Optics miniaturization strategy for demanding Raman spectroscopy applications.

Raman spectroscopy provides non-destructive, label-free quantitative studies of chemical compositions at the microscale as used on NASA's Perseverance rover on Mars. Such capabilities come at the cost of high requirements for instrumentation. Here we present a centimeter-scale miniaturization of a Raman spectrometer using cheap non-stabilized laser diodes, densely packed optics, and non-cooled small sensors.

Quartz-Enhanced Photoacoustic Spectroscopy Assisted by Partial Least-Squares Regression for Multi-Gas Measurements.

We report on the use of quartz-enhanced photoacoustic spectroscopy (QEPAS) for multi-gas detection. Photoacoustic (PA) spectra of mixtures of water (H2O), ammonia (NH3), and methane (CH4) were measured in the mid-infrared (MIR) wavelength range using a mid-infrared (MIR) optical parametric oscillator (OPO) light source. Highly overlapping absorption spectra are a common challenge for gas spectroscopy.

Accurate and fast identification of minimally prepared bacteria phenotypes using Raman spectroscopy assisted by machine learning.

The worldwide increase of antimicrobial resistance (AMR) is a serious threat to human health. To avert the spread of AMR, fast reliable diagnostics tools that facilitate optimal antibiotic stewardship are an unmet need. In this regard, Raman spectroscopy promises rapid label- and culture-free identification and antimicrobial susceptibility testing (AST) in a single step.

Two-colour high-purity Einstein-Podolsky-Rosen photonic state.

We report a high-purity Einstein-Podolsky-Rosen (EPR) state between light modes with the wavelengths separated by more than 200 nm. We demonstrate highly efficient EPR-steering between the modes with the product of conditional variances [Formula: see text]. The modes display - 7.

Quantum frequency conversion of vacuum squeezed light to bright tunable blue squeezed light and higher-order spatial modes.

Quantum frequency conversion, the process of shifting the frequency of an optical quantum state while preserving quantum coherence, can be used to produce non-classical light at otherwise unapproachable wavelengths. We present experimental results based on highly efficient sum-frequency generation (SFG) between a vacuum squeezed state at 1064 nm and a tunable pump source at 850 nm ± 50 nm for the generation of bright squeezed light at 472 nm ± 4 nm, currently limited by the phase-matching of the used nonlinear crystal. We demonstrate that the SFG process conserves part of the quantum coherence as a 4.

Isotopic gas analysis by means of mid-infrared photoacoustic spectroscopy targeting human exhaled air.

There is a great need for cost-efficient non-invasive medical diagnostic tools for analyzing humanly exhaled air. Compared to present day methods, photoacoustic spectroscopy (PAS) can provide a compact and portable (bedside), sensitive and inexpensive solution. We demonstrate a novel portable photoacoustic spectroscopic platform for isotopic measurements of methane ().

Calibration of Quartz-Enhanced Photoacoustic Sensors for Real-Life Adaptation.

We report on the use of quartz-enhanced photoacoustic spectroscopy for continuous carbon-dioxide measurements in humid air over a period of six days. The presence of water molecules alters the relaxation rate of the target molecules and thus the amplitude of the photoacoustic signal. Prior to the measurements, the photoacoustic sensor system was pre-calibrated using CO mole fractions in the range of 0-10 (0-1000 ppm) and at different relative humidities between 0% and 45%, while assuming a model hypothesis that allowed the photoacoustic signal to be perturbed linearly by HO content.

Intrinsic Spectral Resolution Limitations of QEPAS Sensors for Fast and Broad Wavelength Tuning.

Quartz-enhanced photoacoustic sensing is a promising method for low-concentration trace-gas monitoring due to the resonant signal enhancement provided by a high-Q quartz tuning fork. However, quartz-enhanced photoacoustic spectroscopy (QEPAS) is associated with a relatively slow acoustic decay, which results in a reduced spectral resolution and signal-to-noise ratio as the wavelength tuning rate is increased. In this work, we investigate the influence of wavelength scan rate on the spectral resolution and signal-to-noise ratio of QEPAS sensors.

Cavity-enhanced sum-frequency generation of blue light with near-unity conversion efficiency.

We report on double-resonant highly efficient sum-frequency generation in the blue range. The system consists of a 10-mm-long periodically poled KTP crystal placed in a double-resonant bow-tie cavity and pumped by a fiber laser at 1064.5 nm and a Ti:sapphire laser at 849.

Simple and robust speckle detection method for fire and heat detection in harsh environments.

Standard laser-based fire detection systems are often based on measuring the variation of optical signal amplitude. However, mechanical noise interference and loss from dust and steam can obscure the detection signal, resulting in faulty results or the inability to detect a potential fire. The presented fire detection technology will allow the detection of fire in harsh and dusty areas, which are prone to fires, where current systems show limited performance or are unable to operate.

Continuous-wave coherent Raman spectroscopy for improving the accuracy of Raman shifts.

Raman spectroscopy is an appealing technique that probes molecular vibrations in a wide variety of materials with virtually no sample preparation. However, accurate and reliable Raman measurements are still a challenge and require more robust and practical calibration methods. We demonstrate the implementation of a simple low-cost continuous-wave (cw) stimulated Raman spectroscopy scheme for accurate and high-resolution spectroscopy.

Versatile photoacoustic spectrometer based on a mid-infrared pulsed optical parametric oscillator.

We demonstrate the usefulness of a nanosecond-pulsed single-mode mid-infrared (MIR) optical parametric oscillator (OPO) for photoacoustic (PA) spectroscopic measurements. The maximum wavelength ranges for the signal and idler are 1.4 μm to 1.

Off-axis quartz-enhanced photoacoustic spectroscopy using a pulsed nanosecond mid-infrared optical parametric oscillator: publisher's note.

This publisher's note corrects an affiliation error in Opt. Lett.41, 4118 (2016)OPLEDP0146-959210.

Photo-acoustic sensor for detection of oil contamination in compressed air systems.

We demonstrate an online (in-situ) sensor for continuous detection of oil contamination in compressed air systems complying with the ISO-8573 standard. The sensor is based on the photo-acoustic (PA) effect. The online and real-time PA sensor system has the potential to benefit a wide range of users that require high purity compressed air.

Design and experimental verification of a photoacoustic flow sensor using computational fluid dynamics.

A photoacoustic (PA) sensor for fast and real-time gas sensing is demonstrated. The PA sensor is a stand-alone system controlled by a field-programmable gate array. The PA cell has been designed for flow noise immunity using computational fluid dynamics (CFD) analysis.

Compact and versatile laser system for polarization-sensitive stimulated Raman spectroscopy.

We demonstrate a compact and versatile laser system for stimulated Raman spectroscopy (SRS). The system is based on a tunable continuous wave (CW) probe laser combined with a home-built semi-monolithic nanosecond pulsed pump Nd:YVO laser at 1064 nm. The CW operation of the probe laser offers narrow linewidth, low noise and the advantage that temporal synchronization with the pump is not required.

All-optical detection of acoustic pressure waves with applications in photoacoustic spectroscopy.

An all-optical detection method for the detection of acoustic pressure waves is demonstrated. The detection system is based on a stripped (bare) single-mode fiber. The fiber vibrates as a standard cantilever and the optical output from the fiber is imaged to a displacement-sensitive optical detector.

Off-axis quartz-enhanced photoacoustic spectroscopy using a pulsed nanosecond mid-infrared optical parametric oscillator.

A trace-gas sensor, based on quartz-enhanced photoacoustic spectroscopy (QEPAS), consisting of two acoustically coupled micro-resonators (mR) with an off-axis 20 kHz quartz tuning fork (QTF) is demonstrated. The complete acoustically coupled mR system is optimized based on finite-element simulations and is experimentally verified. The QEPAS sensor is pumped resonantly by a nanosecond pulsed single-mode mid-infrared optical parametric oscillator.

Differential high-resolution stimulated CW Raman spectroscopy of hydrogen in a hollow-core fiber.

We demonstrate sensitive high-resolution stimulated Raman measurements of hydrogen using a hollow-core photonic crystal fiber (HC-PCF). The Raman transition is pumped by a narrow linewidth (< 50 kHz) 1064 nm continuous-wave (CW) fiber laser. The probe light is produced by a homebuilt CW optical parametric oscillator (OPO), tunable from around 800 nm to 1300 nm (linewidth ∼ 5 MHz).

A versatile integrating sphere based photoacoustic sensor for trace gas monitoring.

A compact versatile photoacoustic (PA) sensor for trace gas detection is reported. The sensor is based on an integrating sphere as the PA absorption cell with an organ pipe tube attached to increase the sensitivity of the PA sensor. The versatility and enhancement of the sensitivity of the PA signal is investigated by monitoring specific ro-vibrational lines of CO(2) in the 2 μm wavelength region and of NO(2) in the 405 nm region.

Gaussian error correction of quantum states in a correlated noisy channel.

Noise is the main obstacle for the realization of fault-tolerant quantum information processing and secure communication over long distances. In this work, we propose a communication protocol relying on simple linear optics that optimally protects quantum states from non-Markovian or correlated noise. We implement the protocol experimentally and demonstrate the near-ideal protection of coherent and entangled states in an extremely noisy channel.

Quantum-enhanced micromechanical displacement sensitivity.

We report on a hitherto unexplored application of squeezed light: for quantum-enhancement of mechanical transduction sensitivity in microcavity optomechanics. Using a toroidal silica microcavity, we experimentally demonstrate measurement of the transduced phase modulation signal in the frequency range 4-5.8 MHz with a sensitivity -0.

Continuous variable quantum key distribution with modulated entangled states.

Quantum key distribution enables two remote parties to grow a shared key, which they can use for unconditionally secure communication over a certain distance. The maximal distance depends on the loss and the excess noise of the connecting quantum channel. Several quantum key distribution schemes based on coherent states and continuous variable measurements are resilient to high loss in the channel, but are strongly affected by small amounts of channel excess noise.

Experimental investigation of the evolution of gaussian quantum discord in an open system.

Gaussian quantum discord is a measure of quantum correlations in gaussian systems. Using gaussian discord, we quantify the quantum correlations of a bipartite entangled state and a separable two-mode mixture of coherent states. We experimentally analyze the effect of noise addition and dissipation on gaussian discord and show that the former noise degrades the discord, while the latter noise for some states leads to an increase of the discord.

A novel method for polarization squeezing with Photonic Crystal Fibers.

Photonic Crystal Fibers can be tailored to increase the effective Kerr nonlinearity, while producing smaller amounts of excess noise compared to standard silicon fibers. Using these features of Photonic Crystal Fibers we create polarization squeezed states with increased purity compared to standard fiber squeezing experiments. Explicit we produce squeezed states in counter propagating pulses along the same fiber axis to achieve near identical dispersion properties.