We revisit and improve the optical heterodyne technique for the measurement of the laser coherence, by digital acquisition of the beat-note and numerical analysis of the resulting signal. Our main result is that with the same experimental setup we reach the very "short-time linewidth" with the highest accuracy as well as the frequency noise spectrum.
View Article and Find Full Text PDFWe have synthesised a new, pyrene-based, low-molecular-mass, amphiphilic molecule that displays a wealth of properties of potential interest for aggregation and interfacial applications. In order to elucidate some of the key properties of this molecule, which consists of a pyrene-containing hydrophobic head and a short PEG-based hydrophilic tail, we investigate herein some aspects of its concentration-dependent behaviour in aqueous solutions. We show that the inclusion of the hydrophobic pyrene group not only provides the molecule with intriguing bulk and interfacial properties down to low concentrations, but also with various means of assessing its aggregation behaviour by means of its well-characterised fluorescence properties.
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