Publications by authors named "Minxia Shen"

Ultrafine particles play a crucial role in understanding climate change, mitigating adverse health effects, and developing strategies for air pollution control. However, the factors influencing the occurrence and development of new particle formation (NPF) events, as well as the underlying chemical mechanisms, remain inadequately explained. This study compared number concentrations and size distributions of atmospheric ultrafine particles at Xi'an (urban area) and the summit of Mt.

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Article Synopsis
  • The acidity of aerosol and cloud water impacts human health, ecosystems, and climate, and varies by region, with the Guanzhong Plain in China showcasing unique influences from human emissions and natural components.* -
  • In this study, cloud water collected at high altitude (Mt. Hua) was found to be alkaline (pH 7.6), contrasting with more acidic particulate matter (pH 3.2), suggesting a need to reconsider previous assumptions about cloud acidity and pollution.* -
  • The research highlighted that while sulfate (SO) is prevalent in particulate matter, its concentration diminishes in cloud water, with an increase in nitrate (NO) and ammonium (NH), and identified a large presence of dicar
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Oxygenated volatile organic compounds (OVOCs) play important roles in tropospheric chemistry, regulating the oxidation capacity and ozone (O) formation potential of the atmosphere. However, the evolution of OVOCs composition during vertical transport from the near surface to the upper atmosphere layer and the roles of OVOCs in the alpine atmospheric O formation are still poorly understood. In this study, we investigated the carbonyl compounds, the most important chemical group of OVOCs, and other gaseous pollutants simultaneously collected at the top (2060 m a.

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Aerosol pH is not only a diagnostic indicator of secondary aerosol formation, but also a key factor in the specific chemical reaction routes that produce sulfate and nitrate. To understand the characteristics of aerosol acidity in the Mt. Hua, the chemical fractions of water-soluble inorganic ions in the atmospheric PM and size-resolved particle at the top and foot of Mt.

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Glyoxal and methylglyoxal are important volatile organic compounds in the atmosphere. The gas-particle partitioning of these carbonyl compounds makes significant contributions to O formation. In this study, both the gas- and particle-phase glyoxal and methylglyoxal concentrations at the foot and top of Mount Hua were determined simultaneously.

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  • * A study conducted on Mount Hua during summer 2020 measured the distribution and carbon isotopic compositions of these acids at different altitudes, finding higher concentrations at the foot of the mountain due to human emissions.
  • * Oxalic acid was the most prevalent dicarboxylic acid detected, with significant evidence suggesting that anthropogenic sources contribute more to the compounds found in particulate matter than natural sources, and that these compounds can impact atmospheric conditions even at high altitudes.
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Dicarboxylic acids are one of the important water-soluble organic compounds in atmospheric aerosols, causing adverse effects to both climate and human health. More attention has therefore been paid to organic acids in aerosols. In this study, the molecular distribution and diurnal variations of wintertime dicarboxylic acids in a rural site of Guanzhong Plain, Northwest China, were explored.

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In this study, 30 elements in fine particulate matter (PM) were measured in 18 Chinese cities in 2013. Elemental pollution in northern, southwest, and central China were severe, attributing to excessive coal and biomass combustion in these regions. The concentrations of S, Cl, and K in these areas were 8.

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  • The study examined the effects of cooking activities on indoor air quality in various commercial restaurants in Northwestern China, focusing on chemical pollutants like airborne carbonyls, PAHs, and heavy metals during winter with low ventilation from December 2011 to January 2012.
  • The Chinese Barbecue restaurant had the highest total airborne carbonyl concentration, while Indian restaurants showed the greatest per capita carbonyl release, attributed to cooking practices that use high-heat methods.
  • The findings indicate significant health risks due to hazardous substances, including high levels of lead and nickel, alongside the formation of reactive organic species, raising concerns about the safety of indoor dining environments.
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Based on the enhancing effect of chitosan (CS) on luminol-dissolved oxygen chemiluminescence (CL) reaction, a flow injection (FI) luminol-CS CL system was established. It was found that the increase of CL intensity was proportional to the concentrations of CS ranging from 0.7 to 10.

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