Comparative anatomy is an important tool for investigating evolutionary relationships among species, but the lack of scalable imaging tools and stains for rapidly mapping the microscale anatomies of related species poses a major impediment to using comparative anatomy approaches for identifying evolutionary adaptations. We describe a method using synchrotron source micro-x-ray computed tomography (syn-μXCT) combined with machine learning algorithms for high-throughput imaging of Lepidoptera (i.e.
View Article and Find Full Text PDFComplex dynamical systems may exhibit multiple steady states, including time-periodic limit cycles, where the final trajectory depends on initial conditions. With tuning of parameters, limit cycles can proliferate or merge at an exceptional point. Here we ask how dynamics in the vicinity of such a bifurcation are influenced by noise.
View Article and Find Full Text PDFCubic energy materials such as thermoelectrics or hybrid perovskite materials are often understood to be highly disordered. In GeTe and related IV-VI compounds, this is thought to provide the low thermal conductivities needed for thermoelectric applications. Since conventional crystallography cannot distinguish between static disorder and atomic motions, we develop the energy-resolved variable-shutter pair distribution function technique.
View Article and Find Full Text PDFIn the context of a single-electron two orbital Holstein system coupled to dispersionless bosons, we develop a general method to correct the single-particle Green's function using a power series correction (PSC) scheme. We outline the derivations of various flavors of cumulant approximation through the PSC scheme explaining the assumptions and approximations behind them. Finally, we compare the PSC spectral function with cumulant and exact diagonalized spectral functions and elucidate three regimes of this problem-two where the cumulant explains and one where the cumulant fails.
View Article and Find Full Text PDFThe COVID-19 pandemic has brought attention to the need for developing effective respiratory support that can be rapidly implemented during critical surge capacity scenarios in healthcare settings. Lung support with bubble continuous positive airway pressure (B-CPAP) is a well-established therapeutic approach for supporting neonatal patients. However, the effectiveness of B-CPAP in larger pediatric and adult patients has not been addressed.
View Article and Find Full Text PDFA detailed exploration of the-atomic orbital occupancy space for UOis performed using a first principles approach based on density functional theory (DFT), employing a full hybrid functional within a systematic basis set. Specifically, the PBE0 functional is combined with an occupancy biasing scheme implemented in a wavelet-based algorithm which is adapted to large supercells. The results are compared with previous DFT +calculations reported in the literature, while dynamical mean field theory is also performed to provide a further base for comparison.
View Article and Find Full Text PDFExcellent photovoltaic performance is predicted in a pentagonal covalent network of Si in a hollow structure exhibiting both thermal and dynamical stability. Consisting of a combination of sp and sp hybridized Si atomic orbitals, the GW0 computed band structure shows an indirect band gap near the zone edge and also a manifold of directly absorbing transitions at frequencies in the window of visible light, in distinction with conventional Si. Hydrogenation of a single sp site is predicted to lead to a robust local magnetic moment.
View Article and Find Full Text PDFOut of equilibrium, a lack of reciprocity is the rule rather than the exception. Non-reciprocity occurs, for instance, in active matter, non-equilibrium systems, networks of neurons, social groups with conformist and contrarian members, directional interface growth phenomena and metamaterials. Although wave propagation in non-reciprocal media has recently been closely studied, less is known about the consequences of non-reciprocity on the collective behaviour of many-body systems.
View Article and Find Full Text PDFLarge scientific projects in genomics and astronomy are influential not because they answer any single question but because they enable investigation of continuously arising new questions from the same data-rich sources. Advances in automated mapping of the brain's synaptic connections (connectomics) suggest that the complicated circuits underlying brain function are ripe for analysis. We discuss benefits of mapping a mouse brain at the level of synapses.
View Article and Find Full Text PDFWe propose a novel mechanism for a nonequilibrium phase transition in a U(1)-broken phase of an electron-hole-photon system, from a Bose-Einstein condensate of polaritons to a photon laser, induced by the non-Hermitian nature of the condensate. We show that a (uniform) steady state of the condensate can always be classified into two types, namely, arising either from lower or upper-branch polaritons. We prove (for a general model) and demonstrate (for a particular model of polaritons) that an exceptional point where the two types coalesce marks the end point of a first-order-like phase boundary between the two types, similar to a critical point in a liquid-gas phase transition.
View Article and Find Full Text PDFWe predict the existence and dynamical stability of heptagraphene, a new graphitic structure formed of rings of 10 carbon atoms bridged by carbene groups yielding seven-membered rings. Despite the rectangular unit cell, the band structure is topologically equivalent to that of strongly distorted graphene. Density-functional-theory calculations demonstrate that heptagraphene has Dirac cones on symmetry lines that are robust against biaxial strain but which open a gap under shear.
View Article and Find Full Text PDFThe elastic response of suspended NbSe(3) nanowires is studied across the charge density wave phase transition. The nanoscale dimensions of the resonator lead to a large resonant frequency (~10-100 MHz), bringing the excited phonon frequency in close proximity of the plasmon mode of the electronic condensate-a parameter window not accessible in bulk systems. The interaction between the phonon and plasmon modes strongly modifies the elastic properties at high frequencies.
View Article and Find Full Text PDFWe propose a mechanism for binding of diatomic ligands to heme based on a dynamical orbital selection process. This scenario may be described as bonding determined by local valence fluctuations. We support this model using linear-scaling first-principles calculations, in combination with dynamical mean-field theory, applied to heme, the kernel of the hemoglobin metalloprotein central to human respiration.
View Article and Find Full Text PDFVanadium dioxide undergoes a first order metal-insulator transition at 340 K. In this Letter, we develop and carry out state-of-the-art linear scaling density-functional theory calculations refined with nonlocal dynamical mean-field theory. We identify a complex mechanism, a Peierls-assisted orbital selection Mott instability, which is responsible for the insulating M(1) phase, and which furthermore survives a moderate degree of disorder.
View Article and Find Full Text PDFWe create a large exciton-polariton condensate and employ a Michelson interferometer setup to characterize the short- and long-distance behavior of the first order spatial correlation function. Our experimental results show distinct features of both the two-dimensional and nonequilibrium characters of the condensate. We find that the gaussian short-distance decay is followed by a power-law decay at longer distances, as expected for a two-dimensional condensate.
View Article and Find Full Text PDFLocal electrochemical phenomena on the surfaces of the LaAlO(3)-SrTiO(3) heterostructure are explored using unipolar and bipolar dynamic electrochemical strain microscopy (D-ESM). The D-ESM suggests the presence of at least two distinct electrochemical processes, including fast reversible low-voltage process and slow high-voltage process. The latter process is associated with static surface deformations in the sub-nanometer regime.
View Article and Find Full Text PDFCeCoIn5 is an anomalous superconductor which exhibits a high-magnetic-field phase that consists of a modulated magnetic coupling together with persistent superconducting order. Here we use a generic microscopic model to argue that this state is a pattern of coexisting condensates: a d-wave singlet superconducting (SC) state, a staggered π-triplet SC state, and a spin density wave (SDW). Our microscopic picture allows a calculation of the phase diagram, and physical consequences including NMR.
View Article and Find Full Text PDFThe dielectric response in a magnetic field is routinely used to probe the existence of coupled magnetic and elastic order in the multiferroics. However, here we demonstrate that magnetism is not necessary to produce a magnetocapacitance when the material is inhomogeneous. By considering a two-dimensional, two-component composite medium, we find a characteristic dielectric resonance that depends on magnetic field.
View Article and Find Full Text PDFThe superfluid to Mott insulator transition in cavity polariton arrays is analyzed using the variational cluster approach, taking into account quantum fluctuations exactly on finite length scales. Phase diagrams in one and two dimensions exhibit important non-mean-field features. Single-particle excitation spectra in the Mott phase are dominated by particle and hole bands separated by a Mott gap.
View Article and Find Full Text PDFRecent years have witnessed novel and exciting advances on the subject of optical coherence and collective phenomena in nanostructures. This volume overviews the forefront progress in this area, collecting nine reviews and ten new contributions by leading experts in the field. The subfields included in this volume span from two-dimensional electron gases, semiconductor excitons, coupled quantum wells, microcavity polaritons, quantum dots and quantum wires.
View Article and Find Full Text PDFSpin electronics (spintronics) exploits the magnetic nature of electrons, and this principle is commercially applied in, for example, the spin valves of disk-drive read heads. There is currently widespread interest in developing new types of spintronic devices based on industrially relevant semiconductors, in which a spin-polarized current flows through a lateral channel between a spin-polarized source and drain. However, the transformation of spin information into large electrical signals is limited by spin relaxation, so that the magnetoresistive signals are below 1% (ref.
View Article and Find Full Text PDFWe propose a new method of detecting the onset of superfluidity in a two-component ultracold fermionic gas of atoms governed by an attractive short-range interaction. By studying the two-body correlation functions we find that a measurement of the momentum distribution of the density and spin-response functions allows one to access separately the normal and anomalous densities. The change in sign at low momentum transfer of the normal-ordered part of the density response function signals the transition between a BEC and a BCS regime, characterized by small and large pairs, respectively.
View Article and Find Full Text PDFBilayer electron-hole systems, where the electrons and holes are created via doping and are confined to separate layers, undergo excitonic condensation when the distance between the layers is smaller than the typical distance between the particles within the layer. We argue that the excitonic condensate is a novel dipolar superfluid in which the phase of the condensate couples to the gradient of the vector potential. We predict the existence of a dipolar supercurrent which can be tuned by an in-plane magnetic field.
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