We report gamma ray spectroscopy measurements of trinitite samples and analogous samples obtained from detonation sites in Nevada and Semipalatinsk, as well as measurements of topsoil at the Trinity site. We also report the first isotopic composition measurements of trinitite using the novel forensics technique of decay energy spectroscopy (DES) as a complement to traditional forensics techniques. Our gamma spectroscopy and DES measurements are compared to other published results.
View Article and Find Full Text PDFIn this paper, we present a new method to study global atmospheric processes and their changes during the last decade. A cosmogenic radionuclide measured at ground-level, beryllium-7, is utilized as a proxy to study atmospheric dynamics. Beryllium-7 has two advantages: First, this radionuclide, primarily created in the lower stratosphere, attaches to aerosols that are transported downwards to the troposphere and travel around the globe with the general atmospheric circulation.
View Article and Find Full Text PDFJ Radioanal Nucl Chem
September 2015
The impact of Chernobyl on the Cs activities found in wild boars in Europe, even in remote locations from the NPP, has been much greater than the impact of Fukushima on boars in Japan. Although there is great variability within the Cs concentrations throughout the wild boar populations, some boars in southern Germany in recent years exhibit higher activity concentrations (up to 10,000 Bq/kg and higher) than the highest Cs levels found in boars in the governmental food monitoring campaign (7900 Bq/kg) in Fukushima prefecture in Japan. The levels of radiocesium in boar appear to be more persistent than would be indicated by the constantly decreasing Cs inventory observed in the soil which points to a food source that is highly retentive to Cs contamination or to other radioecological anomalies that are not yet fully understood.
View Article and Find Full Text PDFBeryllium-7 ((7)Be) daily data from the four International Monitoring System (IMS) radionuclide particulate stations on mainland Australia are analysed over the period 2001 to 2011. The analysis indicates that levels of (7)Be in surface air at the stations follow annual cycles, with yearly peak activity concentrations occurring later at stations further south. The yearly peak migrates north-south at a rate of approximately 4.
View Article and Find Full Text PDFFission gases such as (133)Xe are used extensively for monitoring the world for signs of nuclear testing in systems such as the International Monitoring System (IMS). These gases are also produced by nuclear reactors and by fission production of (99)Mo for medical use. Recently, medical isotope production facilities have been identified as the major contributor to the background of radioactive xenon isotopes (radioxenon) in the atmosphere (Stocki et al.
View Article and Find Full Text PDFMedical isotope production facilities (MIPF) have recently been identified to emit the major part of the environmental radioxenon measured at many globally distributed monitoring sites deployed to strengthen the radionuclide component of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) verification regime. Efforts to raise a global radioxenon emission inventory revealed that the yearly global total emission from MIPF's is around 15 times higher than the total radioxenon emission from nuclear power plants (NPP's). Given that situation, from mid 2008 until early 2009 two out of the ordinary hemisphere-specific events occured: 1) In the Northern hemisphere, a joint temporary suspension of operations of the three largest MIPF's made it possible to quantify the effects of the emissions related to NPP's.
View Article and Find Full Text PDFRadioxenon isotopes play a major role in confirming whether or not an underground explosion was nuclear in nature. It is then of key importance to understand the sources of environmental radioxenon to be able to distinguish civil sources from those of a nuclear explosion. Based on several years of measurements, combined with advanced atmospheric transport model results, it was recently shown that the main source of radioxenon observations are strong and regular batch releases from a very limited number of medical isotope production facilities.
View Article and Find Full Text PDFThe origin of a series of atmospheric radioxenon events detected at the Comprehensive Test Ban Treaty Organisation (CTBTO) International Monitoring System site in Melbourne, Australia, between November 2008 and February 2009 was investigated. Backward tracking analyses indicated that the events were consistent with releases associated with hot commission testing of the Australian Nuclear Science Technology Organisation (ANSTO) radiopharmaceutical production facility in Sydney, Australia. Forward dispersion analyses were used to estimate release magnitudes and transport times.
View Article and Find Full Text PDFJ Environ Radioact
May 2009
Radioxenon isotopes play a major role in confirming whether or not an underground explosion was nuclear in nature. It is then of key importance to understand the sources of environmental radioxenon to be able to distinguish them from those of a nuclear explosion. Nuclear power plants were long thought to be the main emitters of these noble gases.
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