This study focuses on the chemical composition of cloud water (CW) and rainwater (RW) collected at Sinhagad, a high-altitude station (1450 m AMSL) located in the western region of India. The samples were collected during the monsoon over two years (2016-2017). The chemical analysis suggests that the concentration of total ionic constituents was three times higher in CW than in RW, except for NH (1.
View Article and Find Full Text PDFAerosol-CCN characteristics and dynamics during a pre-monsoon dust storm (April 6-11, 2015) over a high-altitude site ((17.92°N, 73.66°E, and 1348 m above mean sea level (MSL)) in Western Ghats, India, has been studied using ground-based observations, satellite, and reanalysis datasets.
View Article and Find Full Text PDFThe elevated aerosol layer (EAL) plays a vital role in weather and climate by modifying the Earth's radiation budget. In the present study, the EAL occurrence and its characteristics in the pre-monsoon season using micropulse lidar (MPL) observations during 2016-2018 and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) during 2007-2018 over Kattankulathur is being reported. We have collected 147 days (101 cases) of MPL (CALIPSO) observations during clear sky conditions in the pre-monsoon 2016-2018 (2007-2018), out of which EAL is observed for 56 days (61 cases).
View Article and Find Full Text PDFSecond-generation bioenergy, a carbon neutral or negative renewable resource, is crucial to achieving India's net-zero emission targets. Crop residues are being targeted as a bioenergy resource as they are otherwise burned on-field, leading to significant pollutant emissions. But estimating their bioenergy potential is problematic because of broad assumptions about their surplus fractions.
View Article and Find Full Text PDFHygroscopicity of atmospheric aerosol primarily depends on the size and chemical composition of the particle and is important for estimating anthropogenic aerosol radiative forcing. There is limited information exists over the Indian region on size segregated aerosol hygroscopicity (κ) in different seasons. This study presents 'κ' as derived from a Humidified Tandem Differential Mobility Analyzer (HTDMA) over a High Altitude Cloud Physics Laboratory (HACPL) in the Western Ghats, India for more than a year (from May 2019 to May 2020).
View Article and Find Full Text PDFThe characteristics of black carbon (BC) aerosols, their sources, and their impact on atmospheric radiative forcing were extensively studied during the COVID-19 lockdown (28th March-31st May 2020) at a high-altitude rural site over the Western Ghats in southwest India. BC concentration and the contribution of BC originating from biomass burning (BC) estimated from the aethalometer model during the lockdown period were compared with the same periods in 2017 and 2018 and with the pre-lockdown period (1st February to March 20, 2020). BC concentrations were 44, 19, and 17% lower during the lockdown period compared with the pre-lockdown periods of 2020 and similar periods (28th March to 31st May) of 2017 and 2018, respectively.
View Article and Find Full Text PDFTropospheric Biennial Oscillation (TBO) is characterized by a tendency for a relatively stronger monsoon to be followed by a relatively weaker one (positive) or vice-versa (negative). This study examines the distribution of different convective systems occurring during TBO phases over the Indian monsoon region. During negative TBO phase, convection is preferential over the Arabian Sea (AS), whereas during positive TBO phase, it is favoured over the land areas and Bay of Bengal (BoB).
View Article and Find Full Text PDFDiurnal variation of convective storms (CSs) during monsoon season and associated physical mechanisms are significantly important for accurate forecast of short-time and extreme precipitation. The diurnal cycle of CSs is investigated using ground-based X-band radar, Tropical Rainfall Measuring Mission Precipitation Radar, and reanalysis data during the summer monsoon (June-September of 2014) over complex mountain terrain of Western Ghats, India. Diurnally, CSs show a bimodal distribution in the coastal areas, but this bimodality became weak along the upslope regions and on the mountain top.
View Article and Find Full Text PDFThe temporal variability of the planetary boundary layer height (PBLH) over Mahabaleshwar was studied for a period of 1 year from 1 December 2015 to 30 November 2016 using microwave radiometer (MWR) observations. The PBLH over Mahabaleshwar was found to be the highest during the pre-monsoon (March-May) season and lowest during the winter (December-February) season. The seasonal mean of PBLH was estimated to be 339±88 m during winter, 485±70 m during pre-monsoon, 99±153 m during monsoon, and 438±24 m during post-monsoon season.
View Article and Find Full Text PDFThe effect of relative humidity and temperature on the submicron aerosol variability and its ageing process was studied over a high altitude site, Mahabaleshwar in south-west India. The mass composition of non-refractory particulate matter of 1 μm (NR-PM) size was obtained using Time of Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) along with the measurements on a few trace gases during winter (December 2017-February 2018) and summer season (20th March - 5th May 2018). Sulfate exhibited strong dependence on the relative humidity (RH) as its mass fraction increased with the increase in RH.
View Article and Find Full Text PDFAssessment of Sea Salt (SS) and Non-Sea Salt (NSS) aerosols in rainwater is important to understand the characterization of marine and continental aerosols and their source pathways. Sea salt quantification based on standard seawater ratios are primarily constrained with high uncertainty with its own limitations. Here, by the novelty of k-mean clustering and Positive Matrix Factorization (PMF) analysis, we segregate the air masses into two distinct clusters (oceanic and continental) during summer monsoon period signifying the complex intermingle of sources that act concomitantly.
View Article and Find Full Text PDFThis study presents the characteristics of black carbon aerosol (BC) over a high-altitude site, Mahabaleshwar during the monsoon season. The mass concentration of BC exhibits a morning peak and a daytime build-up with a mean mass concentration of 303 ± 142 ng m. The simultaneous measurements of aerosol particle number concentration (PNC), cloud condensation nuclei concentration (CCN), and non-refractory particulate matter less than 1 μm size (NR-PM) were also made by using a Wide-Range Aerosol Spectrometer (WRAS), CCN counter and Aerosol Chemical Speciation Monitor (ACSM) respectively.
View Article and Find Full Text PDFTo understand the boundary layer characteristics and pathways of aerosol-cloud interaction, an Integrated Ground Observational Campaign, concurrent with Cloud Aerosol Interaction and Precipitation Enhancement Experiment, was conducted by the Indian Institute of Tropical Meteorology, Pune, under Ministry of Earth Sciences at Mahabubnagar (a rural environment, which is ~100 km away from an urban city Hyderabad in Andhra Pradesh), during the period of July-November 2011. Collected samples of PM2.5 and PM10 were analyzed for water-soluble ionic species along with organic carbon (OC) and elemental carbon (EC).
View Article and Find Full Text PDFA comprehensive measurement program of effective black carbon (eBC), fine particle (PM2.5), and carbon monoxide (CO) was undertaken during 1 December 2011 to 31 March 2012 (winter period) in Delhi, India. The mean mass concentrations of eBC, PM2.
View Article and Find Full Text PDFThe scattering properties of aerosols over a tropical urban station, Pune, India, (18° 32' N, 73° 51' E, 559 m above mean sea level), are studied with a bistatic, multiwavelength, continuous-wave, argon-ion lidar. The scattered-intensity profiles (up to 1000 m above ground level) measured at four wavelengths (0.4765, 0.
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