Second-harmonic optical spectroscopy on split-ring-resonator arrays.

Previous second-harmonic-generation experiments on metallic split-ring-resonator arrays have been performed at fixed fundamental laser center frequency. Here, we perform nonlinear optical spectroscopy on a first set of samples, revealing pronounced resonances. Furthermore, to clarify the role of higher-order split-ring resonances, we perform additional experiments on a second set of samples in which the fundamental split-ring-resonator resonance frequencies are lithographically tuned, whereas the higher-order resonances are fixed.

Spectral imaging of individual split-ring resonators.

We report on spectral imaging within individual silver split-ring resonators (SRRs) operating in the near infrared-visible range. We classified the optical eigenmodes from the measurement of their energies and nanometer scale spatial distributions. They are plasmonic standing waves that show great similarities with that of nanoantennas.

Electromagnetic interaction of split-ring resonators: The role of separation and relative orientation.

Extinction cross-section spectra of split-ring-resonator dimers have been measured at near-infrared frequencies with a sensitive spatial modulation technique. The resonance frequency of the dimer's coupled mode as well as its extinction cross-section and its quality factor depend on the relative orientation and separation of the two split-ring resonators. The findings can be interpreted in terms of electric and magnetic dipole-dipole interaction.

Experiments on second- and third-harmonic generation from magnetic metamaterials.

Photonic metamaterials could provide optical nonlinearities far exceeding those of natural substances due to the combined action of (magnetic) resonances and local-field enhancements. Here, we present our experiments on second- and third-harmonic generation from magnetic metamaterials composed of nanoscale gold split-ring resonators and from control samples for excitation with 170-fs pulses centered at 1.5-microm wavelength.

Large-area magnetic metamaterials via compact interference lithography.

Magnetic metamaterials with magnetic-dipole resonances around 1.2-mum wavelength are fabricated using an extremely compact and robust version of two- or three-beam interference lithography for 1D and 2D structures, respectively. Our approach employs a single laser beam at 532- nm wavelength impinging onto a suitably shaped dielectric object (roof-top prism or pyramid) - bringing the complexity of fabricating magnetic metamaterials down to that of evaporating usual dielectric/metallic coatings.