Direct observation of a few-photon phase shift induced by a single quantum emitter in a waveguide.

Realizing a sensitive photon-number-dependent phase shift on a light beam is required both in classical and quantum photonics. It may lead to new applications for classical and quantum photonics machine learning or pave the way for realizing photon-photon gate operations. Nonlinear phase-shifts require efficient light-matter interaction, and recently quantum dots coupled to nanophotonic devices have enabled near-deterministic single-photon coupling.

Reconfigurable quantum photonic circuits based on quantum dots.

Quantum photonic integrated circuits, composed of linear-optical elements, offer an efficient way for encoding and processing quantum information on-chip. At their core, these circuits rely on reconfigurable phase shifters, typically constructed from classical components such as thermo- or electro-optical materials, while quantum solid-state emitters such as quantum dots are limited to acting as single-photon sources. Here, we demonstrate the potential of quantum dots as reconfigurable phase shifters.

Independent Electrical Control of Two Quantum Dots Coupled through a Photonic-Crystal Waveguide.

Efficient light-matter interaction at the single-photon level is of fundamental importance in emerging photonic quantum technology. A fundamental challenge is addressing multiple quantum emitters at once, as intrinsic inhomogeneities of solid-state platforms require individual tuning of each emitter. We present the realization of two semiconductor quantum dot emitters that are efficiently coupled to a photonic-crystal waveguide and individually controllable by applying a local electric Stark field.

Integrated Whispering-Gallery-Mode Resonator for Solid-State Coherent Quantum Photonics.

Tailored photonics cavities enhance light-matter interactions, ultimately enabling a fully coherent quantum interface. Here, we report an integrated microdisk cavity containing self-assembled quantum dots to coherently route photons between different access waveguides. We measure a Purcell factor of = 6.

Experimental Reconstruction of the Few-Photon Nonlinear Scattering Matrix from a Single Quantum Dot in a Nanophotonic Waveguide.

Coherent photon-emitter interfaces offer a way to mediate efficient nonlinear photon-photon interactions, much needed for quantum information processing. Here we experimentally study the case of a two-level emitter, a quantum dot, coupled to a single optical mode in a nanophotonic waveguide. We carry out few-photon transport experiments and record the statistics of the light to reconstruct the scattering matrix elements of one- and two-photon components.

Quantum Optics with Near-Lifetime-Limited Quantum-Dot Transitions in a Nanophotonic Waveguide.

Establishing a highly efficient photon-emitter interface where the intrinsic linewidth broadening is limited solely by spontaneous emission is a key step in quantum optics. It opens a pathway to coherent light-matter interaction for, e.g.

Core-Shell Plasmonic Nanohelices.

We introduce core-shell plasmonic nanohelices, highly tunable structures that have a different response in the visible for circularly polarized light of opposite handedness. The glass core of the helices is fabricated using electron beam induced deposition and the pure gold shell is subsequently sputter coated. Optical measurements allow us to explore the chiral nature of the nanohelices, where differences in the response to circularly polarized light of opposite handedness result in a dissymmetry factor of 0.

Chip-Based All-Optical Control of Single Molecules Coherently Coupled to a Nanoguide.

The feasibility of many proposals in nanoquantum-optics depends on the efficient coupling of photons to individual quantum emitters, the possibility to control this interaction on demand, and the scalability of the experimental platform. To address these issues, we report on chip-based systems made of one-dimensional subwavelength dielectric waveguides (nanoguides) and polycyclic aromatic hydrocarbon molecules. We discuss the design and fabrication requirements, present data on extinction spectroscopy of single molecules coupled to a nanoguide mode, and show how an external optical beam can switch the propagation of light via a nonlinear optical process.

Small slot waveguide rings for on-chip quantum optical circuits.

Nanophotonic interfaces between single emitters and light promise to enable new quantum optical technologies. Here, we use a combination of finite element simulations and analytic quantum theory to investigate the interaction of various quantum emitters with slot-waveguide rings. We predict that for rings with radii as small as 1.

Harmonics Generation by Surface Plasmon Polaritons on Single Nanowires.

We present experimental observations of visible wavelength second- and third-harmonic generation on single plasmonic nanowires of variable widths. We identify that near-infrared surface plasmon polaritons, which are guided along the nanowire, act as the source of the harmonics generation. We discuss the underlying mechanism of this nonlinear process, using a combination of spatially resolved measurements and numerical simulations to show that the visible harmonics are generated via a combination of both local and propagating plasmonic modes.

Modal symmetries at the nanoscale: a route toward a complete vectorial near-field mapping.

We use symmetry considerations to understand and unravel near-field measurements, ultimately showing that we can spatially map three distinct fields using only two detectors. As an example, we create 2D field maps of the out-of-plane magnetic field and two in-plane fields for a silicon ridge waveguide. Furthermore, we are able to identify and remove polarization mixing of less than 1/30 of our experimental signals.

Ultracompact (3 μm) silicon slow-light optical modulator.

Wavelength-scale optical modulators are essential building blocks for future on-chip optical interconnects. Any modulator design is a trade-off between bandwidth, size and fabrication complexity, size being particularly important as it determines capacitance and actuation energy. Here, we demonstrate an interesting alternative that is only 3 μm long, only uses silicon on insulator (SOI) material and accommodates several nanometres of optical bandwidth at 1550 nm.

Unravelling nonlinear spectral evolution using nanoscale photonic near-field point-to-point measurements.

We demonstrate nanoscale photonic point-to-point measurements characterizing a single component inside an all-optical signal-processing chip. We perform spectrally resolved near-field scanning optical microscopy on ultrashort pulses propagating inside a slow light photonic crystal waveguide, which is part of a composite sample. A power study reveals a reshaping of the pulse's spectral density, which we model using the nonlinear Schrödinger equation.

Ultrafast tunable optical delay line based on indirect photonic transitions.

We introduce the concept of an indirect photonic transition and demonstrate its use in a dynamic delay line to alter the group velocity of an optical pulse. Operating on an ultrafast time scale, we show continuously tunable delays of up to 20 ps, using a slow light photonic crystal waveguide only 300 μm in length. Our approach is flexible, in that individual pulses in a pulse stream can be controlled independently, which we demonstrate by operating on pulses separated by just 30 ps.

All-optical ultrafast control of beaming through a single sub-wavelength aperture in a metal film.

We propose an ultrafast all-optical technique to control and beam the light emerging from a sub-wavelength slit in a planar gold film by exciting a transient grating in the area around the slit. A FDTD model is used to show how excitation of surface plasmon polaritons by the grating governs the beaming process. Both the grating and the beaming effect are shown to decay on a picosecond time-scale.

Ultrafast silicon-based active plasmonics at telecom wavelengths.

Using a gold/silicon grating coupler and modulating the silicon dielectric constant with 775 nm, 800 fs pump pulses we demonstrate an ultrafast spectral shift to a surface plasmon polariton coupling resonance for 1300-1700 nm probe pulses. With a modest pump fluence of 2.2 mJ cm(-2) the pump-induced free carriers shift the resonance by more than its width, with recovery occurring in 103 ps due to surface recombination.

Ultrafast all-optical coupling of light to surface plasmon polaritons on plain metal surfaces.

We propose and demonstrate an ultrafast all-optical method to couple light to surface plasmon polaritons on planar gold films. By interfering two 150 fs, 810 nm pulses we excite a transient grating in the temperature of the free electrons of the metal, resulting in a grating in the dielectric function, and leading to a 1 ps launch window for plasmonic excitation. We use pump-probe experiments to identify these ultrashort plasmonic excitations between 520 and 570 nm.

Ultrafast control of grating-assisted light coupling to surface plasmons.

We demonstrate subpicosecond control over the coupling of free-space radiation to surface-plasmon polaritons using 830 and 500 nm period gold gratings. Thermal changes to the electron distribution following irradiation by 100 fs, 810 nm pulses produce a shift of the 570 nm plasmon resonance by approximately 0.75 nm with reflectivity change up to 6% and decay time of approximately 1 ps.