Atmospheric mercury plays a crucial role in the biogeochemical cycle of mercury. This study conducted an intensive measurement of atmospheric mercury from 2015 to 2018 at a regional site in eastern China. During this period, the concentration of particle-bound mercury (PBM) decreased by 13%, which was much lower than those of gaseous elemenral mercury (GEM, 30%) and reactive gaseous mercury (GOM, 62%).
View Article and Find Full Text PDFA one-year observation of aerosols on a remote island was conducted and saccharides were applied to reveal the behaviors of organic aerosol in the East China Sea (ECS). The seasonal fluctuations of total saccharides were relatively small, with annual mean concentration of 64.82 ± 26.
View Article and Find Full Text PDFThe aim of this paper was to investigate the influence of Fe (III) on humification and free radicals evolution. The experimental data showed that the experimental group (CT) with Fe(SO) had a better degree of humification than the control group (CK). The humic substances (HS) content was 10% higher in CT (23.
View Article and Find Full Text PDFThe purpose of this paper was to explore the promotion of maleic anhydride on the polymerization of precursors into humus in composting, and analyze the changes of key functional enzymes. The results showed that the content of humus in the treatment group added maleic anhydride (MAH) was higher than that in the control check (CK). The decrease rate of humus precursor concentration of MAH was also higher than that of CK.
View Article and Find Full Text PDFWater soluble organic nitrogen (WSON) had great influences on the aerosol chemistry, hygroscopicity, marine primary productivity, as well as nitrogen biogeochemical cycles. Aerosol sampling was conducted over an offshore island in the East China Sea in four seasons of 2019, aiming to reveal the seasonal sources and secondary formation processes of marine WSON. The annual mean WSON concentration reached 1.
View Article and Find Full Text PDFThis study focused on how adding ionic liquids (IL) affects composting humification. During the warming and thermophilic phases, addition of IL increased precursors content, and increased the polymerization of humus (HS) at later stages. Furthermore, the final HS and humic acid (HA) content of experimental groups (T) groups 129.
View Article and Find Full Text PDFIn this study, the effect of Fe on the quinone redox cycling driving lignocellulosic degradation in composting systems was investigated. The results showed that the degradation rates of cellulose, hemicellulose, and lignin were higher in the experimental group (CT) with Fe(SO) addition than in the blank group (CK) (CT, 52.55 %, 45.
View Article and Find Full Text PDFThis study was the first to explore the effect of shell powder (SP) on lignin degradation and humus (HS) formation during composting. The results showed that the treatment group (T) with SP consumed more polyphenols, reducing sugar and amino acids than the control group (CK), especially the rate of reducing sugar consumption in T (50.61 %) was significantly higher than CK (28.
View Article and Find Full Text PDFIn this study, HCO was used as a co-substrate for cyanate metabolism to investigate its effect on nitrogen cycle in composting. The results showed that the carbamate content in experimental group (T) with HCO added was higher than that in control group (CP) during cooling period. Actinobacteria and Proteobacteria were the dominant phyla for cyanate metabolism, and the process was mediated by cyanase gene (cynS).
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