We report experimental results on the temperature-dependent phase-matching properties of for second-harmonic generation and sum-frequency generation in the 0.7674-10.5910 µm range.
View Article and Find Full Text PDFThis paper reports on new experimental results on the temperature-dependent phase-matching properties of LiGaS for second-harmonic generation and sum-frequency generation in the 0.820-10.5910 μm spectral range.
View Article and Find Full Text PDFFemtosecond time-resolved mid-infrared (MIR) spectroscopy based on chirped-pulse upconversion is a promising method for observing molecular vibrational dynamics. A quantitative study on nonlinear media for upconversion is still essential for wide applications, particularly at the frequencies below 2000 cm. We evaluate wide-bandgap nonlinear crystals of Li-containing ternary chalcogenides based on their performance as the upconversion medium for femtosecond MIR spectroscopy.
View Article and Find Full Text PDFWe report new experimental results on the phase-matching properties of yellow color HgGaS crystals for harmonic generation of an Nd:YAG laser-pumped KTiOPO (KTP) optical parametric oscillator (OPO) and CO lasers in the 0.944-10.5910 μm range.
View Article and Find Full Text PDFThis paper reports on improved Sellmeier and thermo-optic dispersion formulas for LiInS, which provide an excellent reproduction of the temperature-dependent phase-matching conditions for second, sum-, and difference-frequency generation achieved in the 1.0642-10.5910 μm range.
View Article and Find Full Text PDFThis paper reports the high-accuracy Sellmeier and thermo-optic dispersion formulas for the extraordinary ray of 5 mol. % MgO-doped congruent LiNbO(3) that provide excellent reproduction of the temperature-dependent quasi-phase-matching conditions in the 0.39-4.
View Article and Find Full Text PDFThis paper reports on the improved Sellmeier and thermo-optic dispersion formulas for LiInSe₂, which provide a good reproduction of the temperature-dependent phase-matching conditions for the nonlinear frequency-conversion experiments achieved in the 1.0642-10.5910 μm range.
View Article and Find Full Text PDFThis paper reports high-accuracy Sellmeier and thermo-optic dispersion formulas for GaSe that provide excellent reproduction of the phase-matching conditions for second-, third-, and fourth- harmonic generation of CO2 laser radiation at 10.5910 μm in the 20°C-200°C range as well as the data points of Feng et al. [Opt.
View Article and Find Full Text PDFThe Sellmeier equations for GaS and GaSe are constructed from the nonlinear experiments thus far reported in the literature. The model calculations based on these equations were found to reproduce well the phase-matching conditions for second-harmonic generation of the Er:YSGG laser at 2.7960 μm and the CO2 laser lines at 9.
View Article and Find Full Text PDFBiB3O6 has been found to be simultaneously phase matchable for sum-frequency generation at 0.4627 and 0.6260 microm by mixing the outputs of a 0.
View Article and Find Full Text PDFThird-harmonic generation (THG) has been investigated in the monoclinic BiB(3)O(6). The symmetry and birefringence analysis revealed that there are phase-matching conditions for the direct third-order nonlinear process, where the cascading second-order processes are precluded by the zero effective nonlinearity. The first phase-matched pure chi((3)) THG in a noncentrosymmetric crystal is presented together with the improved Sellmeier and thermo-optic dispersion formulas.
View Article and Find Full Text PDFGdCa4O(BO3)3 has been found to have phase-matching points where the temperature variations of the phase-matching angles become zero for type-1 sum-frequency generation in the zx plane. We also found that the temperature sensitivities of the phase-matching conditions in the zx plane are different along the phi = 0 degrees and phi = 180 degrees directions in this material. In addition, the thermo-optic dispersion formula of this material that reproduces the temperature phase-matching properties of GdCa4O(BO3)3 and Gd(x)Y(1-x)Ca4O(BO3)3 is presented.
View Article and Find Full Text PDFK2Al2B2O7 has been found to be phase matchable for type-1 sum-frequency generation (SFG) at 0.193 microm by mixing the Nd:YAG laser wavelength at 1.0642 microm and the SFG output of the RbTiOAsO4 optical parametric oscillator tuned at 0.
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