Monolayer 2D ZrTe transition metal dichalcogenide as nanoscatter for random laser action.

We demonstrate random laser emission from Rhodamine 6G with ZrTe2 transition metal dichalcogenide (TMD) as nanoscatters, both in powder and 2D nanoflakes liquid suspension. The 2D semimetal ZrTe2 was synthesized by a modified redox exfoliation method to provide single layer TMD, which was employed for the first time as the scatter medium to provide feedback in an organic gain medium random laser. In order to exploit random laser emission and its threshold value, replica symmetry breaking leading to a photonic paramagnetic to photonic spin glass transition in both 2D and 3D (powder) ZrTe2 was demonstrated.

Nonlinear effects and photonic phase transitions in Nd-doped nanocrystal-based random lasers.

The interplay between gain and scattering of light propagating in disordered media allows operation of random lasers (RLs)-lasers without conventional optical cavities. In the present paper, we review our recent contributions in this area, which include the demonstration of self-second-harmonic and self-sum-frequency generation, the characterization of Lévy's statistics of the output intensity fluctuations, and replica symmetry breaking (analogue to the spin-glass phase transition) by RLs based on nanocrystals containing trivalent neodymium ions.

A random laser based on electrospun polymeric composite nanofibers with dual-size distribution.

Electrospun fiber-based random lasers are environment-friendly flexible systems in which waveguiding/scattering processes provided by their structure with a broad distribution of diameters are essential elements to generate a suitable lasing mechanism. In this work, we prepared electrospun fibers with dual-size diameter distribution (above and below the critical value for waveguiding), allowing that both optical processes can be established in the polymer network. As a result, random laser emission was observed for the electrospun fibers presenting dual-size diameters with rhodamine 6G as the gain medium, characterizing the combination of waveguiding/scattering as an adequate condition for development of organic nanofibrous random lasers.

Replica Symmetry Breaking in the Photonic Ferromagneticlike Spontaneous Mode-Locking Phase of a Multimode Nd:YAG Laser.

We demonstrate the replica symmetry breaking (RSB) phenomenon in the spontaneous mode-locking regime of a multimode Q-switched Nd:YAG laser. The underlying mechanism is quite distinct from that of the RSB recently observed in random lasers. Here, there is no random medium and the phase is not glassy with incoherently oscillating modes as in random lasers.

Turbulence hierarchy in a random fibre laser.

Turbulence is a challenging feature common to a wide range of complex phenomena. Random fibre lasers are a special class of lasers in which the feedback arises from multiple scattering in a one-dimensional disordered cavity-less medium. Here we report on statistical signatures of turbulence in the distribution of intensity fluctuations in a continuous-wave-pumped erbium-based random fibre laser, with random Bragg grating scatterers.

Observation of photonic paramagnetic to spin-glass transition in a specially designed TiO particle-based dye-colloidal random laser.

Colloidal-based random lasers (RLs) are highly efficient and have been exploited in a wide range of geometries. However, in the particular case of ethanol solutions of rhodamines and TiO particles, the RL behavior is quite unstable due to the fast precipitation of the particles. In this Letter, specially designed amorphous TiO particles were synthesized by a sol-gel method, preventing the degradation of the RL for long operating lifetimes of over 10 shots.

Observation of Lévy distribution and replica symmetry breaking in random lasers from a single set of measurements.

Random lasers have been recently exploited as a photonic platform for studies of complex systems. This cross-disciplinary approach opened up new important avenues for the understanding of random-laser behavior, including Lévy-type distributions of strong intensity fluctuations and phase transitions to a photonic spin-glass phase. In this work, we employ the Nd:YBO random laser system to unveil, from a single set of measurements, the physical origin of the complex correspondence between the Lévy fluctuation regime and the replica-symmetry-breaking transition to the spin-glass phase.

Tunable ultraviolet and blue light generation from Nd:YAB random laser bolstered by second-order nonlinear processes.

Ultraviolet and blue light were obtained by nonlinear frequency conversion in a random laser (RL) based on Nd0.10Y0.90Al3(BO3)4 nanocrystalline powder.