The physical and chemical treatment processes of leachate are not only costly but can also possibly produce harmful by products. Constructed wetlands (CW) has been considered a promising alternative technology for leachate treatment due to less demand for energy, economic, ecological benefits, and simplicity of operations. Various trends and approaches for the application of CW for leachate treatment have been discussed in this review along with offering an informatics peek of the recent innovative developments in CW technology and its perspectives.
View Article and Find Full Text PDFElectroautotrophic microbes at biocathodes in microbial electrolysis cells (MECs) can catalyze the hydrogen evolution reaction with low energy demand, facilitating long-term stable performance through specific and renewable biocatalysts. However, MECs have not yet reached commercialization due to a lack of understanding of the optimal microbial strains and reactor configurations for achieving high performance. Here, we critically analyze the criteria for the inocula selection, with a focus on the effect of hydrogenase activity and microbe-electrode interactions.
View Article and Find Full Text PDFHigh ammonia concentration in wastewater can hinder methane production rate in anaerobic digestion (AD)-microbial electrosynthesis systems (ADMES). To address this issue, a dual-chamber reactor was fabricated using an anion exchange membrane (AEM) to separate the dark-fermentation (DF) and ADMES process, preventing ammonia migration from the DF chamber to the ADMES chamber. As a result, the DF-ADMES achieved a high methane yield based on chemical oxygen demand (COD) of 0.
View Article and Find Full Text PDFMicrobial electrosynthesis (MES) presents a versatile approach for efficiently converting carbon dioxide (CO) into valuable products. However, poor electron uptake by the microorganisms from the cathode severely limits the performance of MES. In this study, a graphitic carbon nitride (g-CN)-metal-organic framework (MOF) i.
View Article and Find Full Text PDFBioresour Technol
October 2022
Biohythane, a balanced mixture of 10%-30% v/v of hydrogen and 70%-90% v/v of methane, could be the backbone of an all-purpose future energy supply. Recently, bioelectrochemical systems (BES) became a new sensation among environmental biotechnology processes with the potential to sustainably generate biohythane. Therefore, to unleash its full potential for scaling up, researchers are consistently improving microbial metabolic pathways, novel reactors, and electrode designs.
View Article and Find Full Text PDFA newly designed microbial electrochemical system (MES) with the addition of a baffle between the electrodes was integrated with the anaerobic digestion (AD) process for biogas upgradation. Novel MES configuration attained an increased methane production rate of 292.6 mL/L∙d and methane yield of 0.
View Article and Find Full Text PDFImplicit interaction of electroactive microbes with solid electrodes is an interesting phenomenon in nature, which supported development of bioelectrochemical systems (BESs), especially the microbial fuel cell (MFCs) for valorization of low-value waste streams into bioelectricity. Intriguingly, the metabolism of interacted microbes with electrode is affected by the microenvironment at electrodes, which influences the current response. For instance, when heavy metal ions (HMIs) are imposed in the medium, the current production decreases due to their intrinsic toxic effect.
View Article and Find Full Text PDFPerformance of methane-producing microbial electrochemical systems (MESs) is highly reliant on electron transfer efficiency from electrode to microorganisms and vice versa. In this study, magnetite nanoparticles were used as electron carriers to enhance extracellular electron transfer in single chamber MESs. The MES with magnetite exhibited the highest methane yield and current generation of 0.
View Article and Find Full Text PDFACS Appl Mater Interfaces
May 2018
A hydroxyl group containing new cardo diamine monomer was synthesized, namely 9,9-bis (hydroxy- (4'-amino(3-trifluoromethyl)biphenyl-4-oxy)-phenyl)-9H-fluorene (mixture of isomers, HAPHPF). HAPHPF, along with a sulfonated diamine monomer, 4,4'-diaminostilbene-2,2'-disulfonic acid (DSDSA), was used to prepare a series of new sulfonated copolyimides by polycondensation with 1,4,5,8-naphthalenetetracarboxylic dianhydride (NTDA). The degree of sulfonation (DS < 1) was adjusted by the feed ratio of DSDSA/HAPHPF and the copolymers were named as DHN-XX, where XX denotes the mole percentage of DSDSA (XX = 50, 60, and 70).
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