Proc Natl Acad Sci U S A
December 2022
In BaNiS, a Dirac nodal line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy (STM), we discover signs of correlated-electron behavior, namely electronic nematicity appearing as a pair of -symmetry striped patterns in the local density-of-states at ∼60 meV above the Fermi energy. In observations of quasiparticle interference, as well as identifying scattering between Dirac cones, we find that the striped patterns in real space stem from a lifting of degeneracy among electron pockets at the Brillouin zone boundary.
View Article and Find Full Text PDFExotic quantum phase transitions in metals, such as the electronic nematic state, have been discovered one after another and found to be universal now. The emergence of unconventional density-wave (DW) order in frustrated kagome metal AVSb and its interplay with exotic superconductivity attract increasing attention. We find that the DW in kagome metal is the bond order, because the sizable intersite attraction is caused by the quantum interference among paramagnons.
View Article and Find Full Text PDFIn the magic-angle twisted bilayer graphene (MATBG), one of the most remarkable observations is the C_{3}-symmetry-breaking nematic state. We identify that the nematicity in MATBG is the E-symmetry ferro bond order, which is the modulation of correlated hopping integrals owing to the E-symmetry particle-hole pairing condensation. The nematicity in MATBG originates from prominent quantum interference among SU(4) valley+spin composite fluctuations.
View Article and Find Full Text PDFNematicity is ubiquitous in the electronic phases of iron-based superconductors. The order parameter that characterizes the nematic phase has been investigated in momentum space, but its real-space arrangement remains largely unexplored. We use linear dichroism (LD) in a low-temperature laser–photoemission electron microscope to map out the nematic order parameter of nonmagentic FeSe and antiferromagnetic BaFe(AsP).
View Article and Find Full Text PDFWe examine electronic and crystal structures of iron-based superconductorsFeAsOH(= La, Sm) under pressure by means of x-ray absorption spectroscopy (XAS), x-ray emission spectroscopy (XES), and x-ray diffraction. In LaFeAsO the pre-edge peak on high-resolution XAS at the Fe-absorption edge gains in intensity on the application of pressure up to 5.7 GPa and it saturates in the higher pressure region.
View Article and Find Full Text PDFA carrier doping by a hydrogen substitution in LaFeAsOHis known to cause two superconducting (SC) domes with the magnetic order at both end sides of the doping. In contrast, SmFeAsOHhas a similar phase diagram but shows single SC dome. Here, we investigated the electronic and crystal structures for iron oxynitrideFeAsOH(= La, Sm) with the range of= 0-0.
View Article and Find Full Text PDFWe report here the superconducting properties of a Laves phase superconductor SrIr, which has a cubic MgCu structure. SrIr is a type-II superconductor, with a T of 5.9 K.
View Article and Find Full Text PDFThe sensitivity and specificity of a new rapid Mycoplasma pneumoniae antigen immunochromatography (IC) test, DK-MP-001, were determined using particle agglutination (PA) antibody response and loop-mediated isothermal amplification (LAMP) gene detection as the gold standard. Of 165 patients, 59 were diagnosed with M. pneumoniae infection based on a ≥fourfold rise of serum PA antibody during the course of the illness.
View Article and Find Full Text PDFThe newly developed rapid diagnostic test (RDT, DK14-CA1, Denka Seiken Co., Ltd.) to detect Campylobacter antigen was evaluated using fecal specimens of patients with enteritis.
View Article and Find Full Text PDFWe report the comprehensive studies between synchrotron X-ray diffraction, electrical resistivity and magnetic susceptibility experiments for the iron arsenides Ca(FePt)PtAs for n = 2 and 3. Both structures crystallize in the monoclinic space group P2/m (#11) with three-dimensional FeAs structures. The horizontal FeAs layers are bridged by inclined FeAs planes through edge-sharing FeAs5 square pyramids, resulting in triangular tunneling structures rather than the simple layered structures found in conventional iron arsenides.
View Article and Find Full Text PDFTo understand the nematicity in Fe-based superconductors, nontrivial k dependence of the orbital polarization [ΔE_{xz}(k), ΔE_{yz}(k)] in the nematic phase, such as the sign reversal of the orbital splitting between Γ and X, Y points in FeSe, provides significant information. To solve this problem, we study the spontaneous symmetry breaking with respect to the orbital polarization and spin susceptibility self-consistently. In FeSe, due to the sign-reversing orbital order, the hole and electron pockets are elongated along the k_{y} and k_{x} axes, respectively, consistently with experiments.
View Article and Find Full Text PDFWe report peculiar momentum-dependent anisotropy in the superconducting gap observed by angle-resolved photoemission spectroscopy in BaFe2(As(1-x)P(x))2 (x = 0.30, Tc = 30 K). Strongly anisotropic gap has been found only in the electron Fermi surface while the gap on the entire hole Fermi surfaces are nearly isotropic.
View Article and Find Full Text PDFThe isostructural transition in the tetragonal phase with a sizable change in the anion height, is realized in heavily H-doped LaFeAsO and (La,P) codoped CaFe2As2. In these compounds, the superconductivity with higher Tc (40-50 K) is realized near the isostructural transition. To find the origin of the anion-height instability and the role in realizing the higher-Tc state, we develop the orbital-spin fluctuation theory by including the vertex correction.
View Article and Find Full Text PDFMotivated by the nematic electronic fluid phase in Sr(3)Ru(2)O(7), we develop a combined scheme of the renormalization-group method and the random-phase-approximation-type method, and analyze orbital susceptibilities of the (d(xz), d(yz))-orbital Hubbard model with high accuracy. It is confirmed that the present model exhibits a ferro-orbital instability near the magnetic or superconducting quantum criticality, due to the Aslamazov-Larkin-type vertex corrections. This mechanism of orbital nematic order presents a natural explanation for the nematic order in Sr(3)Ru(2)O(7), and is expected to be realized in various multiorbital systems, such as Fe-based superconductors.
View Article and Find Full Text PDFWe study the mechanism of orbital or spin fluctuations due to multiorbital Coulomb interaction in iron-based superconductors, going beyond the random-phase approximation. For this purpose, we develop a self-consistent vertex correction (VC) method, and find that multiple orbital fluctuations in addition to spin fluctuations are mutually emphasized by the "multimode interference effect" described by the VC. Then, both antiferro-orbital and ferro-orbital (=nematic) fluctuations simultaneously develop for J/U~0.
View Article and Find Full Text PDFIn iron pnictides, we find that the moderate electron-phonon interaction due to the Fe-ion oscillation can induce the critical d-orbital fluctuations, without being prohibited by the Coulomb interaction. These fluctuations give rise to the strong pairing interaction for the s-wave superconducting (SC) state without sign reversal (s(++)-wave state), which is consistent with experimentally observed robustness of superconductivity against impurities. When the magnetic fluctuations due to Coulomb interaction are also strong, the SC state shows a smooth crossover from the s-wave state with sign reversal (s(+/-)-wave state) to the s(++)-wave state as impurity concentration increases.
View Article and Find Full Text PDFBased on the five-orbital model, we study the effect of local impurity in iron pnictides, and find that the interband impurity scattering is promoted by the d-orbital degree of freedom. This fact means that the fully gapped sign-reversing s-wave state, which is predicted by spin fluctuation theories, is very fragile against impurities. In the BCS theory, only 1% impurities with intermediate strength induce huge pair breaking, resulting in the large in-gap state and prominent reduction in Tc, contrary to the prediction based on simple orbital-less models.
View Article and Find Full Text PDFFor a newly discovered iron-based high T_{c} superconductor LaFeAsO1-xFx, we have constructed a minimal model, where inclusion of all five Fe d bands is found to be necessary. The random-phase approximation is applied to the model to investigate the origin of superconductivity. We conclude that the multiple spin-fluctuation modes arising from the nesting across the disconnected Fermi surfaces realize an extended s-wave pairing, while d-wave pairing can also be another candidate.
View Article and Find Full Text PDFWe analyze the origin of the three-dimensional (3D) magnetism observed in nonhydrated Na-rich Na(x)CoO2 within an itinerant spin picture using a 3D Hubbard model. The origin is identified as the 3D nesting between the inner and outer portions of the Fermi surface, which arise due to the local minimum structure of the a(1g) band at the Gamma-A line. The calculated spin wave dispersion strikingly resembles the neutron scattering result.
View Article and Find Full Text PDFIn order to probe the effect of charge fluctuations on triplet pairing, we study the pairing symmetry in the one-band Hubbard model having the off-site Coulomb repulsion (V) on top of the on-site repulsion as a model for the gamma band of Sr2RuO4, a strong candidate for a triplet pairing superconductor. The result, obtained with the dynamical cluster approximation combined with the quantum Monte Carlo method, and confirmed from the fluctuation exchange approximation, shows that while d(x(2)-y(2)) pairing dominates over p in the absence of V, introduction of V makes p(x+y) and d(xy) dominant. The gap function for the chiral p(x+y)+ip(x-y) has nodes that are consistent with the recent measurement of specific heat in rotated magnetic fields in the ruthenate.
View Article and Find Full Text PDFPhys Rev B Condens Matter
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