Absorbed doses determined with a sealed water calorimeter operated at 4 degrees C are compared with the results obtained using ionization chambers and the IAEA TRS-398 code of practice in a 10 MV photon beam (TPR(20,10) = 0.734) and a 175 MeV proton beam (at a depth corresponding to the residual range, R(res) = 14.7 cm).
View Article and Find Full Text PDFJ Res Natl Inst Stand Technol
July 2016
In a recent publication, we used a reaction model (model III) to calculate the heat defect for the irradiation of aqueous solutions with ionizing radiation at 21 °C. Subsequent work has revealed that the literature value used for one of the rate constants in the model was incorrect. A revised model (model IIIR) incorporates the correct rate constant for 21 °C.
View Article and Find Full Text PDFDomen developed a sealed water calorimeter at NIST to measure absorbed dose to water from ionizing radiation. This calorimeter exhibited anomalous behavior using water saturated with gas mixtures of H and O. Using computer simulations of the radiolysis of water, we show that the observed behavior can be explained if, in the gas mixtures, the amount-of-substance of H and of O differed significantly from 50 %.
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