Interaction between Compliant Surfaces: How Soft Surfaces Can Reduce Friction.

We describe how a long-range repulsive interaction can surreptitiously modify the effective geometry of approaching compliant surfaces, with significant consequences on friction. We investigated the behavior under shear and compression of mica surfaces coated with poly(-isopropylacrylamide) pNIPAM-based cationic microgels. We show that local surface deformations as small as a few nanometers must be considered to understand the response of such surfaces under compression and shear, in particular when the range of action of normal and friction forces are significantly different, as is often the case for macromolecular lubrication.

Compliant Surfaces under Shear: Elastohydrodynamic Lift Force.

In this work, we have investigated the behavior under shear and compression of mica surfaces coated with poly(-isopropylacrylamide) cationic microgels. We have observed the emergence of velocity dependent, shear-induced normal forces, which can be large enough to entrain a fluid film that separates the surfaces out of contact, driving the dynamic system from conditions of boundary to hydrodynamic lubrication. By implementing a feedback-loop control on the surface separation, we were able to quantify the magnitude of the lift force as a function of the surface separation and driving speed.