Time-resolving state-specific molecular dissociation with XUV broadband absorption spectroscopy.

The electronic and nuclear dynamics inside molecules are essential for chemical reactions, where different pathways typically unfold on ultrafast timescales. Extreme ultraviolet (XUV) light pulses generated by free-electron lasers (FELs) allow atomic-site and electronic-state selectivity, triggering specific molecular dynamics while providing femtosecond resolution. Yet, time-resolved experiments are either blind to neutral fragments or limited by the spectral bandwidth of FEL pulses.

Potential hazards and mitigation of X-ray radiation generated by laser-induced plasma from research-grade laser systems.

A large range of laser-matter applications employ ultrashort pulses and high laser intensity. Such processes can lead to unrequired X-ray generation, which represents a hazardous radiation factor even for common laboratory research-grade laser systems. We present here an analysis of the radiation dose rate and X-ray spectrum emitted during ablation of a rotating copper cylinder with respect to several laser parameters.

4D spatio-temporal electric field characterization of ultrashort light pulses undergoing filamentation.

We present an experimental method capable of capturing the complete spatio-temporal dynamics of filamenting ultrashort laser pulses. By employing spatially resolved Fourier transform spectrometry in combination with the capability to terminate the filament at any length, we can follow the nonlinear dynamics in four dimensions, i.e.

Self-probed ptychography from semiconductor high-harmonic generation.

We demonstrate a method to image an object using a self-probing approach based on semiconductor high-harmonic generation. On the one hand, ptychography enables high-resolution imaging from the coherent light diffracted by an object. On the other hand, high-harmonic generation from crystals is emerging as a new source of extreme-ultraviolet ultrafast coherent light.

X-ray Dose Rate and Spectral Measurements during Ultrafast Laser Machining Using a Calibrated (High-Sensitivity) Novel X-ray Detector.

Ultrashort pulse laser machining is subject to increase the processing speeds by scaling average power and pulse repetition rate, accompanied with higher dose rates of X-ray emission generated during laser-matter interaction. In particular, the X-ray energy range below 10 keV is rarely studied in a quantitative approach. We present measurements with a novel calibrated X-ray detector in the detection range of 2-20 keV and show the dependence of X-ray radiation dose rates and the spectral emissions for different laser parameters from frequently used metals, alloys, and ceramics for ultrafast laser machining.

A synchronized VUV light source based on high-order harmonic generation at FLASH.

Ultrafast measurements in the extreme ultraviolet (XUV) spectral region targeting femtosecond timescales rely until today on two complementary XUV laser sources: free electron lasers (FELs) and high-harmonic generation (HHG) based sources. The combination of these two source types was until recently not realized. The complementary properties of both sources including broad bandwidth, high pulse energy, narrowband tunability and femtosecond timing, open new opportunities for two-color pump-probe studies.

Author Correction: All semiconductor enhanced high-harmonic generation from a single nanostructured cone.

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

Generating Ultrabroadband Deep-UV Radiation and Sub-10 nm Gap by Hybrid-Morphology Gold Antennas.

We experimentally investigate the interaction between hybrid-morphology gold optical antennas and a few-cycle Ti:sapphire laser up to ablative intensities, demonstrating rich nonlinear plasmonic effects and promising applications in coherent frequency upconversion and nanofabrication technology. The two-dimensional array of hybrid antennas consists of elliptical apertures combined with bowties in its minor axis. The plasmonic resonance frequency of the bowties is red-shifted with respect to the laser central frequency and thus mainly enhances the third harmonic spectrum at long wavelengths.

All semiconductor enhanced high-harmonic generation from a single nanostructured cone.

The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next generation petahertz optoelectronic devices or compact all solid state EUV sources. Here, we report on the realization of the first nanoscale high harmonic source.

Nano-plasmonic near field phase matching of attosecond pulses.

Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field.

Few-cycle optical pulse characterization via cross-polarized wave generation dispersion scan technique.

We demonstrate a dispersion scan (d-scan) pulse characterization scheme employing cross-polarized wave (XPW) generation as a nonlinear optical process. XPW generation is a degenerate four-wave mixing process with no phase-matching limitations. Therefore, its implementation in the d-scan method is a good choice for the characterization of few-cycle pulses in remote spectral regions.

Direct observation of pulse dynamics and self-compression along a femtosecond filament.

We report on the direct experimental observation of pulse-splitting dynamics along a femtosecond filament. The fundamental pulse experiences a significant self-shortening during the propagation leading to pulse durations of 5.3 fs, corresponding to sub-3 cycles, which is measured without external pulse compression.

Sub-1.5-cycle pulses from a single filament.

The temporal dynamics of ultrashort laser pulses undergoing filamentary propagation are investigated with a real-time stereographic above-threshold ionization (ATI) phasemeter. The experimental setup is capable of measuring the pulse duration as well as the carrier-envelope phase distribution of pulses originating from a femtosecond filament, which is either truncated in length or fully propagated. Truncation, by means of a semi-infinite gas cell, allows to elucidate the nonlinear evolution and temporal dynamics of ultrashort laser pulses as a function of the propagation length.

Gradient enhanced third harmonic generation in a femtosecond filament.

The third harmonic generated during femtosecond filamentation in air is studied. By establishing a gradient from atmospheric pressure to vacuum conditions, we truncate the filament abruptly at defined positions. The introduction of the pressure gradient leads to an enhancement of the generated third harmonic radiation by 3 orders of magnitude.

Tracking spectral shapes and temporal dynamics along a femtosecond filament.

The spectral evolution of a high-intensity light channel formed by filamentation is investigated in a detailed experimental study. We also track the spatio-temporal dynamics by high-order harmonic generation along the filament. Both the spectral and temporal diagnostics are performed as a function of propagation distance, by extracting the light pulses directly from the hot filament core into vacuum via pinholes that terminate the nonlinear propagation.

Generation of high-order harmonics with ultra-short pulses from filamentation.

7-fs-pulses with 0.3 mJ are obtained after filamentation in argon and compression by double-chirped-mirrors. These pulses are used to generate high-order harmonics in a semi-infinite gas cell in different noble gases.

Microjoule pulse energy from a chirped-pulse Ti:sapphire oscillator with cavity dumping.

We demonstrate a chirped-pulse Ti:sapphire laser oscillator with both Kerr-lens and semiconductor- saturable-absorber-mirror-assisted mode locking generating 1.1 microJ pulses at 1 MHz pulse repetition rate. The pulses are coupled out of the laser cavity by means of an acousto-optical cavity dumper, have a spectral width that supports a Fourier limit of 74 fs, and currently have a chirped-pulse duration of 5 ps.