Monochromatization of Electron Beams with Spatially and Temporally Modulated Optical Fields.

Inelastic interaction between coherent light with constant frequency and free electrons enables periodic phase modulation of electron wave packets leading to periodic sidebands in the electron energy spectra. In this Letter, we propose a generalization of the interaction by considering linearly chirped electron wave packets interacting with chirped optical fields. We theoretically demonstrate that when matching the chirp parameters of the electron and light waves, the interaction leads to partial monochromatization of the electron spectra in one of the energy sidebands.

Ultrafast Dynamics of Valley-Polarized Excitons in WSe Monolayer Studied by Few-Cycle Laser Pulses.

We report on the experimental investigation of the ultrafast dynamics of valley-polarized excitons in monolayer WSe2 using transient reflection spectroscopy with few-cycle laser pulses with 7 fs duration. We observe that at room temperature, the anisotropic valley population of excitons decays on two different timescales. The shorter decay time of approximately 120 fs is related to the initial hot exciton relaxation related to the fast direct recombination of excitons from the radiative zone, while the slower picosecond dynamics corresponds to valley depolarization induced by Coloumb exchange-driven transitions of excitons between two inequivalent valleys.