Publications by authors named "Pi K"

Cyanobacterial blooms are prevalent globally and present a significant threat to water security. Titanium salt coagulants have garnered considerable attention due to their superior coagulation properties and the absence of metal residue risks. This paper explored the influencing factors in the coagulation process of titanium xerogel coagulant (TXC), the alterations in cell activity during floc storage, and the release of cyanobacterial organic matters, thereby determining the application scope of TXC for cyanobacterial water treatment.

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Background: The degree of yellowing in tobacco leaves is an important indicator for determining the maturity and harvesting time of tobacco leaves. Decreasing chlorophyll levels helps speed up the ripening process of tobacco leaves for easier mechanical harvesting. Identifying and utilizing genes that regulate yellowing in tobacco leaves are crucial for developing tobacco varieties suitable for mechanized harvesting and understanding the molecular processes that control leaf color changes.

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The photothermal sensitivity of tobacco refers to the degree to which tobacco responds to changes in light and temperature conditions in its growth environment, which is crucial for determining the planting area of cultivars and improving tobacco yield and quality. In order to accurately and effectively evaluate the photothermal sensitivity of tobacco cultivars, this study selected five cultivars and their hybrid combinations with significant differences planted under different ecological conditions from 2021 to 2022 as materials. The experiment was conducted in two locations with significant differences in temperature and light.

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Background: Breast implants, including textured variants, have been widely used in aesthetic and reconstructive mammoplasty. However, the textured type, which is one of the shell texture types of breast implants, has been identified as a possible etiologic factor for lymphoma, specifically breast implant-associated anaplastic large cell lymphoma (BIA-ALCL). Identifying the shell texture type of the implant is critical to diagnosing BIA-ALCL.

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  • - The study explores the electroreduction of toxic chromium (Cr(VI)) in wastewater, where it transforms into less harmful chromium (Cr(III)) through precipitation on the cathode during electrochemical reactions.
  • - Common inorganic anions like nitrate, chloride, phosphate, and sulfate were found to influence this electroreduction process, with sulfate being the most effective at enhancing Cr(VI) reduction but impeding Cr(III) precipitation.
  • - Experimental results showed that the presence of sulfuric anions significantly boosted the reduction efficiency of Cr(VI) (up to 99.9%) at certain concentrations, while lower concentrations of nitrate led to higher total chromium removal (92.8%), highlighting the complex interactions in wastewater treatment
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Geogenic fluorine-contaminated groundwater (F >1 mg/L) prevails in cold Mollisol regions of the world. Seasonal variation of F concentration in groundwater likely renders multiple pathways of toxic-level F exposure, posing unrecognized health risk to many economically challenged communities. Herein, different types of samples within the groundwater-soil-crop-human hair network were collected from the Mollisol regions of northeastern China and assessed by joint approach of medical geochemical assay, hydrogeochemical modeling, and health risk indexation.

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  • This study explores nicotine heterosis in tobacco (Nicotiana tabacum L.), revealing that hybrid varieties can have different nicotine levels due to effective nicotine transport mechanisms.
  • It found a very strong positive correlation (0.98) between transport heterosis and nicotine heterosis in hybrids, with plant height and other physical traits enhancing nicotine transport capacity.
  • The research highlights that non-additive gene effects, especially over-dominant effects, play a critical role in nicotine transport and accumulation, providing insights for breeding strategies and nicotine production efficiency.
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  • Heterosis improves crop performance, particularly in tobacco, but the study of leaf vein ratios and their genetic impacts has been underexplored, leading to inefficiencies in resource use.
  • The research analyzed 12 hybrid combinations to investigate heterosis in leaf vein ratios, revealing that some hybrids, like the F hybrid (G70 × Qinggeng), demonstrated significant negative heterosis of up to -19.79% 80 days post-transplant.
  • A transcriptome analysis uncovered that 39.04% of differentially expressed genes showed dominant patterns, emphasizing the importance of gene expression dynamics in leaf vein ratio heterosis and linking these genes to key biological processes like hormone signaling and plant development.
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Biotransformation of arsenic (As) influences its speciation and mobility, obscuring mechanistic comprehension on spatiotemporal variation of As concentration in geogenic contaminated groundwater. In particular, unresolved processes underlying As redox disequilibrium in comparison to major redox couples discourage practical efforts to rehabilitate the As-contaminated groundwater. Here, quantitative metagenomic sequencing and ultrahigh-resolution mass spectrometry (FT-ICR-MS) were jointly applied to reveal the links between vertical distribution of As metabolic gene assemblages and that of free energy density of dissolved organic matter (DOM) in As-contaminated groundwater of Datong Basin.

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FHWSB as an integrated absorptive catalyst, based on Walnut shell biochar (WSB) via hydrochloric acid modification and ferrous chloride impregnation, was prepared, reacted with HO to generate active free radicals •OH and •O, which oxidized and degraded about 80% of micro-pollutant sulfamethoxazole (SMX) from water, effectively resolving micro-pollutants' removal being inefficient because of high toxicity, persistence, and bioaccumulation in existed methods. It was clarified the specific degradation pathways and mechanisms of SMX by FHWSB synergistic HO via characterization and analysis assisted DFT calculations. Furthermore, it was found that the toxicity of a series of intermediates produced by SMX degraded continued to decline, consistent with its direction of degradation via toxicological analysis.

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To better understand the impact of long-term irrigation practices on arsenic (As) accumulation in agricultural soils, 100 soil samples from depths of 0-20 cm were collected from the Datong basin, where the As-contaminated groundwater has been used for irrigation for several decades. Soil samples were analyzed for major elements, trace elements, and As, Fe speciation. Results reveal As content ranging from 4.

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  • Illite significantly influences arsenic transport in subsurface environments, yet understanding its adsorption mechanisms remains debated due to a lack of direct evidence.
  • The study utilized advanced techniques like transmission electron microscopy and X-ray absorption spectroscopy to demonstrate how As(III) and As(V) are adsorbed onto illite, revealing different adsorption capacities and kinetics for each species.
  • A new surface complexation model was created to describe the adsorption processes, highlighting the role of inner/outer-sphere complexation and the effects of cations and specific bonds in the mechanisms involved.
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Activated persulfate and hydrothermal treatment (HTT) are often employed to treat waste activated sludge, which can improve the efficiency of subsequent sludge treatment and change the distribution of pollutants in the sludge. However, the impact of sludge solid content and temperature on the occurrence and aging of microplastics (MPs) during HTT remains poorly understood. This study investigated the effects of persulfate-HTT (SPS-HTT) co-treatment on the migration, occurrence, and aging of MPs in sludge with different solid contents (2% and 5% solid content).

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Arsenic (As) is a groundwater contaminant of global concern. The degradation of dissolved organic matter (DOM) can provide a reducing environment for As release. However, the interaction of DOM with local microbial communities and how different sources and types of DOM influence the biotransformation of As in aquifers is uncertain.

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Background: Leaves are the nutritional and economic organs of tobacco, and their biomass directly affects tobacco yield and the economic benefits of farmers. In the early stage, our research found that tobacco hybrids have more leaves and larger leaf areas, but the performance and formation reasons of biomass heterosis are not yet clear.

Results: This study selected 5 parents with significant differences in tobacco biomass and paired them with hybrid varieties.

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Massive soil erosion occurs in the world's Mollisol regions due to land use change and climate warming. The migration of Mollisol organic matter to river systems and subsequent changes in carbon biogeochemical flow and greenhouse gas fluxes are of global importance but little understood. By employing comparative mesocosm experiments simulating varying erosion intensity in Mollisol regions of northeastern China, this research highlights that erosion-driven export and biomineralization of terrestrial organic matter facilitates CO and CH emission from receiving rivers.

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  • Mollisols, rich in organic matter, are crucial for storing carbon and selenium, but climate change and agriculture could lead to their loss, particularly through increased soil respiration in colder regions.
  • Experiments showed that even in winter, cultivated Mollisol soils emitted significant amounts of greenhouse gases and methylated selenium, with higher emissions from cultivated soils—around 7.45 g/m²/day for carbon and 1.42 µg/m²/day for selenium.
  • The study revealed that soil moisture influences greenhouse gas emissions, highlighting the link between organic carbon quality and selenium loss, which is vital for managing carbon and selenium resources in agriculture to prevent deficiencies.
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Organoiodine compounds (OICs) are the dominant iodine species in groundwater systems. However, molecular mechanisms underlying the geochemical formation of geogenic OICs-contaminated groundwater remain unclear. Based upon multitarget field monitoring in combination with ultrahigh-resolution molecular characterization of organic components for alluvial-lacustrine aquifers, we identified a total of 939 OICs in groundwater under reducing and circumneutral pH conditions.

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Eutrophication, the over-enrichment with nutrients, for example, nitrogen and phosphorus, of ponds, reservoirs and lakes, is an urgent water quality issue. The most notorious symptom of eutrophication is a massive proliferation of cyanobacteria, which cause aquatic organism death, impair ecosystem and harm human health. The method considered to be most effective to counteract eutrophication is to reduce external nutrient inputs.

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  • Pb soil pollution is a significant health risk, and the most common cleanup method is immobilization, which prevents heavy metals from moving in the soil.
  • A study used municipal sewage sludge to treat Pb-contaminated soils from a lead-acid battery factory, reducing leachable Pb levels significantly over time, with the addition of phosphate fertilizer further enhancing this effect.
  • The remediation process significantly decreased the bioavailability of Pb in plants, with results showing a reduction of Pb absorption in mung bean roots by 87%, attributed to changes in how Pb interacts with soil components during treatment.
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The environmental fate of arsenic (As) relies substantially on its speciation, which occurs frequently coupled to the redox transformation of manganese. While trivalent manganese (Mn(III)), which is known for its high reactivity, is believed to play a role in As mobilization by iron (oxyhydr)oxides in dynamic aquifers, the exact roles and underlying mechanisms are still poorly understood. Using increasingly complex batch experiments that mimick As-affected aquifer conditions in combination with time-resolved characterization, we demonstrate that Mn(III)-NOM complexes play a crucial role in the manganese-mediated immobilization of As(III) by ferrihydrite and goethite.

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Geogenic arsenic (As)-contaminated groundwater is a sustaining global health concern that is tightly constrained by multiple interrelated biogeochemical processes. However, a complete spectrum of the biogeochemical network of high-As groundwater remains to be established, concurrently neglecting systematic zonation of groundwater biogeochemistry on the regional scale. We uncovered the geomicrobial interaction network governing As biogeochemical pathways by merging in-field hydrogeochemical monitoring, metagenomic analyses, and ultrahigh resolution mass spectrometry (FT-ICR MS) characterization of dissolved organic matter.

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Cold stress is a non-biological stressor that adversely affects tobacco yield and leaf quality. Plant photoreceptor proteins, which function as dual light-temperature sensors, play a vital role in temperature changes, making them crucial for responses to non-biological stressors. However, the regulatory mechanisms of PhyA in tobacco remain poorly understood.

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Background: Glutathione S-transferases (GSTs) are large and multifunctional proteases that play an important role in detoxification, protection against biotic and abiotic stresses, and secondary metabolite transportation which is essential for plant growth and development. However, there is limited research on the identification and function of NtGSTs.

Results: This study uses K326 and other six tobacco varieties (Hongda, HG, GDH11, Va116, VG, and GDH88) as materials to conduct comprehensive genome-wide identification and functional characterization of the GST gene in tobacco.

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The potential for the presence of microplastics (MPs) in municipal solid waste incineration bottom ash (MSWI-BA) has not been fully explored. In this study, surfactant-assisted air flotation separation in aqueous media was used to examine the removal of MPs and other pollutants from different particle size fractions of MSWI-BA. The use of 1 mmol L sodium dodecylbenzene sulfonate (SDBS), at a liquid-solid ratio of 60:1, increased by 66 % the quantity of MPs floated from the MSWI-BA 0-0.

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