose experimentally realizable geometries capable of sustaining electronic preturbulence in graphene samples. In particular, preturbulence is predicted to occur at experimentally attainable values of the Reynolds number between 10 and 50, over a broad spectrum of frequencies between 10 and 100 GHz.
View Article and Find Full Text PDFPlasmons, collective oscillations of electron systems, can efficiently couple light and electric current, and thus can be used to create sub-wavelength photodetectors, radiation mixers, and on-chip spectrometers. Despite considerable effort, it has proven challenging to implement plasmonic devices operating at terahertz frequencies. The material capable to meet this challenge is graphene as it supports long-lived electrically tunable plasmons.
View Article and Find Full Text PDFFor many of the envisioned optoelectronic applications of graphene, it is crucial to understand the subpicosecond carrier dynamics immediately following photoexcitation and the effect of photoexcitation on the electrical conductivity-the photoconductivity. Whereas these topics have been studied using various ultrafast experiments and theoretical approaches, controversial and incomplete explanations concerning the sign of the photoconductivity, the occurrence and significance of the creation of additional electron-hole pairs, and, in particular, how the relevant processes depend on Fermi energy have been put forward. We present a unified and intuitive physical picture of the ultrafast carrier dynamics and the photoconductivity, combining optical pump-terahertz probe measurements on a gate-tunable graphene device, with numerical calculations using the Boltzmann equation.
View Article and Find Full Text PDFGraphene is known to possess strong optical nonlinearity which turned out to be suitable for creation of efficient saturable absorbers in mode locked fiber lasers. Nonlinear response of graphene can be further enhanced by the presence of graphene plasmons. Here, we report a novel nonlinear effect observed in nanostructured graphene which comes about due to excitation of graphene plasmons.
View Article and Find Full Text PDFVan der Waals heterostructures have emerged as promising building blocks that offer access to new physics, novel device functionalities and superior electrical and optoelectronic properties . Applications such as thermal management, photodetection, light emission, data communication, high-speed electronics and light harvesting require a thorough understanding of (nanoscale) heat flow. Here, using time-resolved photocurrent measurements, we identify an efficient out-of-plane energy transfer channel, where charge carriers in graphene couple to hyperbolic phonon polaritons in the encapsulating layered material.
View Article and Find Full Text PDFNonlinear optical processes, such as harmonic generation, are of great interest for various applications, e.g., microscopy, therapy, and frequency conversion.
View Article and Find Full Text PDFThe response of electron systems to electrodynamic fields that change rapidly in space is endowed by unique features, including an exquisite spatial nonlocality. This can reveal much about the materials' electronic structure that is invisible in standard probes that use gradually varying fields. Here, we use graphene plasmons, propagating at extremely slow velocities close to the electron Fermi velocity, to probe the nonlocal response of the graphene electron liquid.
View Article and Find Full Text PDFRadiative heat transfer (RHT) between macroscopic bodies at separations that are much smaller than the thermal wavelength is ruled by evanescent electromagnetic modes and can be orders of magnitude more efficient than its far-field counterpart, which is described by the Stefan-Boltzmann law. In this Letter, we present a microscopic theory of RHT in van der Waals stacks comprising graphene and a natural hyperbolic material, i.e.
View Article and Find Full Text PDFAn energy gap can be opened in the spectrum of graphene reaching values as large as 0.2 eV in the case of bilayers. However, such gaps rarely lead to the highly insulating state expected at low temperatures.
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