Mechanically robust, flexible, conductive, and anti-freezing hydrogels reinforced by cellulose of wood skeleton.

Hydrogels are soft and wet materials, but their applications are always limited by insufficient mechanical strength and toughness, and they are prone to freezing at low temperatures. In this study, we introduced an eco-friendly approach to developing wood-based hydrogels reinforced by the naturally aligned wood skeleton (WS) through the Hofmeister effect. The resulting wood-based composite hydrogels exhibited a high tensile strength of 20 MPa and a strain of 35 % in the longitudinal direction.

Initiatorless polymerization of mechanically robust hydrogels reinforced by cellulose of wood skeleton as multifunctional sensors.

Wood-based hydrogel with a unique anisotropic structure is an attractive soft-and-wet material. However, it remains a challenge to simultaneously achieve robust, multi-functional, and multi-response integrations through a sustainable and green approach. Herein, a bioinspired, additive-free method is reported to fabricate composite hydrogels reinforced by naturally high-strength wood skeleton without using any chemical initiators and crosslinking agents.