We demonstrate a sensor card with cholesteric liquid crystals (CLCs) for terahertz (THz) waves generated from a nonlinear crystal pumped by a table-top laser. A beam profile of the THz waves is successfully visualized as color change by the sensor card without additional electronic devices, power supplies, and connecting cables. Above the power density of 4.
View Article and Find Full Text PDFQuasi-monodisperse dielectric particles organized in a periodic hexagonal network on an aluminum surface are exploited numerically and experimentally as a single-layered near-perfect absorber in the terahertz regime. Of particular interest are titanium dioxide (TiO(2)) microspheres because of their large dielectric permittivity and isotropic shape leading to Mie resonances with insensitive polarization. Absorption higher than 80% at normal incidence covering two distinct ranges of frequencies is demonstrated experimentally.
View Article and Find Full Text PDFTransmission spectra of near-self-complementary metallic checkerboard patterns (MCPs) exhibit a drastic change when the metal squares are brought into contact with each other from a noncontact state. Transmission spectra of near-self-complementary samples, which are fabricated by printing technology, show rather gradual systematic change with changing the nominal metal square size while keeping the period because of randomness naturally introduced by the limited accuracy of the printer. The spectra have transmission-invariant frequencies, which means that the spectra are a superposition of two types of spectra, the ratio of which depends on the nominal square size.
View Article and Find Full Text PDFMicrostructures in nature are ultrafine and ordered in biological roles, which have attracted material scientists. Spirulina forms three-dimensional helical microstructure, one of remarkable features in nature beyond our current processing technology such as lithography in terms of mass-productivity and structural multiplicity. Spirulina varies its diameter, helical pitch, and/or length against growing environment.
View Article and Find Full Text PDFTerahertz (THz) transmission modulation through copper phthalocyanine (CuPc)-coated Si under various laser light irradiation conditions was investigated using THz time-domain spectroscopy. The charge carrier transfer from Si to CuPc is crucial for photo-induced metallization, and the thickness of the CuPc layer is a critical parameter for achieving high charge carrier density for metallization. Transmission through a split-ring resonator array metamaterial, fabricated on CuPc-coated Si, can be efficiently modulated by laser light irradiation.
View Article and Find Full Text PDFA stacked metal-dielectric hole array (SHA) containing rectangular holes whose shape gradually varies in-plane is proposed as a means of achieving wavefront control. The dependence of the transmitted phase on the frequency can be tuned by the hole shape, in particular the length of the sides that are normal to the incident polarization. The combination of periodic holes along the polarization direction and the gradual change in hole shape normal to the polarization direction produce an inclined wavefront for 1-dimensional beam steering.
View Article and Find Full Text PDFTransmission phase control is experimentally demonstrated using stacked metal-dielectric hole arrays with a two-dimensional geometric design. The transmission phase varies drastically with small frequency shifts due to structural resonances. Laterally propagating surface plasmon polaritons excited by the periodic hole array roughly determine the resonance frequency, whereas localized resonances in each hole determine the dispersion.
View Article and Find Full Text PDFWe present a frequency-domain electron spin resonance (ESR) measurement system using terahertz time-domain spectroscopy. A crossed polarizer technique is utilized to increase the sensitivity in detecting weak ESR signals of paramagnets caused by magnetic dipole transitions between magnetic sublevels. We demonstrate the measurements of ESR signal of paramagnetic copper(II) sulfate pentahydrate with uniaxial anisotropy of the g-factor under magnetic fields up to 10 T.
View Article and Find Full Text PDFWire-grid polarizer sheets in the terahertz region have been fabricated on flexible substrates by nanoimprint technology. They show an ideal polarization property in the terahertz frequency region, whereas the cost is very low. Since the wire pitch is far smaller than the wavelength, the effective medium theory agrees well with experimental results.
View Article and Find Full Text PDFWe present a reflection-type terahertz time-domain spectroscopic ellipsometry (THz-TDSE) technique for measuring the complex dielectric constants of thin-film materials without replacement of the sample. THz-TDSE provides complex dielectric constants from the ratio of the complex amplitude reflection coefficients between p- and s-polarized THz waves. The measured dielectric constants of doped GaAs thin films show good agreement with predictions of the Drude model, even though the film thickness is of the order of a tenth of the penetration depth of the THz waves.
View Article and Find Full Text PDFWe theoretically predicted the existence of an anomalous optical transmittance dip, which must be observed for a metamaterial structure with two metallic slabs with cut-through slit arrays of a constant period d under a normal incident condition. By changing the relative lateral displacement l between the two slabs, the dip frequency varies across that of a so-called Rayleigh-Wood's (RW) anomaly frequency. The mechanism of this anomaly is quite different from that of the RW anomaly and interpreted in terms of the interference between the propagating and evanescent waves.
View Article and Find Full Text PDFWe investigate characteristics and generation process of surface waves excited on a structured perfect conductor surface in order to clarify the mechanism of resonant transmission in metal hole arrays made of the perfect conductor. By using a metal hole array of kagome lattice, we can separate two modes excited on the perfect conductor surface; a surface wave and an edge mode. Our calculation based on finite-difference time-domain method provides a generation process of the edge mode and the surface wave that is responsible for the resonant transmission in metal hole arrays.
View Article and Find Full Text PDFWe have fabricated Fabry-Perot (FP) cavities in the THz region with a ZnTe crystal as a cavity layer by a simple stacking method. We observed more than a three times enhancement of the THz emission intensity in the FP cavities compared with the bare ZnTe crystal at the frequencies of the resonant modes and stopband edges. On the other hand, suppression of the THz emission occurs at frequencies in the stopband.
View Article and Find Full Text PDFThe absorption spectra of ceftazidime and its generic versions (Modacin, Mosyl, and Mobenzocin) have been measured by terahertz time domain spectroscopy (THz-TDS). Differences in the THz absorption were observed between the original and generic versions. The results show small, but significant differences in the states of ceftazidime hydrate between the original and generic versions.
View Article and Find Full Text PDFWe developed a high-repetition-rate optical delay line based on a micromirror array and galvanometer mirror for terahertz time-domain spectroscopy. The micromirror array is fabricated by using the x-ray lithographic technology. The measurement of terahertz time-domain waveforms with the new optical delay line is demonstrated successfully up to 25 Hz.
View Article and Find Full Text PDFThe characteristics of THz pulse radiation from argon clusters irradiated with intense femtosecond laser pulses have been investigated. The average power of the THz pulses radiated from argon clusters is approximately 40 times greater than that from argon gas. The enhancement of the THz radiation originates from large laser absorption by the clusters.
View Article and Find Full Text PDFWe fabricated a terahertz wire-grid polarizer consisting of a micrometer-pitch Al grating on a Si substrate by photolithography and wet etching. The ratio of TM and TE transmittances (extinction ratio) was over 35 dB at 0.5 THz.
View Article and Find Full Text PDFAbsorption spectra of polycrystalline L-, D-, and DL-tartaric acid have been measured by terahertz time domain spectroscopy (THz-TDS). Different absorption bands are observed for DL-tartaric acid and its enantiomers (L- and D-tartaric acid). This result shows that the THz-TDS can be used for distinguishing between DL-tartaric acid and enantiomers (L- and D-tartaric acid).
View Article and Find Full Text PDFWe have fabricated a three-contact photoconductive antenna for the polarization-sensitive detection of terahertz electromagnetic radiation. Taking into account all three photoconductive signal current components, this three-contact photoconductive antenna can measure the polarization state of pulsed THz radiation at an accuracy comparable to that achieved using the conventional method which employs a set of wire-grid polarizers. The three-contact photoconductive receiver may be useful for polarization-sensitive spectroscopy such as vibrational circular dichroism spectroscopy and ellipsometry in the THz frequency region.
View Article and Find Full Text PDFWe have measured the terahertz (THz) complex dielectric spectra of imidazolium ionic liquids by THz time-domain spectroscopy (THz-TDS) in the frequency range from 5 (0.15 THz) to 140 cm(-1) (4.2 THz).
View Article and Find Full Text PDFGeneration and modulation of circularly polarized terahertz electromagnetic radiation have been demonstrated by using a four-contact photoconductive antenna and a total-reflection Si prism. The quality of the circularly polarized terahertz pulsed radiation has been evaluated by using a polarization sensitive terahertz time-domain spectroscopy system. The characteristic of the dynamic modulation between the left and right circularly polarized states of the THz radiation is also evaluated.
View Article and Find Full Text PDFWe demonstrate frequency tuning of enhanced THz radiation transmitted through a two-dimensional metallic hole array (2D-MHA) by controlling the index of refraction of the medium filling the holes and adjacent to the 2D-MHA on one side. The medium is a nematic liquid crystal (NLC) and its index of refraction is varied using magnetically controlled birefringence of the NLC. With the NLC, the peak transmission frequency of the 2D-MHA shift to the red by 0.
View Article and Find Full Text PDFPhotoconductive (PC) antennas fabricated on InP bombarded with 180 keV protons of different dosages (InP:H+) all exhibit a useful bandwidth of about 30 THz, comparable to that of the LT-GaAs PC antenna. The peak signal current of the best InP: H+ device (dosage of 10;15 ions/cm;2) is slightly higher than that of the LT-GaAs one, while the signal-to-noise ratio (SNR) of the former is about half of that of the latter due to lower resistivity. This suggests that InP: H+ can be a good substrate for THz PC antennas with proper annealing and/or implantation recipe.
View Article and Find Full Text PDFThe polarization characteristics of a terahertz (THz) wave transmitted through two-dimensional (2-D) metallic photonic crystals (MPCs) are investigated. The 2-D MPCs studied in this paper are metal slabs perforated periodically with circular holes. We measured the polarization characteristics of the THz wave using a THz time-domain spectroscopic system with wire grid polarizers in the time and frequency domains.
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